Abstract
In this paper, we present the results of studies of the heat capacity of single-crystal garnets Er3 ‒ xTmxAl5O12 (x = 0, 1, 2, 3) in magnetic fields of up to 9 T and in the temperature range 1.9–220 K. The temperature dependences of the heat capacity are approximated using the sum of the contributions of Schottky anomalies associated with magnetic Er3+ and Tm3+ ions and the Debye and Einstein lattice contributions. Entropy and magnetic entropy are calculated using the heat capacity data. With an increase in the magnetic field, entropy is shown to decrease. This indicates the possibility of using the studied garnets in the adiabatic demagnetization method.
Similar content being viewed by others
REFERENCES
W. Koechner, Solid State Laser Engineering (Springer-Verlag, Berlin, 2006).
A. A. Kaminskii, Laser Crystals (Nauka, Moscow, 1975).
E. V. Shevchenko, E. V. Charnaya, E. N. Khazanov, A. V. Taranov, and A. S. Bugaev, 59, 733 (2017).
J. D. French, J. Zhao, M. P. Harmer, et al., J. Am. Ceram. Soc. 77 (11), 2857 (1994).
A. Kushino, Y. Aoki, N. Y. Yamasaki, et al., J. Appl. Phys. 90, 5812 (2001).
E. V. Shevchenko, E. V. Charnaya, E. N. Khazanov, et al., J. Alloys Compd. 717, 183 (2017).
R. Li, T. Numazawa, T. Hashimoto, et al., in Advances in Cryogenic Engineering Materials, Ed. by K. D. Timmerhaus, R.W. Fast, A. F. Clark, R. P. Reed (Springer US, New York, 1986).
Jr. K. A. Gschneidner, V. K. Pecharsky, and A. O. Tsokol, Rep. Prog. Phys. 68, 1479 (2005).
A. M. Tishin and L. P. Bozkova, J. Appl. Phys. 81, 1000 (1997).
L. Veissier, C. W. Thiel, T. Lutz, et al., Phys. Rev. B 94, 205133 (2016).
E. N. Khazanov, A. V. Taranov, E. V. Shevchenko, and E. V. Charnaya, JETP 121, 48 (2015).
K. I. Portnoi and N. I. Timofeeva, Oxygen Connections of Rare-Earth Elements (Metallurgiya, Moscow, 1986).
A. Tari, The Specific Heat of Matter at Low Temperatures (Imperial College, London, 2003).
M. U. Gutowska, J. Wieckowski, A. Szewczyk, et al., J. Alloys Compd. 670, 175 (2016).
V. Babin, K. Chernenko, M. Hanus, et al., Phys. Status Solidi B 254, 1600570 (2017).
E. V. Shevchenko, E. V. Charnaya, M. K. Lee, et al., Phys. Lett. A, 381, 330 (2017).
K. S. Bagdasarov, A. P. Dodokin, and A. A. Sorokin, Fiz. Tverd. Tela (Leningrad) 30, 1840 (1988).
D. D. Perlov, A. A. Sorokin, V. A. Feodorov, and A. P. Dodokin, J. Mag. Mag. Mater 123 (1–2), 187 (1993).
G. W. Burdick, J. B. Gruber, K. L. Nash, et al., Spectroscopy Lett. 43, 406 (2010).
J. B. Gruber, M. E. Hills, R. M. Macfarlane, et al., Phys. Rev. B 40 (14), 9464 (1989).
C. Tiseanu, A. Lupei, and V. Lupei, J. Phys.: Cond. Matt. 7, 8477 (1995).
M. G. Beghi, C. E. Bottani, and V. Russo, J. Appl. Phys. 87, 1769 (2000).
Z. Huang, J. Feng, and W. Pan, Solid State Sci. 14, 1327 (2012).
U. V. Valiev, J. B. Gruber, I. R. Gapdulkhakov, N. I. Juraeva, A. K. Mukhammadiev, Sh. A. Rakhimov, and I. S. Edel’man, Opt. Spectrosk. 106, 851 (2012).
D. Jang, T. Gruner, A. Steppke, et al., Nature Commun. 6, 8680 (2015).
E. Palacios, J. A. Rodrígues-Velamazán, M. Evangelisti, et al., Phys. Rev. B 90, 214423 (2014).
ACKNOWLEDGMENTS
The authors are grateful to A.A. Kaminskii for providing samples of mixed compositions of erbium–thulium–aluminum garnets.
Funding
This work was supported by the Ministry of Education and Science of the Russian Federation as part of the State Task for 2019 and was partially supported by the Russian Foundation for Basic Research, projects nos. 18-07-00191 and 16-07-00181.
Author information
Authors and Affiliations
Corresponding authors
Additional information
Translated by A. Ivanov
Rights and permissions
About this article
Cite this article
Charnaya, E.V., Shevchenko, E.V., Khazanov, E.N. et al. Features of the Low-Temperature Heat Capacity of Er3 –xTmxAl5O12 Garnet Single Crystals. J. Commun. Technol. Electron. 64, 811–817 (2019). https://doi.org/10.1134/S1064226919070064
Received:
Revised:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1134/S1064226919070064