Skip to main content
SpringerLink
Log in

Methane combustion over Pd/Ni-Al oxide catalysts: Effect of Ni/Al ratio in the Ni-Al oxide support

  • Catalysis, Reaction Engineering
  • Published:
Korean Journal of Chemical Engineering Aims and scope Submit manuscript

Abstract

We prepared xNi-2Al oxide (x=0-1.1) supports via a hydrothermal method, and applied Pd/xNi-2Al catalysts in the catalytic methane combustion reaction. It was found that the physicochemical properties of the xNi-2Al supports varied as a function of the Ni content, and the interaction between support and impregnated Pd was also influenced by the Ni content. Furthermore, variation in the Ni content significantly affected the chemical state and reducibility of the impregnated Pd species. Finally, the catalytic activity and stability of prepared Pd/xNi-2Al catalysts in the methane combustion reaction exhibited a volcano-shaped curve as a function of Ni content, with a maximum being observed for the Pd/1.0Ni-2Al catalyst, which corresponded to the highest Pd2+ composition and reducibility.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Log in via an institution

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Institutional subscriptions

Similar content being viewed by others

References

  1. A. Bill, A. Wokaun, B. Eliasson, E. Killer and U. Kogelschatz, {i mtEnergy Convers. Manage.}, 38, S415 (1997).

    Article  CAS  Google Scholar 

  2. R. Hayes, Chem. Eng. Sci., 59, 4073 (2004).

    Article  CAS  Google Scholar 

  3. J.-H. Park, J. H. Cho, Y. J. Kim, E. S. Kim, H. S. Han and C.-H. Shin, Appl. Catal. B: Environ., 160-161, 135 (2014).

    Article  CAS  Google Scholar 

  4. A. Baylet, S. Royer, P. Marecot, J.-M. Tatibouet and D. Duprez, Appl. Catal. B: Environ., 77, 237 (2008).

    Article  CAS  Google Scholar 

  5. L. Liotta, G. Di Carlo, G. Pantaleo and G. Deganello, Catal. Commun., 6, 329 (2005).

    Article  CAS  Google Scholar 

  6. K. Huang, L. Wang, Y. Xu and D. Wu, Korean J. Chem. Eng., 34, 1366 (2017).

    Article  CAS  Google Scholar 

  7. J. Li, R. Hu, J. Zhang, W. Meng, Y. Du, Y. Si and Z. Zhang, Fuel, 178, 148 (2016).

    Article  CAS  Google Scholar 

  8. Z. Pu, H. Zhou, Y. Zheng, W. Huang and X. Li, Appl. Surf. Sci., 410, 14 (2017).

    Article  CAS  Google Scholar 

  9. K. Persson, A. Ersson, K. Jansson, N. Iverlund and S. Järås, J. Catal., 231, 139 (2005).

    Article  CAS  Google Scholar 

  10. G. Pecchi, P. Reyes, R. Gómez, T. López and J. Fierro, Appl. Catal. B: Environ., 17, L7 (1998).

    Article  CAS  Google Scholar 

  11. G. Diannan, W. Sheng, C. Zhang, Y. Zhongshan and W. Shudong, Chinese J. Catal., 29, 1221 (2008).

    Article  Google Scholar 

  12. B. Yue, R. Zhou, Y. Wang and X. Zheng, Appl. Surf. Sci., 252, 5820 (2006).

    Article  CAS  Google Scholar 

  13. L.-f. Yang, C.-k., Shi, X.-e. He and J.-x. Cai, Appl. Catal. B: Environ., 38, 117 (2002).

    Article  CAS  Google Scholar 

  14. K.-i. Fujimoto, F. H. Ribeiro, M. Avalos-Borja and E. Iglesia, J. Catal., 179, 431 (1998).

    Article  CAS  Google Scholar 

  15. D. Gao, C. Zhang, S. Wang, Z. Yuan and S. Wang, Catal. Commun., 9, 2583 (2008).

    Article  CAS  Google Scholar 

  16. J. E. Park, B. B. Kim and E. D. Park, Korean J. Chem. Eng., 32, 2212 (2015).

    Article  CAS  Google Scholar 

  17. W. Yang, D. Li, D. Xu and X. Wang, J. Nat. Gas Chem., 18, 458 (2009).

    Article  CAS  Google Scholar 

  18. T. Takeguchi, S. Aoyama, J. Ueda, R. Kikuchi and K. Eguchi, Top. Catal., 23, 159 (2003).

    Article  CAS  Google Scholar 

  19. T. Takeguchi, O. Takeoh, S. Aoyama, J. Ueda, R. Kikuchi and K. Eguchi, Appl. Catal. A: Gen., 252, 205 (2003).

    Article  CAS  Google Scholar 

  20. F. Yin, S. Ji, P. Wu, F. Zhao and C. Li, J. Catal., 257, 108 (2008).

    Article  CAS  Google Scholar 

  21. P. Marti, M. Maciejewski and A. Baiker, Appl. Catal. B: Environ., 4, 225 (1994).

    Article  CAS  Google Scholar 

  22. N. Guilhaume and M. Primet, J. Chem. Soc.-Farad. T., 90, 1541 (1994).

    Article  CAS  Google Scholar 

  23. Y. Liu, S. Wang, T. Sun, D. Gao, C. Zhang and S. Wang, Appl. Catal. B: Environ., 119-120, 321 (2012).

    Article  CAS  Google Scholar 

  24. X. Zou, Z. Rui, S. Song and H. Ji, J. Catal., 338, 192 (2016).

    Article  CAS  Google Scholar 

  25. X. Pan, Y. Zhang, Z. Miao and X. Yang, J. Energy Chem., 22, 610 (2013).

    Article  CAS  Google Scholar 

  26. H. Widjaja, K. Sekizawa, K. Eguchi and H. Arai, Catal. Today, 47, 95 (1999).

    Article  CAS  Google Scholar 

  27. M. A. Hoque and K. Kim, Korean J. Chem. Eng., 31(8), 1316 (2014).

    Article  CAS  Google Scholar 

  28. R. Burch, F. Urbano and P. Loader, Appl. Catal. A: Gen., 123, 173 (1995).

    Article  CAS  Google Scholar 

  29. A. Boumaza, L. Favaro, J. Lédion, G. Sattonnay, J. Brubach, P. Berthet, A. Huntz, P. Roy and R. Tétot, J. Solid State Chem., 182, 1171 (2009).

    Article  CAS  Google Scholar 

  30. Y. H. Kim and E. D. Park, Appl. Catal. B: Environ., 96, 41 (2010).

    Article  CAS  Google Scholar 

  31. G. Busca, Catal. Today, 226, 2 (2014).

    Article  CAS  Google Scholar 

  32. S. Rane, Ø. Borg, J. Yang, E. Rytter and A. Holmen, Appl. Catal. A: Gen., 388, 160 (2010).

    Article  CAS  Google Scholar 

  33. B. Rebours, J.-B. d’Espinose de la Caillerie and O. Clause, J. Am. Chem. Soc., 116, 1707 (1994).

    Article  CAS  Google Scholar 

  34. J. Zhang, H. Xu, X. Jin, Q. Ge and W. Li, Appl. Catal. A: Gen., 290, 87 (2005).

    Article  CAS  Google Scholar 

  35. B. Vos, E. Poels and A. Bliek, J. Catal., 198, 77 (2001).

    Article  CAS  Google Scholar 

  36. E. Hong, H.-I. Sim and C.-H. Shin, Chem. Eng. J., 292, 156 (2016).

    Article  CAS  Google Scholar 

  37. E. Hong, S. W. Baek, M. Shin, Y.-W. Suh and C.-H. Shin, J. Ind. Eng. Chem., 54, 137 (2017).

    Article  CAS  Google Scholar 

  38. S. Pyen, E. Hong, M. Shin, Y.-W. Suh and C.-H. Shin, Mol. Catal., 448, 71 (2018).

    Article  CAS  Google Scholar 

  39. C. O. Areán, M. P. Mentruit, A. L. López and J. Parra, Colloids Surf., A, 180, 253 (2001).

    Article  Google Scholar 

  40. J. Shen, R. E. Hayes, X. Wu and N. Semagina, ACS Catal., 5, 2916 (2015).

    Article  CAS  Google Scholar 

  41. K. Otto and L. Haack, Appl. Catal. B: Environ., 1, 1 (1992).

    Article  CAS  Google Scholar 

  42. J. G. McCarty, Catal. Today, 26, 283 (1995).

    Article  CAS  Google Scholar 

  43. L. Borkó, I. Nagy, Z. Schay and L. Guczi, Appl. Catal. A: Gen., 147, 95 (1996).

    Article  Google Scholar 

  44. C. A. Müller, M. Maciejewski, R. A. Koeppel and A. Baiker, Catal. Today, 47, 245 (1999).

    Article  Google Scholar 

  45. P. Castellazzi, G. Groppi, P. Forzatti, A. Baylet, P. Marécot and D. Duprez, Catal. Today, 155, 18 (2010).

    Article  CAS  Google Scholar 

  46. C.-k. Shi, L.-f. Yang, Z.-c. Wang, X.-e. He, J.-x. Cai, G. Li and X.-s. Wang, Appl. Catal. A: Gen., 243, 379 (2003).

    Article  CAS  Google Scholar 

Download references

Author information

Authors and Affiliations

  1. Department of Chemical Engineering, Chungbuk National University, Chungbuk, 28644, Korea

    Eunpyo Hong, Su-A Jeon & Chae-Ho Shin

  2. Department of Environmental Engineering, Chungbuk National University, Chungbuk, 28644, Korea

    Sang-Sup Lee

Authors
  1. Eunpyo Hong
    View author publications

    You can also search for this author in PubMed Google Scholar

  2. Su-A Jeon
    View author publications

    You can also search for this author in PubMed Google Scholar

  3. Sang-Sup Lee
    View author publications

    You can also search for this author in PubMed Google Scholar

  4. Chae-Ho Shin
    View author publications

    You can also search for this author in PubMed Google Scholar

Corresponding author

Correspondence to Chae-Ho Shin.

Electronic supplementary material

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Hong, E., Jeon, SA., Lee, SS. et al. Methane combustion over Pd/Ni-Al oxide catalysts: Effect of Ni/Al ratio in the Ni-Al oxide support. Korean J. Chem. Eng. 35, 1815–1822 (2018). https://doi.org/10.1007/s11814-018-0090-0

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11814-018-0090-0

Keywords

Search

Navigation