Abstract
A brief review of works performed by Russian scientists in the field of atmospheric chemistry from 2003 through 2006, including works on the chemistry of the troposphere, the chemistry of the ozone layer, and the role of chemistry in climate changes, is presented. This review was prepared in the Commission on Atmospheric Chemistry and Global Pollution of the Section of Meteorology and Atmospheric Sciences of the National Geophysical Committee.
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References
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A. N. Ermakov, I. K. Larin, A. A. Ugarov, and A. P. Purmal’, “Catalysis of SO2 Oxidation in the Atmosphere by Iron Ions,” Kinet. Katal. 44, 524–537 (2003).
A. N. Ermakov, I. K. Larin, A. A. Ugarov, and A. P. Purmal’, “Effect of Droplet Sizes on the Rate and Mechanism of SO2 Oxidation in Tropospheric Clouds,” Kinet. Katal. 47, 836–848 (2006).
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K. P. Kutsenogii and P. K. Kutsenogii, “Method of Identifying Atmospheric-Aerosol Sources in the Siberian Region,” Geogr. Prir. Resursy., Spets. Vyp. 43–53 (2004).
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N. N. Ulyumdzhieva, N. E. Chubarova, and B. Kholben, “Optical Properties of Atmospheric Aerosol in the Period of Forest Fires in 2002 in the Moscow Region,” Meteorol. Gidrol., No. 3, 45–52 (2005).
I. D. Eremina, “Multiyear Observations of the Chemical Composition of Atmospheric Precipitation in Moscow,” Vestn. Mosk. Univ., Ser. 5, Geogr. No. 2, 21–26 (2004).
I. D. Eremina, “Acidity and Ion Composition of Atmospheric Precipitation in Moscow,” in Handbook on Ecoclimatological Characteristics of Moscow (MGU, Moscow, 2005), 2, pp. 143–153 [in Russian].
I. D. Eremina, “Variations in Atmospheric Precipitation Acidity in Recent Years from Observations of the MSU Meteorological Observatory,” in Climate, Quality of Atmospheric Air, and Health of Muscovites, Ed. by B. A. Revich (Adamant Moscow, 2006) [in Russian].
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G. Krueger and N. Elansky, et al., “Input of Trichloroacetic Acid into the Vegetation of Various Climate Zones — Measurements on Several Continents,” Chemosphere 52, 443–449 (2003).
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V. V. Zelenov, E. V. Aparina, M. Yu. Gershenzon, et al., “Kinetic Mechanisms for Entraining Atmospheric Gases by the Surfaces of Sea Salts: IV. Initial Stage of Entraining NO3 on NaCl and NaBr Salts,” Khim. Fiz. 22(11), 37–48 (2003).
V. V. Zelenov, E. V. Aparina, D. V. Shestakov, and Yu. M. Gershenzon, “Kinetic Mechanisms for Entraining Atmospheric Gases by the Surfaces of Sea Salts: V. Entraining NO3 on the Coating Deposited from the Mixture of MgCl2 6H2O and NaCl Salts,” Khim. Fiz. 23(1), 18–26 (2004).
A. P. Dement’ev, V. V. Zelenov, E. V. Aparina, et al., “Kinetic Mechanisms for Entraining Atmospheric Gases by the Surfaces of Sea Salts: VI. MgCl2 · 6H2O Segregation on the Surface of NaCl Salt Doped by MgCl2 · 6H2O and Its Influence on the Rate of a Heterogeneous Reaction with NO3,” Khim. Fiz. 23(11), 54–59 (2004).
V. V. Zelenov, E. V. Aparina, S. A. Kashtanov, et al., “Kinetic Mechanisms for Entraining Atmospheric Gases by the Surfaces of Sea Salts: VII. Entraining ClNO3 by ythe Surface of Dry NaCl Salt,” Khim. Fiz. 25(11), 35–49 (2006).
V. V. Zelenov, E. V. Aparina, S. A. Kashtanov, et al., “Kinetic Mechanism of ClONO2 Uptake on Polycrystalline of NaCl,” J. Phys. Chem. A 110, 6771–6780 (2006).
V. V. Zelenov, V. M. Grigor’eva, E. V. Aparina, et al., “Kinetic Mechanisms for Entraining Atmospheric Gases by the Surfaces of Sea Salts: VIII. Entraining ClNO3 on Moistened NaCl Salt: Chlorine Activation and Oxidative Ability of Coastal Zones,” Khim. Fiz. 25(5), 31–34 (2006).
V. S. Zakharenko and A. N. Moseichuk, “Adsorption of Freons by Calcium Carbonate under Atmospheric Conditions,” Opt. Atmos. Okeana 18, 506–510 (2005).
M. J. Kurylo and V. L. Orkin, “Determination of Atmospheric Lifetimes via the Measurement of OH Radical Kinetics,” Chem. Rev. 103, 5049–5076 (2003).
E. S. Vasil’ev, I. I. Morozov, W. Hack, et al., “Kinetics and Mechanism of Atmospheric Reactions of Partially Fluorinated Alcohols,” Kinet. Catal. 47, 834–845 (2006).
S. N. Kozlov, V. L. Orkin, and M. J. Kurylo, “An Investigation of the Reactivity of OH with Fluoroethanes: CH3CH2F (HFC-161), CH2FCH2F (HFC-152), and CH3CHF2 (HFC-152a),” J. Phys. Chem. A 107, 2239–2246 (2003).
S. N. Kozlov, V. L. Orkin, and M. J. Kurylo, “The OH Reactivity and UV Spectra of Propane, n-Propyl Bromide, and Isopropyl Bromide,” J. Phys. Chem. A 107, 1333–1338 (2003).
D. F. Hurst, P. A. Romashkin, J. Elkins, et al., “Emissions of Ozone-Depleted Substances in Russia deuring 2001,” J. Geophys. Res. 109, D14303 (2004).
A. N. Rublev, N. E. Chubarova, A. N. Trotsenko, and G. I. Gorchakov, “Determination of NO2 Column Amounts from AERONET Data,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 40, 62–77 (2004) [Izv., Atmos. Ocean. Phys. 40, 54–67 (2004)].
A. V. Zinchenko, N. N. Paramonov, V. I. Privalov, and A. I. Reshetnikov, “Analysis of Measurements of the Atmospheric Methane Concentration near St. Petersburg,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 40(1), 90–95 (2004) [Izv., Atmos. Ocean. Phys. 40, 80–85 (2004)].
F. V. Kashin, V. N. Aref’ev, Yu. I. Baranov, et al., “Variability of the Methane Content in the Atmospheric Surface Layer and in the Atmospheric Column,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 40, 403–409 (2004) [Izv., Atmos. Ocean. Phys. 40, 356–361 (2004)].
D. V. Ionov, T. A. Egorova, V. A. Zubov, and E. V. Rozanov, “Global Fields of the Total Ozone and Nitrogen Dioxide Contents Retrieved from Satellite Measurements and a Three-Dimensional Simulation,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 39, 620–630 (2003) [Izv., Atmos. Ocean. Phys. 39, 558–567 (2003)].
M. V. Makarova, A. V. Poberovskii, and Yu. M. Timofeev, “Temporal Variability of Total Atmospheric Carbon Monoxide over St. Petersburg,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 40, 355–365 (2004) [Izv., Atmos. Ocean. Phys. 40, 313–322 (2004)].
T. A. Markova, N. F. Elanskii, I. B. Belikov, et al., “Distribution of Nitrogen Oxides in the Atmospheric Surface Layer over Continental Regions of Russia,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 40, 811–823 (2004) [Izv., Atmos. Ocean. Phys. 40, 713–724 (2004)].
O. V. Postylyakov, A. S. Elokhov, I. B. Belikov, et al., Observations of Ozone and Nitrogen Dioxide Profiles in TROICA Experiments,” in Proceeding of the XX Quadrennial Ozone Symposium (Kos, Greece, 2004), Ed. by Christos S. Serefos (Univ. of Athens, Athens, 2004), pp. 1026–1027.
N. F. Elansky, V. N. Kozhevnikov, G. I. Kuznetsov, and B. I. Volkov, “Effect of Orographic Disturbances on Ozone Redistribution in the Atmosphere by the Example of Airflow about the Antarctic Peninsula,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 39, 105–120 (2003) [Izv., Atmos. Ocean. Phys. 39, 93–107 (2003)].
A. M. Zvyagintsev, “Similarity of Long-Term Surface Ozone Series Obtained at the Dolgoprudnyi (Moscow Oblast) and Belsk (Poland) Stations,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 39, 510–514 (2003) [Izv., Atmos. Ocean. Phys. 39, 461–465 (2003)].
N. F. Elansky, A. Ya. Arabov, I. A. Senik, et al., “The Study of the Surface Ozone Variations of Different Time Scales at Some Regions of Russia,” in EUROTRAC-2, TOR-2 Tropospheric Ozone Research, Final Report (ISS, Germany, 2003), pp. 63–68.
O. A. Tarasova, N. F. Elansky, G. I. Kuznetsov, et al., “Impact of Air Transport on Seasonal Variations and Trends of Surface Ozone at Kislovodsk High Mountain Station,” J. Atmos. Chem. 45, 245–259 (2003).
O. A. Tarasova, G. I. Kuznetsov, N. F. Elansky, et al., “Features in Seasonal Variations and Trends of Surface Ozone Concentration at the Kislovodsk High-Altitude Scientific Station,” Vestn. Mosk. Univ., Ser. 3, Fiz., Astron., No. 3b, 45–49 (2003).
A. N. Zvyagintsev, G. M. Kruchenitskii, and A. A. Chernikov, “Long-Term Variations in Tropospheric Ozone Content,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 41, 66–77 (2005) [Izv., Atmos. Ocean. Phys. 41, 56–66 (2005)].
N. F. Elansky, A. M. Zvyagintsev, and O. A. Tarasova, “Studies of Tropospheric Ozone in Europe and Russia,” Meteorol. Gidrol., No. 1, 125–127 (2003).
N. F. Elansky, I. B. Belikov, T. A. Markova, et al., “Experiment TROICA on Surface Ozone and Its Precursor Distributions over Continental Regions of Russia,” in Proceeding of the XX Quadrennial Ozone Symposium (, Kos, Greece, 2004), Ed. by Christos S. Serefos (Univ. of Athens, Athens, 2004), pp. 867–868.
N. F. Elansky, K. B. Moiseenko, and N. V. Pankratova, “Photochemical Generation of Ozone in the Plumes of Anthropogenic Emissions over the Khabarovsk Territory,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 41, 511–519 (2005) [Izv., Atmos. Ocean. Phys. 41, 461–468 (2005)].
A. A. Kiselev and I. L. Karol’, “Response of Tropospheric Gas Composition in Northern Midlatitudes to a Possible Methane Outbreak from the Erath’s Subsoil to the Atmosphere,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 39, 579–588 (2003) [Izv., Atmos. Ocean. Phys. 39, 521–529 (2003)].
N. F. Elansky, K. B. Moiseenko, and L. V. Panin, “Effect of Corona Discharges at High-Voltage Power Transmission Lines on the Chemical Composition of Surface Air,” in Proceedings of the Meeting on Atmospheric Physics: Electric Processes, Radiophysical Methods of Study (Nizhni Novgorod, 2003), pp. 68–70 [in Russian].
I. K. Larin, A. I. Spasskii, E. M. Trofimova, and L. E. Turkin, “Mechanism and Kinetics of the Reaction between Iodine Methyl and Ozone,” Kinet. Katal. 47(6), 1–7 (2006).
I. K. Larin, A. I. Spasskii, E. M. Trofimova, and L. E. Turkin, “Experimental Evidence for Acceleration of Reaction between Iodine Monoxide and Chlorine Monoxide at the Reactor Surface,” Kinet. Catal. 44, 202–209 (2003).
V. L. Orkin, V. G. Khamaganov, and I. K. Larin, “In Situ Separation of Heterogeneous and Homogeneous Reaction Components in Flow Experiment,” Int. J. Chem. Kinet. 25, 67–78 (2004).
A. I. Chichinin, “Chemical Propetries of Electronically Excited Halogen Atoms X(2P 3/2, 1/2) (X = F, Cl, Br, I),” J. Phys. Chem. Ref. Data 2, 869–928 (2006).
A. I. Chichinin, T. Einfel’d, K. Maul’, and K.-Kh. Gerike, “Direct Measurement of Three-Dimensional Distributions of Cl(2R3/2, 1/2) Atoms over Rates during the Photodissociation of COCl2, CSCl2, S2Cl2, and SOCl2 Molecules,” Dokl. Akad. Nauk 407, 203–207 (2006).
K. V. Vid’ma, G. A. Bogdanchikov, A. V. Baklanov, et al., “Study of the Photodissociation of (CH3I)2 and (HI)2 Van der Waals Complexes with the Aid of a KrF Laser by the Method of Time-of-Flight Mass Spectrometry with Resolution in Ion Kinetic Energy,” Khim. Fiz. 25(2), 34–45.
A. Chichinin, T. Einfeld, K.-H. Gerike, et al., “Protodis-sociation Dynamics of SOCl2,” Phys. Chem. 7, 301–309 (2005).
G. A. Bogdanchikov, A. V. Baklanov, and D. H. Parker, “The Substitution Reactions RH + O2 → RO2 + H: Transition State Theory Calculations Based on the ab initio and DFT Potential Energy Surface,” Chem. Phys. Lett. 385, 486–490 (2004).
A. M. Zvyagintsev and G. M. Kruchenitskii, “Relationship between Total Ozone Content in the Northern Hemisphere and the Arctic and North Atlantic Oscillations,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 39, 505–509 (2003) [Izv., Atmos. Ocean. Phys. 39, 456–460 (2003)].
V. I. Bekoryukov, V. N. Glazkov, E. A. Zhadin, et al., “Assessment of the Contributions of Dynamic and Chemical Factors to Variations in the Total Ozone Content in the Extratropical Latitudes of the Northern Hemisphere,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 40, 397–402 (2004) [Izv., Atmos. Ocean. Phys. 40, 351–355 (2004)].
V. N. Marichev, I. L. Galkina, and G. M. Kruchenitskii, “Influence of Global Geophysical Processes on the Formation of the Vertical Distribution of Ozone and Temperature over Western Siberia,” Meteorol. Gidrol., No. 11, 44–53 (2003).
A. N. Gruzdev and G. P. Brasseur, “Influence of the 11-Year Solar Cycle on Characteristics of the Annual Cycle of Total Ozone,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 43, 379–391 (2007) [Izv., Atmos. Ocean. Phys. 43, 344–356 (2007)].
S. P. Smyshlyaev, V. Ya. Galin, P. A. Zimenko, and A. P. Kudryavtsev, “Modeling the Effect of Variations in Spectral Fluxes of Solar Radiation Caused by Solar Activity on the Atmospheric Ozone Content,” Meteorol. Gidrol., No. 8, 25–37 (2005).
I. G. Dyominov and A. M. Zadorozhnyi, “Contribution of Natural and Anthropogenic Factors to Long-Term Changes in the Earth’s Ozone Layer at the End of the 20th Century,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 41,51–65 (2005)) [Izv., Atmos. Ocean. Phys. 41, 43–55 (2005)].
I. K. Larin, “On the Contribution of Natural Facors to the Atmospheric Ozone Trend in 1979–1990,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 42, 285–288 (2006) [Izv., Atmos. Ocean. Phys. 42, 262–264 (2006)]
A. E. Ulanovskii, A. N. Luk’yanov, V. A. Yushkov, et al., “Estimation of the Chemical Loss of Ozone in the Antarctic Atmosphere in the 1999 Winter-Spring Season from Direct Measurements and Simulations,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 40, 776–785 (2004) [Izv., Atmos. Ocean. Phys. 40, 695–703 (2004)].
V. F. Radionov and E. N. Rusina, “Measurements of the Total Ozone Content in the Central Arctic Basin,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 42, 716–719 (2006) [Izv., Atmos. Ocean. Phys. 42, 658–662 (2006)].
Yu. E. Ozolin, I. L. Karol’, A. A. Kiselev, and V. A. Zubov, “Trajectory Modeling of Air Mass Transport and Photochemistry in the Antarctic Stratospheric Polar Vortex,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 39, 291–303 (2003) [Izv., Atmos. Ocean. Phys. 39, 444–455 (2003)].
P. N. Vargin and E. A. Zhadin, “Effect of Atratospheric Warming on the Antarctic Ozone Hole in 2002,” Meteorol. Gidrol., No. 8, 36–45 (2004).
G. P. Gushchin, “Ozone-Hole Theory,” Opt. Atmos. Okeana 17, 583–597 (2004).
I. K. Larin and A. A. Ugarov, “Climatic Prognosis for 2000–2100: II. Role of Atmospheric Chemical Processes in Climate Changes,” Khim. Fiz. 22(4), 21–28 (2003).
G. A. Zherebtsov, V. A. Kovalenko, S. I. Molodykh, and O. A. Rubtsova, “Model of Solar-Activity Impact on Climatic Characteristics of the Earth’s Troposphere,” Opt. Atmos. Okeana 18, 1042–1050 (2005).
E. A. Kasatkina, O. I. Shumilov, and A. G. Kanat’ev, “Manifestations of the Cycles of Solar Activity in the Atmosphere of Northern Atlantic and Europe,” Meteorol. Gidrol., No. 1, 55–59 (2006).
G. A. Zherebtsov, V. A. Kovalenko, and S. I. Molodykh, “Radiation Balance of the Atmosphere and Climatic Manifestations of Solar Variability,” Opt. Atmos. Okeana 17, 1003–1017 (2004).
L. L. Golubyatnikov, I. I. Mokhov, E. A. Denisenko, and V. A. Tikhonov, “Model Estimates of Climate Change Impact on the Vegetation Cover and Atmospheric Carbon Sink,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 41, 22–32 (2005) [Izv., Atmos. Ocean. Phys. 41, 19–28 (2005)].
S. L. Bondarenko, V. V. Zuev, N. E. Zueva, and M. A. Bondarenko, “Effect of the Ozonosphere’s Oscillations and Related Solar UV-B Radiation on the Growth and Productivity of Coniferous Forests,” Opt. Atmos. Okeana 18, 120–123 (2005).
V. V. Zuev, B. D. Belan, N. E. Zueva, et al., “Relationship of the Carbon Dioxide Sink from the Atmosphere over Siberian to Boreal Forests to the Ozonosphere’s Oscillations,” Opt. Atmos. Okeana 18, 618–620 (2005).
V. V. Zuev, N. E. Zueva, and S. L. Bondarenko, “Influence of the Ozonosphere’s Long-Period Oscillations on Variations in the Global CO2 Content in the Atmosphere,” Opt. Atmos. Okeana 18, 621–626 (2005).
A. N. Gruzdev and G. P. Brasseur, “Long-Term Changes in the Mesosphere Calculated by a Two-Dimensional Model,” J. Geophys. Res. 110, doi: 10.1029/2003JD004410, D03304 (2005).
P. F. Demchenko, A. V. Eliseev, M. M. Arzhanov, and I. I. Mokhov, “Impact of Global Warming Rate on Permafrost Degradation,” Izv. Akad. Nauk, Fiz. Atmos. Okeana 42(1), 35–43 (2006)) [Izv., Atmos. Ocean. Phys. 42, 32–39 (2006)].
E. K. Mol’kentin, E. D. Nadezhina, and O. B. Shklyarevich, “Model Estimations of the Effect of Cover on Permafrost Degradation during Climate Warming,” Meteorol. Gidrol., No. 3, 87–95 (2003).
Yu. A. Izrael’, A. V. Pavlov, Yu. A. Anokhin, et al., “Statistical Estimates for Climate-Element Variations in Russian Permafrost Regions,” Meteorol. Gidrol., No. 5, 27–38 (2006).
A. V. Shcherbakov and V. V. Malakhova, “Modeling the Spatial Distribution of Methanehydrates in the World Ocean and of the Methane Flux to the Atmosphere,” Opt. Atmos. Okeana 19, 530–535 (2006).
K. Ya. Kondrat’ev, “Aerosol and Climate: Current State and Prospects for Developments: 1. Aerosol Formation and Properties and Their Transformation,” Opt. Atmos. Okeana 19, 5–22 (2006).
K. Ya. Kondrat’ev, “Aerosol and Climate: Current State and Prospects for Developments: 3. Aerosol Radiation Disturbing Impact,” Opt. Atmos. Okeana 19, 565–575 (2006).
K. Ya. Kondrat’ev, “Aerosol and Climate: Current State and Prospects for Developments: 2. ACE-Asia Field Observation Experiment,” Opt. Atmos. Okeana 19, 375–395 (2006).
I. A. Gorchakova, P. P. Anikin, and E. V. Romashova, “Estimations of the Aerosol Radiation Forcing from Measurements at the IAP RAS Zvenigorod Scientific Station in March 2004,” Opt. Atmos. Okeana 19, 481–483 (2006).
V. V. Zuev, V. D. Burlakov, A. V. El’nikov, and A. V. Nevzorov, “Lidar Observations of the Midlatitudinal Stratospheric Aerosol Layer over a Long Seismically Quiet Period,” Opt. Atmos. Okeana 19, 598–603 (2006).
V. V. Zuev, “Relationship between Siberian Climate Warmings in the 20th Century and the Activity of Tropical Volcanoes,” Opt. Atmos. Okeana 19, 887–893 (2006).
K. Ya. Kondrat’ev, “From Nano- to Global Scales: Properties, Formation Processes, and Consequences of Actions of Atmospheric Aerosol: 7. Aerosol Radiation Disturbing Impact on Climate,” Opt. Atmos. Okeana 18, 535–556 (2005).
V. V. Bychkov, V. N. Marichev, G. G. Matvienko, and B. M. Shevtsov, “Mechanisms of Forming Aerosol Layers in the Stratosphere in the Periods of Increased Magnetic Activity,” Opt. Atmos. Okeana 18, 1083–1088 (2005).
K. Ya. Kondrat’ev, “Atmospheric Aerosol as a Climate-Forming Atmospheric Component: 1. Properties of Different Types of Aerosols,” Opt. Atmos. Okeana 17, 5–24 (2004).
K. Ya. Kondrat’ev, “Atmospheric Aerosol as a Climate-Forming Atmospheric Component: 2. Remote Sensing of the Global Spatiotemporal Variability of Aerosol and Its Impact on Climate,” Opt. Atmos. Okeana 17, 25–35 (2004).
K. Ya. Kondrat’ev, “From Nano- to Global Scales: Properties, Formation Processes, and Consequences of Actions of Atmospheric Aerosol: 1. Field Observation Experiments (Africa and Asia),” Opt. Atmos. Okeana 17, 699–714 (2004).
K. Ya. Kondrat’ev, “From Nano- to Global Scales: Properties, Formation Processes, and Consequences of Actions of Atmospheric Aerosol: 1. Field Observation Experiments (America, Western Europe, and High Latitudes),” Opt. Atmos. Okeana 17, 715–742 (2004).
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Original Russian Text © I.K. Larin, 2009, published in Izvestiya AN. Fizika Atmosfery i Okeana, 2009, Vol. 45, No. 2, pp. 209–217.
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Larin, I.K. Russian investigations in atmospheric chemistry for 2003–2006. Izv. Atmos. Ocean. Phys. 45, 198–206 (2009). https://doi.org/10.1134/S0001433809020054
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DOI: https://doi.org/10.1134/S0001433809020054