Skip to main content
Log in

Prompt Fission Neutron Spectra of 240Pu(n, F), 239Pu(n, F), and 238U(n, F)

  • PHYSICS OF ELEMENTARY PARTICLES AND ATOMIC NUCLEI. THEORY
  • Published:
Physics of Particles and Nuclei Letters Aims and scope Submit manuscript

Abstract

Pre-fission neutron spectra are indicators of the distribution of fission reaction energy between the kinetic energy of fragments and prompt fission neutrons. Using the 240Pu(n, F), 239Pu(n, F), and 238U(n, F) reactions as an example, it is shown how the shape of the observed prompt fission neutron spectra (PFNS) depends on the fissility (fission probability) of compound and residual nuclei. A correlation of this effect with the contributions of the (n, xnf) emission fission to the observed fission cross section and the competition of the (n, nγ) and (n, xn)1,...x reactions is established. The exclusive spectra of the (n, xnf)1,...x neutrons correspond to the consistent description of the observed cross sections for the 240Pu(n, F), 239Pu(n, F), 238Pu(n, F), 237Pu(n, F), and 236Pu(n, F) fission reactions, as well as 239Pu(n, xn) neutron emission spectra for neutrons with energies up to 20 MeV. The initial values of the model parameters for describing the 240Pu(n, F) PFNS are fixed when describing the prompt neutron spectra of 240Pu(sf) spontaneous fission. Taking into account the influence of the exclusive spectra of 240Pu (n, xnf)1,...x prefission neutrons, the prompt fission neutron spectra, the total kinetic energy (TKE) of fragments and fission products, and the average number of 240Pu(n, F) prompt fission neutrons are predicted.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1.
Fig. 2.
Fig. 3.
Fig. 4.
Fig. 5.
Fig. 6.
Fig. 7.
Fig. 8.
Fig. 9.
Fig. 10.
Fig. 11.
Fig. 12.
Fig. 13.

Similar content being viewed by others

REFERENCES

  1. V. M. Maslov, “Prompt fission neutron spectra of 235U and 239Pu,” in Proceedings of ‘Nucleus–2022’ 72nd International Conference “Fundamental Problems and Applications”, Moscow, 2022, p. 111. https:// events.sinp.msu.ru/event/8/attachments/181/875nucleus– 2022–book–of–abstracts–www.pdf.

    Google Scholar 

  2. V. M. Maslov, “Anisotropy in pre-fission and (n, n'γ) neutron spectra of 238U + n,” in Proceedings of ‘Nucleus–2022’ 72nd International Conference “Fundamental Problems and Applications”, Moscow, 2022, p. 168.

  3. V. M. Maslov, “Pre–fission (n, 2nf)1, 2 neutrons in 235U(n, f) and 239Pu(n, f),” in Proceedings of ‘Nucleus–2022’ 72nd International Conference “Fundamental Problems and Applications”, Moscow, 2022, p. 169.

  4. Yu. A. Vasil’ev, Yu. S. Zamyatnin, Yu. I. Il’in, E. I. Sirotinin, P. V. Toropov, and E. F. Fomushkin, “Measurements of the spectra and average number of neutrons in the fission of 235U and 238U by neutrons with an energy of 14.3 MeV,” Zh. Eksp. Teor. Fiz. 38, 671 (1960).

    Google Scholar 

  5. W. F. Weisscopf, “Statistics and nuclear reactions,” Phys. Rev. 52, 295 (1937).

    Article  ADS  Google Scholar 

  6. B. E. Watt, “Energy spectrum of neutrons from thermal fission of 235U,” Phys. Rev. 87, 1037 (1952).

    Article  ADS  Google Scholar 

  7. G. S. Boikov, V. D. Dmitriev, G. A. Kudyaev, M. I. Svirin, and G. N. Smirenkin, “Neutron spectrum of 232Th, 235U, and 238U fission by neutrons with an energy of 2.1 MeV and 14.7 MeV (below and above the emission fission threshold),” Yad. Fiz. 53, 628 (1991).

    Google Scholar 

  8. M. Devlin, E. A. Bennett, M. Q. Buckner, et al., “Experimental prompt fission neutron spectra for the 235, 238U(n, f), 239Pu(n, f) and 240, 242Pu(sf),” https://indico.frib.msu.edu/event/52/contributions/616/.

  9. V. M. Maslov, Yu. V. Porodzinskij, M. Baba, A. Hasegawa, N. V. Kornilov, A. B. Kagalenko, and N. A. Tetereva, “Prompt fission neutron spectra of 238U(n, f) and 232Th(n, f) above emissive fission threshold,” Phys. Rev. C 69, 034607 (2004).

    Article  ADS  Google Scholar 

  10. N. V. Kornilov, A. B. Kagalenko, and F.-J.Hambsch, “Calculation of prompt fission neutron spectra based on new systematics of experimental data,” Yad. Fiz. 62, 209 (1999).

    Google Scholar 

  11. Fission neutron Spectra of Uranium-235, NEA, NEA/WEC-9, OECD, 2003.

  12. D. Hilscher and H. Rossner, “Dissipation in nuclear fission,” Annales des Pysique 17, 471 (1992).

    Article  ADS  Google Scholar 

  13. B. I. Starostov, V. N. Nefedov, and A. A. Boitsov, “Spectra of prompt neutrons of U-233, U-235, Pu-239 fission by thermal neutrons and spontaneous fission of Cf-252 in the energy range 0.01-12 MeV,” Vopr. At. Nauki Tekh. Ser. Yad. Konst. No. 3, 16 (1985).

    Google Scholar 

  14. V. M. Maslov, V. G. Pronyaev, N. A. Tetereva, et al., “235U(n, F), 233U(n, F) and 239Pu(n, F) prompt fission neutron spectra,” J. Korean Phys. Soc. 59, 1337 (2011).

    Article  ADS  Google Scholar 

  15. B. Gerasimenko, L. Drapchinsky, O. Kostochkin, et al., “Precision measurements of prompt neutron spectra in 240Pu and 242Pu spontaneous fission,” J. Nucl. Sci. Technol. 2, 362 (2002).

    Article  Google Scholar 

  16. K. Shibata, O. Iwamoto, T. Nakagawa, et al., “JENDL-4.0: a new library for nuclear science and engineering,” J. Nucl. Sci. Technol. 48, 1 (2011).

    Article  Google Scholar 

  17. D. A. Brown, M. B. Chadwick, R. Capote, et al., “ENDF/B–VIII.0: The 8th major release of the nuclear reaction data library with CIELO–project cross sections, new standards and thermal scattering data,” Nucl. Data Sheets 148, 1 (2018).

    Article  ADS  Google Scholar 

  18. D. Madland, “Total prompt energy release in the neutron-induced fission of 235U, 238U and 239Pu neutron spectra and average prompt neutron multiplicities,” Nucl. Phys. A 772, 113 (2006).

    Article  ADS  Google Scholar 

  19. C. Zoller, PhD Thesis (Technische Hochschule, Darmstadt, 1995). http://www-win.gsi.de/charms/data.htm.

  20. D. L. Duke, F. Tovesson, A. B. Laptev, et al., “Fission-fragment properties in 238U(n, f) between 1 and 30 MeV," Phys. Rev. C 94, 054604 (2016).

    Article  ADS  Google Scholar 

  21. V. M. Maslov, “Total kinetic energies in 232Th(n, F), 238U(n, F),” http://isinn.jinr.ru/past-isinns/isinn-27/abstracts/.

  22. Yu. A. Khokhlov, I. A. Ivanin, V. I. In’kov, et al., “Measurements results of average neutron multiplicity from neutron induced fission of actinides in 0.5–10 MeV energy range,” in Proceedings of the International Conference on Nuclear Data for Science and Technology, Gatlinburg, TN, 1994, Vol. 1, p. 272.

  23. V. M. Maslov, “Spectra of prompt neutrons from 238U fission,” Yad. Fiz. 71, 11 (2008).

    Google Scholar 

  24. V. M. Maslov, “Spectra of prompt U and Pu fission neutrons above the emission fission threshold,” Vopr. At. Nauki Tekh. Ser. Fiz. Yad. Reakt. No. 2, 33 (2006). http://vniief.ru/wps/wcm/connect/vniief/site/publishing/ publications/nuclearreactor/y2006/y2-2006/vipusk2_2006.

  25. V. M. Maslov, “Spectra of prompt neutrons from 239Pu fission,” At. Energy 103, 119 (2007).

    Article  Google Scholar 

  26. N. V. Kornilov, “Spectra of prompt neutrons from 238U fission,” Vopr. At. Nauki Tekh. Ser. Fiz. Yad. Reakt. No. 4, 46 (1985).

    Google Scholar 

  27. G. N. Lovchikova, A. M. Trufanov, M. I. Svirin, et al., “Spectra and mean energies of prompt neutrons from 238U fission induced by primary neutrons of energy in the region E n <20 MeV,” Phys. At. Nucl. 67, 1246–1263.

  28. J. Frehaut, A. Bertin, and R. Bois, “Measurement of the fission neutron energy spectra for the fast neutron induced fission of U-235 and U-238,” in Proceedings of 3rd All-Union Conference on Neutron Physics, Kiev, 1975, Vol. 5, pp. 349—362.

  29. V. M. Maslov, “Direct and compound interactions for the neutron-induced fission cross section determination,” EPJ Web Conf. 8, 02002 (2010).

  30. J. L. Kammerdiener, “Neutron spectra emitted by 239Pu, 238U, 235U, Pb, Nb, Ni, Al and C irradiated by 14 MeV neutrons,” UCRL-51232, 1972.

  31. M. Baba, H. Wakabayashi, N. Ito, et al., “Measurements of prompt fission neutron spectra and double-differential neutron inelastic-scattering cross sections for 238U and 232Th,” J. Nucl. Sci. Technol. 27, 601 (1990).

    Article  Google Scholar 

  32. V. M. Maslov, Yu. V. Porodzinskij, N. A. Tetereva, et al., “Excitation of octupole, beta- and gamma-vibration band levels of 238U by inelastic neutron scattering,” Nucl. Phys. A 764, 212 (2006).

    Article  ADS  Google Scholar 

  33. M. Dupuis, S. Hilaire, and S. Peru, “Microscopic modeling of direct pre-equilibrium emission from neutron induced reactions on even and odd actinides,” EPJ Web Conf. 146, 12002 (2017).

  34. K. J. Kelly, T. Kawano, J. M. O’Donnel, et al., “Pre-equilibrium asymmetries in the 239Pu(n, f) prompt fission neutron spectrum,” Phys. Rev. Lett. 122, 072503 (2019).

    Article  ADS  Google Scholar 

  35. P. Marini, J. Taieb, B. Laurent, et al., “Prompt-fission-neutron spectra in the 239Pu(n, f) reaction,” Phys. Rev. C 101, 044614 (2020).

    Article  ADS  Google Scholar 

  36. K. J. Kelly, M. Devlin, J. M. O’Donnel, et al., “Measurement of the 239Pu(n, f) prompt fission neutron spectrum from 10 keV to 10 MeV induced by neutrons of energy 1-20 MeV,” Phys. Rev. C 102, 034615 (2020).

    Article  ADS  Google Scholar 

  37. K. J. Kelly, J. A. Gomez, M. Devlin, et al., “Measurement of the 235U(n, f) prompt fission neutron spectrum from 10 keV to 10 MeV induced by neutrons of energy 1–20 MeV,” Phys. Rev. C 105, 044615 (2022).

    Article  ADS  Google Scholar 

  38. V. M. Maslov, N. A. Tetereva, V. G. Pronyaev, et al., “Spectrum of prompt fission neutrons 235U(n, f), At. Energy 108, 352 (2010).

    Google Scholar 

  39. V. M. Maslov, “Prompt fission neutron spectra of 235U(n, F) and 239Pu(n, F),” https://events.sinp. msu.ru/event/8/contributions/586/attachments/568/881/ mvmNucl2022%2B.pdf.

  40. V. M. Maslov, N. V. Kornilov, A. B. Kagalenko, and N. A. Tetereva, “Prompt fission neutron spectra of 235U up above emissive fission threshold,” Nucl. Phys. A 760, 274 (2005).

    Article  ADS  Google Scholar 

  41. V. M. Maslov, Yu. V. Porodzinskij, M. Baba, A. Hasegawa, N. V. Kornilov, A. B. Kagalenko, and N. A. Tetereva, “Prompt fission neutron spectra of 238U(n, f) above emissive fission threshold,” Eur. Phys. J. A 18, 93 (2003).

    Article  ADS  Google Scholar 

  42. A. Pica, A. T. Chemey, and W. Loveland, “The fast neutron induced fission of 240Pu and 242Pu,” Phys. Rev. C 106, 044603 (2022).

    Article  ADS  Google Scholar 

  43. V. G. Vorob’eva, N. P. D’yachenko, B. D. Kuz’minov, et al., “Definition of energy dependence υ for 238U, 240Pu and 242Pu using energy balance analysis,” At. Energy 36, 32 (1974).

    Google Scholar 

  44. K. Shimada, Ch. Ishizuka, F. A. Ivanyuk, et al., “Dependence of total kinetic energy of fission fragments on the excitation energy of fissioning systems,” Phys. Rev. C 104, 054609 (2021).

    Article  ADS  Google Scholar 

  45. A. S. Vorob’ev and O. A. Shcherbakov, “Integrated spectra of prompt neutrons from 235U and 239Pu fission by thermal neutrons,” Vopr. At. Nauki Tekh. Ser. Yad. Konst. No. 2, 52 (2016).

    Google Scholar 

  46. V. M. Maslov, in Proceedings of 4th International Workshop on Nuclear Fission and Fission–Product Spectroscopy, Ed. by A. Chatillon, H. Faust, G. Fioni, D. Goutte, and H. Goutte (AIP, 2009), CP1175.

  47. V. M. Maslov, “Symmetric vs asymmetric nucleon-induced fission of thorium up to 200 MeV,” Phys. Lett. B 649, 376 (2007).

    Article  ADS  Google Scholar 

  48. V. M. Maslov, “Symmetric/asymmetric p- and n-induced fission of Th, Pa, U, Np, Pu and Am,” J. Korean Phys. Soc. 59, 863 (2011).

    Article  ADS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to V. M. Maslov.

Ethics declarations

The author declares that he has no conflicts of interest.

Additional information

Translated by E. Chernokozhin

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Maslov, V.M. Prompt Fission Neutron Spectra of 240Pu(n, F), 239Pu(n, F), and 238U(n, F). Phys. Part. Nuclei Lett. 20, 565–576 (2023). https://doi.org/10.1134/S1547477123040490

Download citation

  • Received:

  • Revised:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1134/S1547477123040490

Navigation