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A literature review of MOF derivatives of electromagnetic wave absorbers mainly based on pyrolysis

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Abstract

Growing electromagnetic pollution has plagued researchers in the field of electromagnetic (EM) energy dissipation for many years; it is increasingly important to solve this problem efficiently. Metal—organic frameworks (MOFs), a shining star of functional materials, have attracted great attention for their advantages, which include highly tunable porosity, structure, and versatility. MOF-derived electromagnetic wave (EMW) absorbers, with advantages such as light weight, thin matching thickness, strong capacity, and wide effective bandwidth, are widely reported. However, current studies lack a systematic summary of the ternary synergistic effects of the precursor component—structure—EMW absorption behavior of MOF derivatives. Here we describe in detail the electromagnetic (EM) energy dissipation mechanism and strategy for preparing MOF-derived EMW absorbers. On the basis of this description, the following means are suggested for adjusting the EM parameters of MOF derivatives, achieving excellent EM energy dissipation: (1) changing the metal and ligands to regulate the chemical composition and morphology of the precursor, (2) controlling pyrolysis parameters (including temperature, heating rate, and gas atmosphere) to manipulate the structure and components of derivatives, and (3) compounding with enhancement phases, including carbon nanomaterials, metals, or other MOFs.

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Acknowledgements

This work was financially supported by the Natural Science Foundation of Jiangsu Province (No. BK20221336), the Jiangsu Agricultural Science and Technology Independent Innovation Fund (No. CX(20)3041), the National Natural Science Foundation of China (No. 31971740), the Research Project of the Jiangxi Forestry Bureau (No. 202134), and the Nanping Science and Technology Planning Project (No. 2020Z001).

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  1. The authors contributed equally to this paper.

Authors and Affiliations

  1. Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Nanjing Forestry University, Nanjing, 210037, China

    Qiuyi Wang, Jie Liu, Zhichao Lou & Yanjun Li

  2. College of Materials Science and Engineering, Nanjing Forestry University, Nanjing, 210037, China

    Qiuyi Wang, Jie Liu, Zhichao Lou & Yanjun Li

  3. Henan Science & Technology Exchange Center with Foreign Countries, Zhengzhou, 450000, China

    Yadong Li

  4. College of Engineering, University of Georgia, Athens, 30605, USA

    Zhichao Lou

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  1. Qiuyi Wang
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  2. Jie Liu
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  5. Yanjun Li
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Correspondence to Zhichao Lou or Yanjun Li.

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Wang, Q., Liu, J., Li, Y. et al. A literature review of MOF derivatives of electromagnetic wave absorbers mainly based on pyrolysis. Int J Miner Metall Mater 30, 446–473 (2023). https://doi.org/10.1007/s12613-022-2562-9

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