Abstract—
A process has been developed for the preparation of high-purity granulated zinc for the growth of Zn82Se scintillator crystals intended for investigation of neutrinoless double beta decay, 2β(0ν), of the 82Se isotope in the CUPID-0 experiment. We have determined the chemical and isotopic compositions of high-purity zinc prepared by this process and assessed its radionuclide purity. The background spectrum of the high-purity zinc, measured with a germanium detector, showed no peaks of natural 40K, 60Co, or 137Cs radionuclides or ones from the uranium–thorium decay series. We have noticed an increased activity of the 54Mn, 56Со, 57Со, 58Co, and 65Zn nuclides, resulting mainly from the exposure to cosmic rays.
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REFERENCES
Barabash, A.S., Double beta decay experiments: current status and prospects, Usp. Fiz. Nauk, 2014, vol. 184, no. 5, pp. 524–530. https://doi.org/10.3367/UFNr.0184.201405f.0524
Gironi, L., Scintillating bolometers for double beta decay search, Nucl. Instrum. Meth. A, 2010, vol. 617, nos. 1–3, pp. 478–481. https://doi.org/10.1016/j.nima.2009.10.080
Arnaboldi, C., Capelli, S., Cremonesi, O., Gironi, L., Pavan, M., Pessina, G., and Pirro, S., Characterization of ZnSe scintillating bolometers for double beta decay, Astropart. Phys., 2011, vol. 34, no. 6, pp. 344–353. https://doi.org/10.1016/j.astropartphys.2010.09.004
Kovtun, G.P. and Shcherban’, A.P., Ukr. Patent 1246, Byull. Izobret., 2002, no. 5.
Shcherban’, A.P., Preparation of high-purity metals for the fabrication of low-background scintillation detectors for rare events, Vopr. At. Nauki Tekh., Ser.: Vakuum, Chistye Mater., Sverkhprovodn., 2011, no. 6 (19), pp. 3–10. https://vant.kipt.kharkov.ua/TABFRAME.html
Shcherban’, A.P., Kovtun, G.P., Gorbenko, Yu.V., Solopikhin, D.A., Virich, V.D., and Pirozhenko, L.A., Preparation of high-purity granulated cadmium, zinc, and lead metals, Tekhnol. Konstruir. Elektron. Apparat., 2017, nos. 1–2, pp. 55–60. https://doi.org/10.15222/TKEA2017.1-2.55
Berglund, M. and Wieser, M.E., Isotopic compositions of the elements 2009 (IUPAC technical report), Pure Appl. Chem., 2011, vol. 83, no. 2, pp. 397–410. https://doi.org/10.1351/PAC-REP-10-06-02
Arpesella, C., A low background counting facility at Laboratori Nazionali del Grans Sasso, Appl. Radiat. Isot., 1996, vol. 47, nos. 9–10, pp. 991–996. https://doi.org/10.1016/S0969-8043(96)00097-8
Neder, N., Heusser, G., and Laubenstein, M., Low-level germanium-spectrometer to measure very low primordial radionuclide concentrations, Appl. Radiat. Isot., 2000, vol. 53, nos. 1–2, pp. 191–195. https://doi.org/10.1016/S0969-8043(00)00132-9
Heusser, G., Laubenstein, M., and Neder, N., Low-level germanium-ray spectrometry at the Bq/kg level and future developments towards higher sensitivity, Radioactivity Environment, 2006, vol. 8, pp. 495–510. https://doi.org/10.1016/S1569-4860(05)08039-3
Budjas, D., Hampel, W., Heisel, M., Heusser, G., Keillor, M., Laubenstein, M., Maneschg, W., Rugel, G., Schönert, S., Simgen, H., and Strecker, H., Highly sensitive gamma-spectrometers of GERDA for material screening: part 2, Proc. XIV Int. Baksan School “Particles and Cosmology,” Baksan Valley, Kabardino-Balkaria, Russia, 2007, pp. 233–238.
Boswell, M. et al., MaGe—a Geant4-based Monte Carlo application framework for low-background germanium experiments, IEEE Trans Nucl. Sci., 2011, vol. 58, pp. 1212–1220. https://doi.org/10.1109/TNS.2011.2144619
Heisel, M., Kaether, F., and Simgen, H., Statistical analysis of low-level screening measurements via gamma-spectroscopy, Appl. Radiat. Isot., 2009, vol. 67, no. 5, pp. 741–745. https://doi.org/10.1016/j.apradiso.2009.01.028
ACKNOWLEDGMENTS
We are deeply grateful to our colleagues at the Gran Sasso National Laboratory (LNGS, Assergi, Italy) for performing the measurements and providing data on the isotopic composition and radionuclide content of the high-purity zinc.
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Kovtun, G.P., Shcherban’, A.P., Solopikhin, D.A. et al. High-Purity Zinc for Low-Background Experiments. Inorg Mater 56, 178–181 (2020). https://doi.org/10.1134/S0020168520010082
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DOI: https://doi.org/10.1134/S0020168520010082