Skip to main content
Log in

Uniaxial Electro-Mechanically Coupled Cyclic Deformation of VHB 4905 Dielectric Elastomer: Experiment and Constitutive Model

  • Technical Article
  • Published:
Journal of Materials Engineering and Performance Aims and scope Submit manuscript

Abstract

In the uniaxial deformation mode, the electro-mechanically coupled cyclic deformation of VHB 4905 dielectric elastomer (DE) is systematically studied by the experimental observation and constitutive modeling. From a series of uniaxial electro-mechanically coupled cyclic tests, it is found that with applying a constant voltage, the cyclic softening and ratchetting of VHB 4905 DE are more apparent than that without applying any voltage, which indicate that the VHB 4905 DE exhibits an electro-mechanically coupled effect. Also, the uniaxial electro-mechanically coupled cyclic deformation of VHB 4905 DE presents a strong rate-dependence and remarkable stress-level-dependence. Based on the experimental results, an electro-mechanically coupled visco-hyperelastic constitutive model is proposed by considering the remarkable nonlinear viscosity of VHB 4905 DE and the effect of applied voltage on the cyclic deformation. Comparing the predicted results with correspondent experimental data, it is concluded that the proposed constitutive model reasonably reproduces the uniaxial electro-mechanically coupled cyclic deformation of VHB 4905 DE, including the cyclic softening and ratchetting.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8
Fig. 9
Fig. 10
Fig. 11
Fig. 12
Fig. 13
Fig. 14

Similar content being viewed by others

References

  1. B. Huang, M.Y. Li, T. Mei, D. McCoul, S.H. Qin, Z.F. Zhao, and J.W. Zhao, Wearable Stretch Sensors for Motion Measurement of the Wrist Joint Based on Dielectric Elastomers, Sensors, 2017, 17(12), p 2708.

    Article  PubMed  PubMed Central  Google Scholar 

  2. O.A. Araromi, S. Rosset, and H.R. Shea, High-Resolution, Large-Area Fabrication of Compliant Electrodes via Laser Ablation for Robust, Stretchable Dielectric Elastomer Actuators and Sensors, ACS Appl. Mater. Interfaces, 2015, 7(32), p 18046–18053.

    Article  CAS  PubMed  Google Scholar 

  3. C.T. Nguyen, H. Phung, T.D. Nguyen, C. Lee, U. Kim, D. Lee, H. Moon, J. Koo, J.D. Nam, and H.R. Choi, A Small Biomimetic Quadruped Robot Driven by Multistacked Dielectric Elastomer Actuators, Smart Mater. Struct., 2014, 23(6), p 065005.

    Article  CAS  Google Scholar 

  4. I.A. Anderson, T.A. Gisby, T.G. McKay, B.M. O’Brien, and E.P. Calius, Multi-Functional Dielectric Elastomer Artificial Muscles for Soft and Smart Machines, J. Appl. Phys., 2012, 112(4), p 041101.

    Article  Google Scholar 

  5. K. Di, K.W. Bao, H.J. Chen, X.J. Xie, J.B. Tan, Y.X. Shao, Y.X. Li, W.J. Xia, Z.S. Xu, and E. Shiju, Dielectric Elastomer Generator for Electromechanical Energy Conversion: A Mini Review, Sustainability, 2021, 13(17), p 9881.

    Article  CAS  Google Scholar 

  6. M. Wissler and E. Mazza, Mechanical Behavior of an Acrylic Elastomer Used in Dielectric Elastomer Actuators, Sens. Actuator A Phys., 2007, 134(2), p 494–504.

    Article  CAS  Google Scholar 

  7. M. Hossain, D.K. Vu, and P. Steinmann, Experimental Study and Numerical Modelling of VHB 4910 Polymer, Comput. Mater. Sci., 2012, 59, p 65–74.

    Article  CAS  Google Scholar 

  8. A. Helal, M. Doumit, and R. Shaheen, Biaxial Experimental and Analytical Characterization of a Dielectric Elastomer, Appl. Phys. A Mater. Sci. Process., 2018, 124(2), p 1–11.

    CAS  Google Scholar 

  9. D. Ahmad, S.K. Sahu, and K. Patra, Fracture Toughness, Hysteresis and Stretchability of Dielectric Elastomers Under Equibiaxial and Biaxial Loading, Polym. Test., 2019, 79, p 106038.

    Article  Google Scholar 

  10. D. Ahmad and K. Patra, Experimental and Theoretical Analysis of Laterally Pre-Stretched Pure Shear Deformation of Dielectric Elastomer, Polym. Test., 2019, 75, p 291–297.

    Article  CAS  Google Scholar 

  11. Z.S. Liao, M. Hossain, X.H. Yao, M. Mehnert, and P. Steinmann, On Thermo-Viscoelastic Experimental Characterization and Numerical Modelling of VHB Polymer, Int. J. Nonlinear Mech., 2020, 118, p 103263.

    Article  Google Scholar 

  12. J.S. Zhang, X.J. Liu, L. Liu, Z.C. Yang, P.F. Li, and H.L. Chen, Modeling and Experimental Study on Dielectric Elastomers Incorporating Humidity Effect, EPL, 2020, 129(5), p 57002.

    Article  CAS  Google Scholar 

  13. M. Hossain, D.K. Vu, and P. Steinmann, A Comprehensive Characterization of the Electro-Mechanically Coupled Properties of VHB 4910 Polymer, Arch. Appl. Mech., 2015, 85(4), p 523–537.

    Article  Google Scholar 

  14. M. Mehnert, M. Hossain, and P. Steinmann, Experimental and Numerical Investigations of the Electro-Viscoelastic Behavior of VHB 4905 (TM), Eur. J. Mech. A Solids, 2019, 77, p 103797.

    Article  Google Scholar 

  15. M. Mehnert, M. Hossain, and P. Steinmann, A Complete Thermo-Electro-Viscoelastic Characterization of Dielectric Elastomers, Part I: Experimental Investigations, J. Mech. Phys. Solids, 2021, 157, p 104603.

    Article  CAS  Google Scholar 

  16. R.K. Sahu and K. Patra, Rate-Dependent Mechanical Behavior of VHB 4910 Elastomer, Mech. Adv. Mater. Struct., 2016, 23(2), p 170–179.

    Article  Google Scholar 

  17. S. Thylander, A. Menzel, M. Ristinmaa, S. Hall, and J. Engqvist, Electro-Viscoelastic Response of an Acrylic Elastomer Analysed by Digital Image Correlation, Smart Mater. Struct., 2017, 26(8), p 085021.

    Article  Google Scholar 

  18. Y.F. Chen, G.Z. Kang, J.H. Yuan, and T.F. Li, Experimental Study on Pure-Shear-Like Cyclic Deformation of VHB 4910 Dielectric Elastomer, J. Polym. Res., 2019, 26(8), p 1–15.

    Article  Google Scholar 

  19. W. Huang and G. Kang, Experimental Study on Uniaxial Ratchetting of VHB 4910 Dielectric Elastomer, Polym. Test., 2022, 109, p 107557.

    Article  CAS  Google Scholar 

  20. Y.F. Chen, G.Z. Kang, J.H. Yuan, T.F. Li, and S.X. Qu, Experimental Investigation on Electro-Mechanically Coupled Cyclic Deformation of Laterally Constrained Dielectric Elastomer, Polym. Test., 2020, 81, p 106220.

    Article  CAS  Google Scholar 

  21. K. Patra and R.K. Sahu, A Visco-Hyperelastic Approach to Modelling Rate-Dependent Large Deformation of a Dielectric Acrylic Elastomer, Int. J. Mech. Mater. Des., 2015, 11(1), p 79–90.

    Article  CAS  Google Scholar 

  22. J.S. Zhang, J. Ru, H.L. Chen, D.C. Li, and J. Lu, Viscoelastic Creep and Relaxation of Dielectric Elastomers Characterized by a Kelvin-Voigt-Maxwell Model, Appl. Phys. Lett., 2017, 110(4), p 044104.

    Article  Google Scholar 

  23. Y.F. Chen, G.Z. Kang, J.H. Yuan, Y.H. Hu, T.F. Li, and S.X. Qu, An Electro-Mechanically Coupled Visco-Hyperelastic-Plastic Constitutive Model for Cyclic Deformation of Dielectric Elastomers, Mech. Mater., 2020, 150, p 103575.

    Article  Google Scholar 

  24. M. Wissler and E. Mazza, Electromechanical Coupling in Dielectric Elastomer Actuators, Sens. Actuator A Phys., 2007, 138(2), p 384–393.

    Article  CAS  Google Scholar 

  25. Z.G. Suo, Theory of Dielectric Elastomers, Acta Mech. Solida Sin., 2010, 23(6), p 549–578.

    Article  Google Scholar 

  26. M. Mehnert, M. Hossain, and P. Steinmann, Numerical Modeling of Thermo-Electro-Viscoelasticity with Field-Dependent Material Parameters, Int. J. Nonlinear Mech., 2018, 106, p 13–24.

    Article  Google Scholar 

  27. M. Mehnert, M. Hossain, and P. Steinmann, A Complete Thermo-Electro-Viscoelastic Characterization of Dielectric Elastomers Part II: Continuum Modeling Approach, J. Mech. Phys. Solids, 2021, 157, p 104625.

    Article  CAS  Google Scholar 

  28. S. Thylander, A. Menzel, and M. Ristinmaa, A Non-Affine Electro-Viscoelastic Microsphere Model for Dielectric Elastomers: Application to VHB 4910 Based Actuators, J. Intell. Mater. Syst. Struct., 2017, 28(5), p 627–639.

    Article  Google Scholar 

  29. X. Zhao and Z. Suo, Theory of Dielectric Elastomers Capable of Giant Deformation of Actuation, Phys. Rev. Lett., 2010, 104(17), p 178302.

    Article  PubMed  Google Scholar 

  30. B. Li, H. Chen, J. Qiang, S. Hu, Z. Zhu, and Y. Wang, Effect of Mechanical Pre-Stretch on the Stabilization of Dielectric Elastomer Actuation, J. Phys. D Appl. Phys., 2011, 44(15), p 155301.

    Article  Google Scholar 

  31. S. Reese and S. Govindjee, A Theory of Finite Viscoelasticity and Numerical Aspects, Int. J. Solids Struct., 1998, 35(26–27), p 3455–3482.

    Article  Google Scholar 

  32. R.W. Ogden, Large Deformation Isotropic Elasticity–on the Correlation of Theory and Experiment for Incompressible Rubberlike Solids, Rubber Chem. Technol., 1973, 46(2), p 398–416.

    Article  Google Scholar 

  33. L. Dorfmann and R.W. Ogden, Nonlinear Electroelasticity: Material Properties, Continuum Theory and Applications, Proc. R. Soc. A Math. Phys. Eng. Sci., 2017, 473, p 20170311.

    Google Scholar 

  34. N. Cohen, S.S. Oren, and G. Debotton, The Evolution of the Dielectric Constant in Various Polymers Subjected to Uniaxial Stretch, Extrem. Mech. Lett., 2017, 16, p 1–5.

    Article  Google Scholar 

  35. X.H. Zhao and Z.G. Suo, Electrostriction in Elastic Dielectrics Undergoing Large Deformation, J. Appl. Phys., 2008, 104(12), p 123530.

    Article  Google Scholar 

Download references

Acknowledgments

The work is supported by the National Natural Science Foundation of China under Grant No.11972312.

Author information

Authors and Affiliations

Authors

Contributions

WH: Conceptualization, Investigation, Methodology, Validation, Formal Analysis, Data Curation, Visualization, Software, Writing—Original Draft. GK: Conceptualization, Supervision, Funding Acquisition, Writing—Review & Editing. PM: Investigation, Validation, Formal Analysis, Data Curation.

Corresponding author

Correspondence to Guozheng Kang.

Ethics declarations

Conflict of interest

There are no conflicts of interest declared by any of the authors.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Appendix 1

Appendix 1

Size design of uniaxial specimen.

In the uniaxial electro-mechanically coupled deformation tests, the size of specimen is set as 100 mm × 50 mm, that is, the aspect ratio is 2:1. Through two tests, it is verified that the uniaxial deformation condition can be satisfied experimentally by using the specimen with a size of 100 mm × 50 mm. The details are provided as follows:

Firstly, the surface of the designed specimen is colored, and then a strain of 3.0 is applied to the specimen. Figure 

Fig. 15
figure 15

Verification tests for the uniaxial deformation mode: (a) before deformation; (b) after deformation; (c) pixel coordinates and linear fitting

15(a) and (b) give the shapes of the specimen before and after deformation, respectively. The black line in Fig. 15(c) shows the pixel coordinates of the upper and lower edges in the deformed specimen; while the red line is a straight line that linearly fits the homogeneous portion in the middle and extends to the left of the specimen. Note that, only a half of deformed specimen is considered here, because the specimen is symmetrical in the whole deformation stage. As shown in Fig. 15c, the deformation is nonhomogeneous when the longitudinal pixels are located within the region from about 200 to 600, that is, for the specimen with a size of 100 mm × 50 mm and a strain of 3.0, the proportion of the homogeneous deformation part to the whole specimen is about 67%. Moreover, according to the longitudinal pixels, it is found that the longitudinal elongation \(\, \lambda_{1}^{{}} = 4\), and the lateral elongation \(\, \lambda_{2}^{{}} \approx 0.495\). From the assumption that VHB 4905 DE is an incompressible material, it yields \(\, \lambda_{3}^{{}} \approx 0.505\). Thus, the deformation in the middle part of the specimen can be approximately considered as a uniaxial deformation mode.

Secondly, the relationship between the global strain and local strain is investigated. The specimen is first marked in the middle and then loaded at a strain rate of 0.05 s−1 to a strain of 3.0, as shown in Fig. 

Fig. 16
figure 16

Calibration tests: (a) at the strain of 0; (b) at the strain of 1.0; (c) at the strain of 2.0; (d) at the strain of 3.0

16. In this process, the global and local coordinates are recorded every 3 s, and then are converted into the strains to make the relationship between the global strain and local strain. Finally, a linear relationship is used to fit the obtained data. The results are given in Fig. 

Fig. 17
figure 17

Calibration of experimental results

17. It is found that the linear relationship between the global strain and local strain is very strong, so the global strain measured by the tests can approximately replace the local strain in the middle part of the specimen.

According to the above analysis, for the specimen with a size of 100 mm × 50 mm, the homogeneous deformation part of the specimen is in a uniaxial deformation mode, and the local strain is basically linear with the global strain. Therefore, the specimen size used in the uniaxial electro-mechanically coupled deformation tests of VHB 4905 DE can be selected as 100 mm × 50 mm.

Rights and permissions

Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Huang, W., Kang, G. & Ma, P. Uniaxial Electro-Mechanically Coupled Cyclic Deformation of VHB 4905 Dielectric Elastomer: Experiment and Constitutive Model. J. of Materi Eng and Perform 33, 2952–2967 (2024). https://doi.org/10.1007/s11665-023-08179-8

Download citation

  • Received:

  • Revised:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11665-023-08179-8

Keywords

Navigation