Abstract
The results of an experimental investigation of low-temperature optical spectra and phase relaxation of electronic excitations of Pr3+ impurity ions in a Y2SiO5 crystal are reported. It is established that at low temperatures spectral lines are broadened by a mechanism that is uncharacteristic for crystals and is due to the interaction of impurity ions with two-level systems. The constants characterizing the interaction of Pr3+ impurity ions with phonons and two-level systems are found.
Similar content being viewed by others
References
V. M. Agranovich and R. M. Hochstrasser [Eds.], Spectroscopy and Excitation Dynamics of Condensed Molecular Systems (Elsevier, N. Y., 1983) [Nauka, Moscow, 1987].
P. De Bree and D. A. Wiersma, J. Chem. Phys. 70, 790 (1979).
I. S. Osad’ko, Usp. Fiz. Nauk 128, 31 (1979) [Sov. Phys. Usp. 22, 311 (1979)].
A. A. Kaplyanskii and R. M. Macfarlane [Eds.], Spectroscopy of Solids Containing Rare Earth Ions (North-Holland, Amsterdam, 1987).
É. A. Manykin and V. V. Samartsev, Optical Echo Spectroscopy (Nauka, Moscow, 1984).
K. M. Macfarlane, J. Lumin. 45, 1 (1990).
J. L. Skinner, B. B. Laird, and L. Koot, J. Lumin. 45, 6 (1990).
É. V. Shpol’skii, Usp. Fiz. Nauk 71, 215 (1960) [Sov. Phys. Usp. 3, 372 (1960)].
R. I. Personov, B. I. Al’shits, and L. A. Bykovskaya, Zh. Éksp. Teor. Fiz. 65, 1825 (1973) [Sov. Phys. JETP 38, 912 (1974)].
M. Stoneham, Rev. Mod. Phys. 41, 82 (1969).
R. Jankowiak and G. J. Small, Science 237, 618 (1987).
H. C. Meijers and D. A. Wiersma, J. Chem. Phys. 101, 6927 (1994).
I. S. Osad’ko, Phys. Rep. 206, 43 (1991).
I. S. Osad’ko, Adv. Polym. Sci. 114, 123 (1994).
R. Flach, D. S. Hamilton, P. S. Selzer et al., Phys. Rev. Lett. 35, 1034 (1975).
P. S. Selzer, D. S. Hamilton, and W. M. Yen, Phys. Rev. Lett. 38, 858 (1977).
P. W. Anderson, B. I. Halperin, and C. M. Varma, Philos. Mag. 25, 1 (1972).
W. A. Phillips, J. Low Temp. Phys. 7, 351 (1972).
A. J. Horsewill, P. J. McDonald, and D. Vijayaraghavan, J. Chem. Phys. 100, 1889 (1994).
J. L. Skinner and H. P. Trommsdorff, J. Chem. Phys. 89, 897 (1988).
A. M. Alsanoosi and A. J. Horsewill, Chem. Phys. 160, 25 (1992).
J. P. Sethna, Phys. Rev. 24, 698 (1981).
C. P. Flynn and A. M. Stoneham, Phys. Rev. 1, 3966 (1970).
M. Neumann, M. R. Johnson, and H. P. Trommsdorff, J. Lumin. 66–67, 146 (1996).
B. A. Maksimov, V. V. Ilyukhin, Yu. A. Kharitonov et al., Kristallografiya 15, 926 (1970) [Sov. Phys. Crystallogr. 15, 806 (1970)].
A. M. Tkachuk, A. K. Przhevusskii, L. G. Morozova et al., Opt. spektrosk. 60, 288 (1986) [Opt. Spectrosc. 60, 176 (1986)].
M. Mitsunaga, T. Takagahara, K. Yano et al., Phys. Rev. Lett. 68, 3216 (1992).
N. V. Kuleshov, V. P. Mikhailov, S. A. Radkevich et al., Opt. spektrosk. 77, 244 (1994) [Opt. Spectrosc. 77, 220 (1994)].
K. Holliday, M. Croci, E. Vanthey et al., Phys. Rev. 47, 14741 (1993).
Yu. V. Malyukin, N. L. Pogrebnyak, V. P. Seminozhenko et al., Zh. Éksp. Teor. Fiz. 108, 485 (1995) [JETP 81, 260 (1995)].
P. N. Zhmurin, N. L. Pogrebnyak, V. P. Seminozhenko et al., Ukr. Fiz. Zh. 39, 791 (1994).
I. B. Bersuker, Electronic Structure and Properties of Coordination Compounds (Khimiya, Leningrad, 1986).
W. H. Flygare, Molecular Structure and Dynamics (Prentice-Hall, Englewood Cliffs, N. J., 1978) [Russian translation, Mir, Moscow, 1982, Vol. 1].
W. N. Yen, W. C. Scot, and A. L. Schawlow, Phys. Rev. 136, 271 (1964).
C. A. Morrison and R. P. Leavit, J. Chem. Phys. 71(6), 2366 (1979).
H. H. Caspers, H. E. Rast, and R. A. Buchanan, J. Chem. Phys. 43(6), 2124 (1965).
S. Matthies and D. Welsch, Phys. Status Solidi B 6S, 125 (1975).
B. R. Reddy and L. E. Erickson, Phys. Rev. 27(9), 5217 (1983).
E. S. Makarov, Isomorphism of Atoms in Crystals (Atomizdat, Moscow, 1973).
N. Takeuchi, J. Lumin. 12/13, 743 (1978).
A. M. Stoneham, The Theory of Defects in Solids: The Electronic Structure of Defects in Insulators and Semiconductors (Clarendon Press, Oxford, 1975) [Russian translation, Mir, Moscow, 1978, Vol. 1).
Author information
Authors and Affiliations
Additional information
Zh. Éksp. Teor. Fiz. 115, 704–715 (February 1999)
Rights and permissions
About this article
Cite this article
Borisov, R.S., Grinev, B.V., Malyukin, Y.V. et al. Echo spectroscopy of two-level systems in a Y2SiO5: Pr3+ crystal. J. Exp. Theor. Phys. 88, 385–391 (1999). https://doi.org/10.1134/1.558807
Received:
Issue Date:
DOI: https://doi.org/10.1134/1.558807