Abstract
Advanced technology has led to the generation of the massive amount of electrical and electronic wastes, including compact discs and digital versatile discs. These optical discs are often ended up in landfills and incinerators, resulting in severe environmental degradation. This research aims to recover polycarbonate from waste optical discs and exploring its potential as a sorbent for the removal of mercury in water. The recovered polycarbonate was nitrated to enhance its efficiency in removing mercury (II) ion. The nitrated polycarbonate was characterized using Fourier-transform infrared spectroscopy, field emission scanning electron microscopy, thermogravimetric analysis, energy-dispersive X-ray spectroscopy and Brunauer–Emmett–Teller surface area analysis. Response surface methodology was employed to investigate the effects of agitation rate, contact time, pH, initial concentration, sorbent dosage on the mercury (II) ion removal efficiency via a central composite design. According to the quadratic model, an optimum response can be achieved at 188.6 rpm of agitation, 150 min of contact time, pH 7.55 and 1.50 mg/L of initial mercury (II) ion concentration. The adsorption process was found to follow the Freundlich isotherm model, and the adsorption mechanism was found to obey the pseudo-second-order kinetic model that indicates the chemisorption process. The results of this study showed that the nitrated PC with a maximum adsorption capacity of 0.289 mg/g has the potential to be used as a sorbent in water treatment for the removal of mercury (II) ion in water.
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Abas SNA, Ismail MHS, Kamal ML, Izhar S (2013) Adsorption process of heavy metals by low-cost adsorbent: a review. World Appl Sci J 28:1518–1530. https://doi.org/10.5829/idosi.wasj.2013.28.11.1874
Achilias DS, Antonakou EV, Koutsokosta E, Lappas AA (2009) Chemical recycling of polymers from waste electric and electronic equipment. J Appl Polym Sci 114:212–221. https://doi.org/10.1002/app.30533
Al-Ghouti MA, Da’ana D, Abu-Dieyeh M, Khraisheh M (2019) Adsorptive removal of mercury from water by adsorbents derived from date pits. Sci Rep-UK 9:1–15. https://doi.org/10.1038/s41598-019-51594-y
Al-Hamouz OCS, Sweileh BA, Al-Salah HA (2006) Synthesis and characterization of polycarbonates by melt-phase interchange reactions with alkylene and arylene diphenyl dicarbonates. J Appl Polym Sci 102:3597–3609. https://doi.org/10.1002/app.23996
Alimohammady M, Jahangiri M, Kiani F, Tahermansouri H (2017) Highly efficient simultaneous adsorption of Cd (II), Hg (II) and As (III) ions from aqueous solutions by modification of graphene oxide with 3-aminopyrazole: central composite design optimization. New J Chem 41:8905–8919. https://doi.org/10.1039/C7NJ01450C
Anbia M, Amirmahmoodi S (2016) Removal of Hg (II) and Mn (II) from aqueous solution using nanoporous carbon impregnated with surfactants. Arab J Chem 9:S319–S325. https://doi.org/10.1016/j.arabjc.2011.04.004
Delpech MC, Coutinho FM, Habibe MES (2002) Bisphenol A-based polycarbonates: characterization of commercial samples. Polym Test 21:155–161. https://doi.org/10.1016/S0142-9418(01)00063-0
Dewez JL, Deren A, Rouxhet PG, Schneider YJ, Legras R (1991) Surface study of polycarbonate membranes used as a substratum for animal cell culture. Surf Interface Anal 17:499–502. https://doi.org/10.1002/sia.740170715
Fierro V, Torné-Fernández V, Montané D, Celzard A (2008) Adsorption of phenol onto activated carbons having different textural and surface properties. Microporous Mesoporous Mater 111:276–284. https://doi.org/10.1016/j.micromeso.2007.08.002
Grömping U (2015) Augmented half normal effects plots in the presence of a few error degrees of freedom. Qual Reliab Eng Int 31:1185–1196. https://doi.org/10.1002/qre.1842
Guo YF, Deng J, Zhu JY, Zhou XJ, Bai RB (2016) Removal of mercury(II) and methylene blue from a wastewater environment with magnetic graphene oxide: adsorption kinetics, isotherms and mechanism. RSC Adv 6:82523–82536. https://doi.org/10.1039/c6ra14651a
Herman P, Fábián I, Kalmár J (2020) Mesoporous silica–gelatin aerogels for the selective adsorption of aqueous Hg(II). ACS Appl Nano Mater 3:195–206. https://doi.org/10.1021/acsanm.9b01903
Hong S, Lyonga FN, Kang J, Seo E, Lee C, Jeong S, Hong S, Park S (2020) Synthesis of Fe-impregnated biochar from food waste for Selenium(VI) removal from aqueous solution through adsorption: Process optimization and assessment. Chemosphere 252:126475. https://doi.org/10.1016/j.chemosphere.2020.126475
Jafari SA, Cheraghi S (2014) Mercury removal from aqueous solution by dried biomass of indigenous Vibrio parahaemolyticus PG02: kinetic, equilibrium, and thermodynamic studies. Int Biodeterior Biodegrad 92:12–19. https://doi.org/10.1016/j.ibiod.2014.01.024
Jain S, Chattopadhyay S, Jackeray R, Abid CZ, Kohli GS, Singh H (2012) Highly sensitive detection of Salmonella typhi using surface aminated polycarbonate membrane enhanced-ELISA. Biosens Bioelectron 31:37–43. https://doi.org/10.1016/j.bios.2011.09.031
Jeon C, Solis KL, An H, Hong Y, Igalavithana AD, Ok YS (2020) Sustainable removal of Hg(II) by sulfur-modified pine-needle biochar. J Hazard Mater 388:122048. https://doi.org/10.1016/j.jhazmat.2020.122048
Krishnaiah K, Shahabudeen P (2012) Applied design of experiments and Taguchi methods. PHI Learning Pvt Ltd, New Delhi
Khor SW, Lee YK, Abas MRB, Tay KS (2017) Application of chalcone-based dithiocarbamate derivative incorporated sol–gel for the removal of Hg (II) ion from water. J Sol–Gel Sci Technol 82:834–845. https://doi.org/10.1007/s10971-017-4362-7
Kim MY, Seo H, Lee TG (2020) Removal of Hg(II) ions from aqueous solution by poly(allylamine-co-methacrylamide-co-dimethylthiourea). J Ind Eng Chem 84:82–86. https://doi.org/10.1016/j.jiec.2019.12.023
Larosa C, Patra N, Salerno M, Mikac L, Meri RM, Ivanda M (2017) Preparation and characterization of polycarbonate/multiwalled carbon nanotube nanocomposites. Beilstein J Nanotechnol 8:2026. https://doi.org/10.3762/bjnano.8.203
Leone C, Genna S, Caggiano A (2015) Resource efficient low power laser cleaning of compact discs for material reuse by polycarbonate recovery. CIRP J Manuf Sci Tec 9:39–50. https://doi.org/10.1016/j.cirpj.2015.01.005
Noorimotlagh Z, Mirzaee SA, Martinez SS, Alavi S, Ahmadi M, Jaafarzadeh N (2019) Adsorption of textile dye in activated carbons prepared from DVD and CD wastes modified with multi-wall carbon nanotubes: Equilibrium isotherms, kinetics and thermodynamic study. Chem Eng Res Des 141:290–301. https://doi.org/10.1016/j.cherd.2018.11.007
Ogończyk D, Jankowski P, Garstecki P (2012) Functionalization of polycarbonate with proteins; open-tubular enzymatic microreactors. Lab Chip 12:2743–2748. https://doi.org/10.1039/c2lc40204a
Petrie B, Lopardo L, Proctor K, Youdan J, Barden R, Kasprzyk-Hordern B (2019) Assessment of bisphenol-A in the urban water cycle. Sci Total Environ 650:900–907. https://doi.org/10.1016/j.scitotenv.2018.09.011
Ravindran B, Kassim M, Mohamed M (2019) Screening of medium constituents for the cultivation of scenedesmus dimorphus UTEX 1237 using 2k factorial design approach. IOP Conf Ser Mater Sci Eng 716:012003. https://doi.org/10.1088/1757-899X/716/1/012003
Tran L, Wu PX, Zhu YJ, Yang L, Zhu NW (2015) Highly enhanced adsorption for the removal of Hg(II) from aqueous solution by Mercaptoethylamine/Mercaptopropyltrimethoxysilane functionalized vermiculites. J Colloid Interface Sci 445:348–356. https://doi.org/10.1016/j.jcis.2015.01.006
Vani K, Thomas S, Prabhawathi V, Boobalan T, Sawant SN, Doble M (2013) In vitro biocompatiblity of modified polycarbonate as a biomaterial. Colloids Surf B 108:191–198. https://doi.org/10.1016/j.colsurfb.2013.01.067
Verma A, Chakraborty S, Basu J (2006) Adsorption study of hexavalent chromium using tamarind hull-based adsorbents. Sep Purif Technol 50:336–341. https://doi.org/10.1016/j.seppur.2005.12.007
Weeden JGS, Soepriatna NH, Wang N-HL (2015) Method for efficient recovery of high-purity polycarbonates from electronic waste. Environ Sci Technol 49:2425–2433. https://doi.org/10.1021/es5055786
Xu M, Yin P, Liu X, Dong X, Yang Y, Wang Z, Qu R (2013) Optimization of biosorption parameters of Hg (II) from aqueous solutions by the buckwheat hulls using respond surface methodology. Desalin Water Treat 51:4546–4555. https://doi.org/10.1080/19443994.2013.770591
Yilmaz S, Sahan T, Karabakan A (2017) Response surface approach for optimization of Hg(II) adsorption by 3-mercaptopropyl trimethoxysilane-modified kaolin minerals from aqueous solution. Korean J Chem Eng 34:2225–2235. https://doi.org/10.1007/s11814-017-0116-z
Zarnoch KP (1994) Surface functionalization and metallization of Lexan® polycarbonate. J Adhes Sci Technol 8:501–509. https://doi.org/10.1163/156856194X00195
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The authors gratefully thank Ministry of Education Malaysia (FRGS FP074-2018A) and University of Malaya (PG206-2016A) for financial supports.
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Abdallah, S.A., Tay, K.S. & Low, K.H. Feasibility of mercury (II) ion removal by nitrated polycarbonate derived from waste optical discs. Int. J. Environ. Sci. Technol. 17, 4161–4170 (2020). https://doi.org/10.1007/s13762-020-02758-1
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DOI: https://doi.org/10.1007/s13762-020-02758-1