Abstract.
We investigate non-equilibrium concentration fluctuations during the free diffusion of a colloidal suspension against pure water. We investigate Fe2O3 superparamagnetic nanocolloids with sizes between 1 and 10 nm by means of a shadowgraph apparatus to determine the mixture mass diffusion coefficient and kinematic viscosity. The experiments were performed in three distinct conditions: Experiment 1 is without any magnetic field; Experiment 2 with a vertical magnetic field; Experiment 3 after turning off the magnetic field. We found no correlation between the kinematic viscosity coefficient and the external magnetic field. Conversely, we found that the mass diffusion coefficient decreases in the presence of the external magnetic field and slowly rebounds after the magnetic field was turned off.
Graphical abstract
Similar content being viewed by others
References
J.M. Ortiz de Zárate, J.V. Sengers (Editors), Hydrodynamic Fluctuations in Fluids and Fluid Mixtures (Elsevier, Amsterdam, 2006)
A. Oprisan, S.A. Oprisan, A. Teklu, Appl. Opt. 49, 86 (2010)
A. Oprisan, A.L. Payne, Opt. Commun. 290, 100 (2013)
F. Croccolo, J. Ortiz de Zarate, J. Sengers, Eur. J. Phys. E 39, 125 (2016)
A. Oprisan, S.A. Oprisan, J.J. Hegseth, Y. Garrabos, C. Lecoutre, D. Beysens, Eur. Phys. J. E 38, 1 (2015)
D. Brogioli, A. Vailati, M. Giglio, Phys. Rev. E 61, R1 (2000)
P. Guenoun, F. Perrot, D. Beysens, Phys. Rev. Lett. 63, 1152 (1989)
S. Mazzoni, R. Cerbino, A. Vailati, M. Giglio, Ann. N. Y. Acad. Sci. 1077, 351 (2006)
P.N. Segre, R.W. Gammon, J.V. Sengers, Phys. Rev. E 47, 1026 (1993)
J.V. Sengers, J.M. Ortiz de Zárate, J. Non-Equilib. Thermodyn. 32, 319 (2007)
A. Oprisan, B. Bayley, S.A. Oprisan, J.J. Hegseth, Y. Garrabos, C. Lecoutre, D. Beysens, Proc. SPIE 7701, 77010W (2010)
A. Oprisan, S.A. Oprisan, B. Bayley, J.J. Hegseth, Y. Garrabos, C. Lecoutre-Chabot, D. Beysens, Phys. Rev. E 86, 061501 (2012)
P.N. Segre, J.V. Sengers, Physica A 198, 46 (1993)
A. Vailati, M. Giglio, Nature 390, 262 (1997)
J.M. Ortiz de Zárate, J.V. Sengers, J. Stat. Phys. 115, 1341 (2004)
F. Giavazzi, A. Vailati, Phys. Rev. E 80, 015303 (2009)
D. Brogioli, F. Croccolo, A. Vailati, Phys. Rev. E 94, 022142 (2016)
J.M. Ortiz de Zárate, J.A. Fornés, J.V. Sengers, Phys. Rev. E 74, 046305 (2006)
A. Vailati, R. Cerbino, S. Mazzoni, C.J. Takacs, D.S. Cannell, M. Giglio, Nat. Commun. 2, 290 (2011)
C. Giraudet, H. Bataller, Y. Sun, A. Donev, J.M.O. de Zárate, F. Croccolo, EPL 111, 60013 (2015)
J.M. Ortiz de Zárate, J.V. Sengers, Physica A 300, 25 (2001)
F. Croccolo, H. Bataller, F. Scheffold, J. Chem. Phys. 137, 234202 (2012)
F. Croccolo, F. Scheffold, H. Bataller, C. R. Mec. 341, 378 (2013)
C. Giraudet, H. Bataller, F. Croccolo, Eur. Phys. J. E 37, 107 (2014)
F. Croccolo, C. Giraudet, H. Bataller, R. Cerbino, A. Vailati, Micrograv. Sci. Technol. 28, 467 (2016)
I. Lizarraga, C. Giraudet, F. Croccolo, M.M. Bou-Ali, H. Bataller, Micrograv. Sci. Technol. 28, 1 (2016)
F. Croccolo, PhD Thesis, University of Milano (2005)
F. Croccolo, D. Brogioli, A. Vailati, M. Giglio, D.S. Cannell, Ann. N. Y. Acad. Sci. 1077, 365 (2006)
F. Croccolo, D. Brogioli, A. Vailati, M. Giglio, D.S. Cannell, Appl. Opt. 45, 2166 (2006)
J.J. Hegseth, A. Oprisan, Y. Garrabos, D. Beysens, Phys. Rev. E 90, 022127 (2014)
C.J. Takacs, A. Vailati, R. Cerbino, S. Mazzoni, M. Giglio, D.S. Cannell, Phys. Rev. Lett. 106, 244502 (2011)
Q.A. Pankhurst, J. Connolly, S.K. Jones, J. Dobson, J. Phys. D: Appl. Phys. 36, R167 (2003)
C.C. Berry, A.S.G. Curtis, J. Phys. D: Appl. Phys. 36, R198 (2003)
R.A. Frimpong, J.Z. Hilt, Nanomedicine 5, 1401 (2010)
J. Dobson, Gene Ther. 13, 283 (2006)
J. Siepmann, R.A. Siegel, M.J. Rathbone, Fundamentals and Applications of Controlled Release Drug Delivery, Advances in Delivery Science and Technology (Springer US, 2011)
G.F. Goya, V. Grazu, M.R. Ibarra, Current Nanosci. 4, 1 (2008)
M. Banobre-Lopez, A. Teijeiro, J. Rivas, Rep. Practical Oncol. Radiother. 18, 397 (2013) Selected Papers Presented at the XVII SEOR Congress, Vigo, 18-21 June 2013
N.M. Mahmoodi, J. Abdi, D.a. Bastani, J. Environ. Health Sci. Eng. 12, 1501 (2004)
A.F. Ngomsik, A. Bee, M. Draye, G. Cote, V. Cabuil, C. R. Chim. 8, 963 (2005)
S. Martel, C.C. Tremblay, S. Ngakeng, G. Langlois, Appl. Phys. Lett. 89, 233904 (2006)
J.R. Basore, N.V. Lavrik, L.A. Baker, Adv. Mater. 22, 2759 (2010)
P. Rinklin, H.J. Krause, B. Wolfrum, Phys. Status Solidi A 209, 871 (2012)
P.A. Liberti, C.G. Rao, L.W. Terstappen, J. Magn. & Magn. Mater. 225, 301 (2001) Proceedings of the Third International Conference on Scientific and Clinical Applications of Magnetic Carriers
F.Z. Sehrig, S. Majidi, N. Nikzamir, N. Nikzamir, M. Nikzamir, A. Akbarzadeh, Artificial Cells, Nanomed. Biotechnol. 44, 918 (2016)
F. Paul, D. Melville, S. Roath, D. Warhurst, IEEE Trans. Magn. 17, 2822 (1981)
K. Chen, C. Yuen, Y. Aniweh, P. Preiser, Q. Liu, Sci. Rep. 6, 20177 (2016)
J.D. Unciti-Broceta, V. Cano-Cortes, P. Altea-Manzano, S. Pernagallo, J.J. Diaz-Mochon, R.M. Sanchez-Martin, Sci. Rep. 5, 10091 (2015)
B.L. Frankamp, A.K. Boal, V.M. Rotello, J. Am. Chem. Soc. 124, 15146 (2002)
B. Bharti, A.L. Fameau, M. Rubinstein, O.D. Velev, Nat. Mater. 14, 1104 (2015)
S.A. Maier, M.L. Brongersma, P.G. Kik, S. Meltzer, A.A.G. Requicha, H.A. Atwater, Adv. Mater. 13, 1501 (2001)
M. Han, X. Gao, J.Z. Su, S. Nie, Nat. Biotechnol. 19, 631 (2001)
J.N. Anker, W.P. Hall, O. Lyandres, N.C. Shah, J. Zhao, R.P. Van Duyne, Nat. Mater. 7, 442 (2008)
D.I. Gittins, F. Caruso, ChemPhysChem 3, 110 (2002)
R. Sardar, J.S. Shumaker-Parry, Nano Lett. 8, 731 (2008)
A. Gentile, F. Ruffino, M.G. Grimaldi, Nanomaterials 6, 110 (2008)
M.S. Hu, H.L. Chen, C.H. Shen, L.S. Hong, B.R. Huang, K.H. Chen, L.C. Chen, Nat. Mater. 5, 102 (2006)
J. Ge, Y. Hu, M. Biasini, W. Beyermann, Y. Yin, Angew. Chem. Int. Ed. 46, 4342 (2007)
A.V. Alekseeva, V.A. Bogatyrev, B.N. Khlebtsov, A.G. Melʼnikov, L.A. Dykman, N.G. Khlebtsov, Colloid J. 68, 661 (2006)
K. Vasilev, T. Zhu, M. Wilms, G. Gillies, I. Lieberwirth, S. Mittler, W. Knoll, M. Kreiter, Langmuir 21, 12399 (2005)
J.E. Millstone, S. Park, K.L. Shuford, L. Qin, G.C. Schatz, C.A. Mirkin, J. Am. Chem. Soc. 127, 5312 (2005)
E. Kowsari, J. Nanoparticle Res. 13, 3363 (2011)
Y. Yang, Y. Zhao, Y. Yan, Y. Wang, C. Guo, J. Zhang, J. Phys. Chem. B 119, 14807 (2015)
M. Tsuji, S. Gomi, Y. Maeda, M. Matsunaga, S. Hikino, K. Uto, T. Tsuji, H. Kawazumi, Langmuir 28, 8845 (2012)
D. Brogioli, D. Salerno, V. Cassina, S. Sacanna, A.P. Philipse, F. Croccolo, F. Mantegazza, Opt. Express 17, 1222 (2009)
I. Martchenko, H. Dietsch, C. Moitzi, P. Schurtenberger, J. Phys. Chem. B 115, 14838 (2011)
A. Wittmeier, A.L. Holterhoff, J. Johnson, J.G. Gibbs, Langmuir 31, 10402 (2015)
M.A. Escobedo-Sánchez, H.A. De la Cruz-Burelo, J.L. Arauz-Lara, C. Haro-Pérez, L.F. Rojas-Ochoa, J. Chem. Phys. 143, 044902 (2015)
C. Passow, B. ten Hagen, H. Löwen, J. Wagner, J. Chem. Phys. 143, 044903 (2015)
C. Geers, L. Rodriguez-Lorenzo, D.A. Urban, C. Kinnear, A.S. Fink, S. Balog, Nanoscale 8, 15813 (2016)
F. Giavazzi, G. Savorana, A. Vailati, R. Cerbino, Soft Matter 12, 6588 (2016)
W. Russel, D.A. Saville, W.R. Schowalter, Colloidal Dispersions (Cambridge University Press, Cambridge, 1989)
D. Beysens, D. Estève, Phys. Rev. Lett. 54, 2123 (1985)
M.L. Broide, Y. Garrabos, D. Beysens, Phys. Rev. E 47, 3768 (1993)
N. Fuchs, Z. Phys. 89, 736 (1934)
M.E. Fisher, P.G. de Gennes, C. R. Acad. Sci. Ser. B 287, 207 (1978)
P.G. de Gennes, C. R. Acad. Sci. Ser. II 292, 701 (1981)
H.B.G. Casimir, Proc. K. Ned. Akad. Wet. 51, 793 (1948)
T. Kirkpatrick, J. Ortiz de Zarate, J. Sengers, Phys. Rev. Lett. 115, 035901 (2015)
J.M. Ortiz de Zarate, T.R. Kirkpatrick, J.V. Sengers, Eur. Phys. J. E 38, 99 (2015)
T.R. Kirkpatrick, J.M. Ortiz de Zárate, J.V. Sengers, Phys. Rev. E 93, 012148 (2016)
T.R. Kirkpatrick, J.M. Ortiz de Zárate, J.V. Sengers, Phys. Rev. E 93, 032117 (2016)
A. Donev, E. Vanden-Eijnden, A.L. Garcia, J.B. Bell, Commun. Appl. Math. Comput. Sci. 5, 149 (2010)
F. Usabiaga, J. Bell, R. Delgado-Buscalioni, A. Donev, T. Fai, B. Griffith, C. Peskin, Multiscale Model. Simul. 10, 1369 (2012)
S. Delong, Y. Sun, B.E. Griffith, E. Vanden-Eijnden, A. Donev, Phys. Rev. E 90, 063312 (2014)
A. Chaudhri, J.B. Bell, A.L. Garcia, A. Donev, Phys. Rev. E 90, 033014 (2014)
R. Cerbino, Y. Sun, A. Donev, A. Vailati, Sci. Rep. 5, 14486 (2015)
A. Donev, J.B. Bell, A. de la Fuente, A.L. Garcia, Phys. Rev. Lett. 106, 204501 (2011)
A. Donev, A. Nonaka, Y. Sun, T. Fai, A. Garcia, J. Bell, Commun. Appl. Math. Comput. Sci. 9, 47 (2014)
A. Nonaka, Y. Sun, J. Bell, A. Donev, Commun. Appl. Math. Comput. Sci. 10, 163 (2015)
A.K. Bhattacharjee, K. Balakrishnan, A.L. Garcia, J.B. Bell, A. Donev, J. Chem. Phys. 142, 224107 (2015)
A. Donev, E. Vanden-Eijnden, J. Chem. Phys. 140, 234115 (2014)
A. Donev, A. Nonaka, A.K. Bhattacharjee, A.L. Garcia, J.B. Bell, Phys. Fluids 27, 037103 (2015)
F. Croccolo, D. Brogioli, Appl. Opt. 50, 3419 (2011)
F. Croccolo, D. Brogioli, A. Vailati, M. Giglio, D.S. Cannell, Phys. Rev. E 76, 041112 (2007)
K.D. Sattler, Handbook of Nanophysics: Nanoparticles and Quantum Dots (CRC Press, 2016)
X. Cao, Y. Koltypin, R. Prozorov, G. Kataby, A. Gedanken, J. Mater. Chem. 7, 2447 (1997)
A. Loman, I. Gregor, C. Stutz, M. Mund, J. Enderlein, Photochem. Photobiol. Sci. 9, 627 (2010)
S.P. Trainoff, D.S. Cannell, Phys. Fluids 14, 1340 (2002)
M. Wu, G. Ahlers, D.S. Cannell, Phys. Rev. Lett. 75, 1743 (1995)
M. Giglio, M. Carpineti, A. Vailati, Phys. Rev. Lett. 85, 1416 (2000)
F. Ferri, D. Magatti, D. Pescini, M. Potenza, M. Giglio, Phys. Rev. E 70, 041405 (2004)
S.W. Morris, E. Bodenschatz, D.S. Cannell, G. Ahlers, Physica D 97, 164 (1996)
J.R. de Bruyn, E. Bodenschatz, S.W. Morris, S.P. Trainoff, Y. Hu, D.S. Cannell, G. Ahlers, Rev. Sci. Instrum. 67, 2043 (1996)
G. Cerchiari, F. Croccolo, F. Cardinaux, F. Scheffold, Rev. Sci. Instrum. 83, 106101 (2012)
J. Faraudo, J.S. Andreu, J. Camacho, Soft Matter 9, 6654 (2013)
J. Faraudo, J.S. Andreu, C. Calero, J. Camacho, Adv. Funct. Mater. 26, 3837 (2016)
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Oprisan, A., Rice, A., Oprisan, S.A. et al. Non-equilibrium concentration fluctuations in superparamagnetic nanocolloids. Eur. Phys. J. E 40, 14 (2017). https://doi.org/10.1140/epje/i2017-11503-y
Received:
Accepted:
Published:
DOI: https://doi.org/10.1140/epje/i2017-11503-y