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Durable washable wearable antibacterial thermoplastic polyurethane/carbon nanotube@silver nanoparticles electrospun membrane strain sensors by multi-conductive network

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Abstract

Highly stretchable strain sensors with high sensitivity, wide sensing range, and high durability have broader application prospects in the fields of wearable sensors, electronic skin, and soft robots. However, it is still challenging to fabricate strain sensors with high sensitivity, wide working range, excellent durability, and antibacterial properties. Herein, a highly stretchable and porous thermoplastic polyurethane/carbon nanotube@silver nanoparticles (TPU/CNT@AgNPs) strain sensor was facilely prepared by electrospinning combined with dip coating CNT and reduction of AgNO3. The TPU/CNT@AgNPs strain sensor exhibited high sensitivity (the maximum gauge factor of 930), favorable conductivity (539.7 S m−1), wide sensing range (0.1 ~ 500% strain), a fast response time (100 ms at 1% strain), high dynamic response performance (2400 mm/min), air permeability, and antibacterial activity, due to the synergetic effect of the multi-conductive network between CNT and AgNPs. Benefiting from the in situ generated AgNPs and the π–π interaction between the benzene ring structure of TPU and CNT, the TPU/CNT@AgNPs strain sensor exhibited excellent durability (1400 cycles for 200% strain) and could work even after being immersed in harsh conditions (acidic and alkaline solution). Besides, the strain sensor can be successfully employed in monitoring human motion from tiny pulse beats to large bending movements of fingers, wrists, and knees. This work provides a feasible approach to preparing a strain sensor with outstanding overall performance, which has a perspective and alluring application in the realm of wearable electronics.

Graphical Abstract

Highly stretchable TPU/CNT@AgNPs strain sensor with high sensitivity was prepared by dipping CNT and AgNPs reduction on electrospun TPU mat.

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The TPU/3CNT@AgNPs-4 stain sensor is breathable, and when worn on the skin, it can provide a breathable environment for the skin and improve comfort. This is just a subjective guess without actual measurement.

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Funding

This work was supported by National Natural Science Foundation of China (No. 52203034 and 52273032), Natural Science Foundation of Fujian Province (2020J05190 and 2020J02007), Major Science and Technology Project of Fuzhou City (2021-ZD-285), and Scientific Research Foundation of Fujian University of Technology (GY-Z19048, GY-Z21014, and GY-Z17073).

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Authors and Affiliations

  1. Key Laboratory of Polymer Materials and Products, College of Materials Science and Engineering, Fujian University of Technology, Fuzhou, 350118, China

    An Huang, Yu Guo, Yiwei Zhu, Tingjie Chen, Zhenyu Yang, Yao Song, Shuqiang Peng & Xiangfang Peng

  2. CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research On the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, China

    Shuqiang Peng

  3. Mechanical and Construction Engineering, Faculty of Engineering and Environment, Northumbria University, Newcastle Upon Tyne, NE1 8ST, UK

    Priyanka Wasnik, Handong Li & Zhanhu Guo

  4. College of Materials Science and Engineering, Taiyuan University of Science and Technology, Taiyuan, 030024, China

    Handong Li

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  1. An Huang
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Contributions

An Huang: investigation, resources, validation, and writing—review and editing. Yu Guo: investigation, data curation, validation, and writing—original draft. Yiwei Zhu: methodology and data curation. Tingjie Chen: methodology and formal analysis. Zhenyu Yang: investigation and software. Yao Song: investigation and software. Priyanka Wasnik: writing—original draft and format checking. Handong Li: data analysis. Shuqiang Peng: conceptualization, methodology, and writing—review and editing. Zhanhu Guo: supervision and writing—original draft. Xiangfang Peng: supervision, methodology, conceptualization, and funding acquisition.

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Huang, A., Guo, Y., Zhu, Y. et al. Durable washable wearable antibacterial thermoplastic polyurethane/carbon nanotube@silver nanoparticles electrospun membrane strain sensors by multi-conductive network. Adv Compos Hybrid Mater 6, 101 (2023). https://doi.org/10.1007/s42114-023-00684-7

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