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Preparation of NH2-MIL-101(Fe)@Viscose Spunlaced Nonwoven Porous Carbon Material for Organic Dye Adsorption

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Abstract

A kind of NH2-MIL-101(Fe)@viscose spunlaced nonwoven material (VSN) was prepared by in situ solvothermal method for the adsorption of organic dyes in wastewater and then carbonized in a tube furnace under N2 atmosphere at 300 °C to improve the adsorption performances. The results showed that the synthesized NH2-MIL-101(Fe) particles with a polyhedral structure were uniformly loaded on the VSN surface. After being carbonized, the NH2-MIL-101(Fe)@viscose spunlaced nonwoven porous carbon material (VSNC) were obtained. Compared with uncarbonized NH2-MIL-101(Fe)@VSN, the adsorption efficiency of NH2-MIL-101(Fe)@VSNC for methylene blue (MB) significantly enhanced and could reach 98.3% under the condition of water bath temperature of 30 °C and pH 9. According to adsorption thermodynamic analysis, the MB adsorption process by NH2-MIL-101(Fe)@VSNC was spontaneous. The quasi-secondary adsorption kinetic model was more suitable to describe the whole adsorption process of NH2-MIL-101(Fe)@VSNC, implying that the adsorption mechanism of NH2-MIL-101(Fe)@VSNC for MB was mainly chemical adsorption. NH2-MIL-101(Fe)@VSNC presented good structure stability and reusability during the adsorption process. After being recycled five times, the MB adsorption efficiency still maintained about 86.3%.

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Acknowledgements

This work was supported by the Zhejiang Provincial Natural Science Foundation of China (No. LTGS23E030005) and the Jiangsu Province Natural Science Foundation of China (No. BK20201182).

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Authors and Affiliations

  1. College of Textiles Science and Engineering, Zhejiang Sci-Tech University, 928 Second Avenue, Xiasha Higher Education Zone, Hangzhou, 310018, China

    Jiangli Feng, Hui Sun, Bin Yu, Xiaodong Yang, Lei Xu, Peng Liu & Xiaogang Cui

  2. Zhejiang Provincial Innovation Center of Advanced Textile Technology, Shaoxing, 312000, China

    Jiangli Feng, Hui Sun, Bin Yu, Xiaodong Yang, Lei Xu, Peng Liu & Xiaogang Cui

  3. School of Textile and Clothing and Art and Media, Suzhou Institute of Trade & Commerce, 287 Xuefu Road, Suzhou, 215009, Jiangsu, China

    Lei Xu

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  1. Jiangli Feng
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Feng, J., Sun, H., Yu, B. et al. Preparation of NH2-MIL-101(Fe)@Viscose Spunlaced Nonwoven Porous Carbon Material for Organic Dye Adsorption. Fibers Polym 24, 1983–1994 (2023). https://doi.org/10.1007/s12221-023-00163-2

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