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Fungus bran-derived nanoporous carbon with layered structure and rime-like support for enhanced symmetric supercapacitors

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Abstract

Integrating and utilizing natural resources rationally is an important strategy for sustainable development. Herein, a novel nanoporous carbon material with rime scenery-like support was firstly established, in which waste biomass fungus bran was skillfully selected as the layered structure carbon skeletons for loading carboxymethyl cellulose derived carbon particles. The dual biomass-derived carbon with the aid of activating by KMnO4 has a unique structure and favorable electrical conductivity. The resulting sample also has a high micropore ratio, which is optimum for the formation of double layer in aqueous electrolyte. Profiting from hierarchical nanopore structure and nitrogen self-doping, the optimized carbon electrode exhibited excellent specific capacitance of 407 F g−1 at 0.5 A g−1, remarkable rate characteristic, and superior cycling performance (96.9% remained after 5000 cycles). More importantly, the assembled symmetric supercapacitor exhibited a high energy density of 11.4 Wh kg−1 and outstanding electrochemical performance in aqueous electrolyte, which benefited from well-connected networks and multipath channels. This research realizes the utilization of waste biomass in carbon-based electrodes and offers the basis of preparation method for the next generation of sustainable energy storage devices.

Graphic abstract

The fabricated rime scenery-like nanoporous carbon materials exhibit ultra-high specific capacitance and the symmetric supercapacitor possesses a high energy density and power density.

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Acknowledgements

This work was supported by the National Natural Science Foundation of China (No. 31670592, 32071713), and the Outstanding Youth Foundation Project of Heilongjiang Province (JQ2019C001).

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  1. Keqi Qu and Weicong Wang are equally contributed to this work.

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  1. Key Laboratory of Bio-Based Material Science and Technology, Material Science and Engineering College, Northeast Forestry University, Harbin, 150040, China

    Keqi Qu, Weicong Wang, Cai Shi, Zhe Sun, Houjuan Qi, Junming Shi, Shuai Yang & Zhanhua Huang

  2. Integrated Composites Laboratory (ICL), Department of Chemical and Bimolecular Engineering, University of Tennessee, Knoxville, TN, 37996, USA

    Zhanhu Guo

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Qu, K., Wang, W., Shi, C. et al. Fungus bran-derived nanoporous carbon with layered structure and rime-like support for enhanced symmetric supercapacitors. J Nanostruct Chem 11, 769–784 (2021). https://doi.org/10.1007/s40097-021-00448-z

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