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Low temperature oxidation of CO using alkali- and alkaline-earth metal-modified ceria-supported metal catalysts: a review

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Abstract

The present review devoted to the complete oxidation of CO using alkali- and alkaline-earth metal (AM/AEM)-modified ceria supported/mixed with noble metal and non-noble metal (NM). The AM/AEM-modified Ce supported/mixed with noble metal showed comparable CO oxidation with unmodified catalyst. However, AM/AEM-modified NM showed higher CO oxidation at lower temperature compared to the unmodified catalyst. The AM and AEM modifications were responsible for the formation of oxygen vacancies in Ce, which leads to the decrease in the CO and O2 activation barrier. The dissociative oxygen adsorption on AM/AEM-modified Ce-supported/mixed with NM favours the CO oxidation at a lower temperature. However, AM/AEM-modified Ce-supported/mixed with noble metal showed CO adsorption with formation of superoxy and peroxy species, which leads to the comparable oxidation activity. The plausible mechanism for CO oxidation is explained in detail with correlation to the characterizations.

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Acknowledgements

The WOS-A (Woman Scientist – A) grant from the Department of Science and Technology (KIRAN DIVISION) having project SR/WOS-A/CS-110/2018(G) and early career research award (ECR/2016/000823) from SERB-DST are acknowledged for financial support.

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  1. Department of Chemistry, Institute of Chemical Technology, Mumbai, 400019, India

    Jyoti Waikar & Pavan More

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  1. Jyoti Waikar
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  2. Pavan More
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Correspondence to Pavan More.

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Waikar, J., More, P. Low temperature oxidation of CO using alkali- and alkaline-earth metal-modified ceria-supported metal catalysts: a review. Bull Mater Sci 44, 263 (2021). https://doi.org/10.1007/s12034-021-02547-7

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