Skip to main content
Log in

Crystal structure and magnetic properties of Fe/Cr/Gd superlattices

  • Electrical and Magnetic Properties
  • Published:
Physics of Metals and Metallography Aims and scope Submit manuscript

Abstract

Results of investigations of structural and magnetic properties of Fe/Cr/Gd superlattices that differ in the thicknesses of the Cr interlayer have been reported. The insertion of the Cr interlayer between Gd and Fe layers has been found to lead to structural changes in Gd layers and the appearance of an additional fcc phase in them along with the main hcp phase. The new fcc phase is uniformly distributed across the thickness of the layer and is not localized near layer boundaries or in the center of Gd layers. Polarized-neutron reflectometry was used to show that the aforementioned structural changes are accompanied by a substantial (two-fold to threefold) decrease in the average magnetization of gadolinium over a wide temperature range. Near interfaces of the Gd layer, a layer appears that is two-to-three monatomic layers thick and characterized by increased magnetic moment.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. C. F. Majkrzak, J. Kwo, M. Yjng, Y. Yafet, D. Gibbs, C. L. Chen, and J. Bohr, “Magnetic rare earth superlattices,” Adv. Phys. 40, 99–189 (1991).

    Article  Google Scholar 

  2. Ultrathin Magnetic Structures, Ed. by B. Heinrich and J. A. C. Bland (Springer-Verlag, Berlin, 2005), Vols. I–IV.

  3. D. Haskel, G. Srajer, J. C. Lang, J. Pollmann, C. S. Nelson, J. S. Jiang, and S. D. Bader, “Enhanced interfacial magnetic coupling of Gd/Fe multilayers,” Phys. Rev. Lett. 87, 207201 (2001).

    Article  Google Scholar 

  4. E. Kravtsov, D. Haskel, S. G. E. te Velthuis, J. S. Jiang, and B. J. Kirby, “Complementary polarized neutron and resonant X-ray magnetic reflectometry measurements in Fe/Gd heterostructures: Case of inhomogeneous intralayer magnetic structure,” Phys. Rev. B: Condens. Matter Mater. Phys. 79, 134438 (2009).

    Article  Google Scholar 

  5. B. Sanyal, C. Antoniak, T. Burkert, B. Krumme, A. Warland, F. Stromberg, Ch. Praetorius, K. Fauth, H. Wende, and O. Eriksson, “Forcing ferromagnetic coupling between rare-earth-metal and 3d ferromagnetic films,” Phys. Rev. Lett. 104, 156402 (2010).

    Article  Google Scholar 

  6. A. B. Drovosekov, N. M. Kreines, A. O. Savitskii, E. A. Kravtsov, D. V. Blagodatkov, M. V. Ryabukhina, M. A. Milyaev, V. V. Ustinov, E. M. Pashaev, I. A. Subbotin, and G. V. Prutskov, “Interlayer coupling in Fe/Cr/Gd multilayer structures,” J. Exp. Theor. Phys. 120, 1041–1054 (2015).

    Article  Google Scholar 

  7. M. V. Ryabukhina, E. A. Kravtsov, D. V. Blagodatkov, L. I. Naumova, V. V. Proglyado, V. V. Ustinov, and Yu. Khaydukov, “Polarized neutron reflectometry of Fe/Cr/Gd superlattices,” J. Surf. Invest.: X-ray, Synchr. Neutr. Techn. 8, 983–986 (2014).

    Article  Google Scholar 

  8. M. V. Ryabukhina, E. A. Kravtsov, D. V. Blagodatkov, L. I. Naumova, Yu. V. Nikitenko, V. V. Proglyado, and Yu. Khaidukov, “Magnetism of Fe/Cr/Gd superlattices,” J. Surf. Invest.: X-ray, Synchr. Neutr. Techn. 9, 41–43 (2015).

    Article  Google Scholar 

  9. C. Ward, G. Scheunert, W. R. Hendren, R. Hardeman, M. A. Gubbins, and R. M. Bowman, “Realizing a high magnetic moment in Gd/Cr/FeCo: The role of the rare earth,” Appl. Phys. Lett. 102, 092403 (2013).

    Article  Google Scholar 

  10. G. Scheunert, W. R. Hendren, C. Ward, and R. M. Bowman, “Magnetization of 2.6 T in Gadolinium Thin Films,” Appl. Phys. Lett 101, 142407 (2012).

    Article  Google Scholar 

  11. G. Scheunert, C. Ward, W. R. Hendren, A. A. Lapicki, R. Hardeman, M. Mooney, M. A. Gubbins, and R. M. Bowman, “Influence of strain and polycrystalline ordering on magnetic properties of high moment rare earth metals and alloys,” J. Phys. D: Appl. Phys. 47, 415005 (2014).

    Article  Google Scholar 

  12. I. N. Yakovkin, Komesu. Takashi, and P. A. Dowben, “Band structure of strained Gd (0001) films,” Phys. Rev. B: Condens. Matter Mater. Phys. 66, 035406 (2002).

    Article  Google Scholar 

  13. T. Komesu, C. Waldfried, and P. A. Dowben, “The origin of enhanced magnetization in strained gadolinium,” Phys. Lett. A 256, 81–87 (1999).

    Article  Google Scholar 

  14. H. F. Kirby, D. D. Belyea, J. T. Willman, and C. W. Miller, “Effects of preparation conditions on the magnetocaloric properties of Gd thin films,” J. Vac. Sci. Technol., A 31, 031506 (2013).

    Article  Google Scholar 

  15. F. Stromberg, C. Antoniak, U. von Horsten, W. Keune, B. Sanyal, O. Eriksson, and H. Wende, “Textured growth of the high moment material Gd(0 0 0 1)/Cr(0 0 1)/Fe(0 0 1),” J. Phys. D: Appl. Phys. 44, 265004 (2011).

    Article  Google Scholar 

  16. T. P. Bertelli, E. C. Passamani, C. Larica, V. P. Nascimento, and A. Y. Takeuchi, “Ferromagnetic properties of fcc Gd thin films,” J. Appl. Phys. 117, 203904 (2015).

    Article  Google Scholar 

  17. G. Scheunert, O. Heinonen, R. Hardeman, A. Lapicki, M. Gubbins, and R. M. Bowman, “A review of high magnetic moment thin films for microscale and nanotechnology applications,” Appl. Phys. Rev. 3, 011301 (2016).

    Article  Google Scholar 

  18. A. E. Curzon and H. G. Chlebek, “The observation of face centred cubic Gd, Tb, Dy, Ho, Er and Tm in the form of thin films and their oxidation,” J. Phys. F: Met. Phys. 3, 1–5 (1979).

    Article  Google Scholar 

  19. Chin-Jui Hsu, S. V. Prikhodko, Wang Chiu-Yen, Chen Lih-Juann, and G. P. Carman, “Magnetic anisotropy in nanostructured gadolinium,” J. Appl. Phys. 111, 053916 (2012).

    Article  Google Scholar 

  20. M. Bouroushian and T. Kosanovic, “Characterization of thin films by low incidence X-ray diffraction,” Cryst. Struct. Appl. 1, 35–39 (2012).

    Google Scholar 

  21. M. F. Toney and S. Brennan, “Structural depth profiling of iron oxide thin films using grazing incidence asymmetric Bragg X-ray diffraction,” J. Appl. Phys. 65, 4763–4768 (1989).

    Article  Google Scholar 

  22. R. J. Elliott, Magnetic Properties of Rare Earth Metals (Springer-Verlag, New York, 1972).

    Book  Google Scholar 

  23. P. E. Chizhov, A. N. Kostigov, and V. I. Petinov, “Structure and magnetic properties of rare earth small particles,” Solid State Commun. 42, 323–326 (1982).

    Article  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to M. V. Ryabukhina.

Additional information

Original Russian Text © M.V. Ryabukhina, E.A. Kravtsov, L.I. Naumova, V.V. Proglyado, Yu.N. Khaidukov, V.V. Ustinov, 2017, published in Fizika Metallov i Metallovedenie, 2017, Vol. 118, No. 2, pp. 151–157.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Ryabukhina, M.V., Kravtsov, E.A., Naumova, L.I. et al. Crystal structure and magnetic properties of Fe/Cr/Gd superlattices. Phys. Metals Metallogr. 118, 143–149 (2017). https://doi.org/10.1134/S0031918X17020119

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1134/S0031918X17020119

Keywords

Navigation