Skip to main content
Log in

The observability of possible atmospheric removal processes for chlorfluorocarbons 11 and 12

  • Article
  • Published:

From Nature

View current issue Submit your manuscript

Abstract

The existence of tropospheric sinks for CFCs 11 and 12 would have a large impact on projected stratospheric ozone effects. The existence of such sinks, distinct from no sinks, cannot at present be discerned from atmospheric measurements. As presently analysed, tens of years may pass before such a distinction would be possible. This article scrutinises transient mechanisms that could contribute to accomplishing this critical distinction in 10 yr or less.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. Stolarski, R. S. & Cicerone, R. J. Can. J. Chem. 52, 1610–1615 (1974).

    Article  CAS  Google Scholar 

  2. Molina, M. J. & Rowland, F. S. Nature 249, 810–812 (1974).

    Article  ADS  CAS  Google Scholar 

  3. Crutzen, P. Geophys. Res. Lett. 1, 205–208 (1974).

    Article  ADS  CAS  Google Scholar 

  4. Wofsy, S. C. & McElroy, M. B. Can. J. Chem. 52, 1582–1591 (1974).

    Article  CAS  Google Scholar 

  5. Rowland, F. S. & Molina, M. J. Rev. Geophys. Space Phys. 13, 1 (1975).

    Article  ADS  CAS  Google Scholar 

  6. Crutzen, P. J. & Isaksen, I. S. A. Impact of the chlorocarbon industry on the ozone layer (preprint 1975).

    Google Scholar 

  7. Wofsy, S. C., McElroy, M. B. & Sze, N. D. Science 187, 535 (1975).

    Article  ADS  CAS  Google Scholar 

  8. Gelinas, R. J. Address to Manufacturing Chemists Association Meeting, Andover, Mass. (June 10, 1975).

  9. Scientific review: The effect of fluorocarbons on the concentration of atmospheric ozone (Technical Panel on Fluorocarbon Research, Manufacturing Chemists Association, March 1, 1976).

  10. Towland, F. S. & Molina, M. J. J. Phys. Chem. (in the press).

  11. Sundararaman, N. Initial summary of upper atmospheric data, Rep. FAA-EQ-76-4 (US Dep. Transportation Federal Aviation Administration Office of Environmental Quality, April, 1976).

    Google Scholar 

  12. McCarthy, R. L. Am. Chem. Soc. Mg. (Philadelphia, Pa. 1975).

  13. Chang, J. S. Proc. 3rd Conf. on CIAP, DOT-TSC-OST-74-15, 330–341 (Department of Transportation, Cambridge, Mass., 1974).

    Google Scholar 

  14. Jesson, J. P., Meakin, P. & Glasgow, L. C. The fluorocarbon-ozone theory II: tropospheric lifetimes. An experimental estimate of the tropospheric lifetime of CCI3F (preprint 1976).

    Google Scholar 

  15. Panel on Atmospheric Chemistry Halocarbons: Effects on Stratospheric Ozone (Committee on Impacts of Stratospheric Change, National Academy of Science, Washington, DC, 1976).

  16. U. S. Standard Atmosphere, Supplement (1966) US Government Printing Office, Washington, D. C., (1962).

  17. Gelinas, R. J., Bender, C., Ellsaesser, H., Ide, R. & MacCracken, M. C. Lawrence Livermore Lab. Rep. UCLLL 00736 (1971).

  18. MacCracken, M. C., Crawford, T. V., Peterson, K. R. & Knox, J. B. Proc. Joint Automatic Control Conf., Stanford University (August, 1972).

    Google Scholar 

  19. Gelinas, R. J. J. comput. Phys. 9, 222 (1972).

    Article  ADS  CAS  Google Scholar 

  20. Chang, J. S., Hindmarsh, A. C. & Madsen, N. K. in Stiff Differential Systems (ed. Willoughby, R. A. ) 51–65 (Plenum, New York, 1974).

    Book  Google Scholar 

  21. Grobecker, A. J. (ed.) CIAP Monogr. 3, DOT-TST-75-53, 5–48 (Dep. Transportation, Washington, DC, 1975).

  22. MacCracken, M. C. & Sauter, G. D. Lawrence Livermore Lab. Rep. UCRL-51920, 1 & 2 (1975).

  23. MacCracken, M. C., Duewer, W. H., Grant, K. E., Walton, J. J. & Wenbbles, D. J. Lawrence Livermore Lab. Rep. UCRL-77475. Parts 1 and 2 (1975).

  24. Luther, F. & Gelinas, R. J. geophys. Res. 81, 1125 1976).

    Article  ADS  CAS  Google Scholar 

  25. Gelinas, R. J. Proc. Int. Conf. Structure, Composition and General Circulation of the Upper and Lower Atmospheres and Possible Anthropogenic Perturbations. Melbourne, Australia, (January 14–25, 1974).

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Rights and permissions

Reprints and permissions

About this article

Cite this article

Gelinas, R., Hall, D. & Nelson, R. The observability of possible atmospheric removal processes for chlorfluorocarbons 11 and 12. Nature 266, 229–231 (1977). https://doi.org/10.1038/266229a0

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1038/266229a0

  • Springer Nature Limited

Navigation