Skip to main content
Log in

High Mobility and Stability of Thin-Film Transistors Using Silicon-Doped Amorphous Indium Tin Oxide Semiconductors

  • Published:
Journal of Electronic Materials Aims and scope Submit manuscript

Abstract

We report the fabrication of high-performance thin-film transistors (TFTs) with an amorphous silicon indium tin oxide (a-SITO) channel, which was deposited by cosputtering a silicon dioxide and an indium tin oxide target. The effect of the silicon doping on the device performance and stability of the a-SITO TFTs was investigated. The field-effect mobility and stability under positive bias stress of the a-SITO TFTs with optimized Si content (0.22 at.% Si) dramatically improved to 28.7 cm2/Vs and 1.5 V shift of threshold voltage, respectively, compared with the values (0.72 cm2/Vs and 8.9 V shift) for a-SITO TFTs with 4.22 at.% Si. The role of silicon in a-SITO TFTs is discussed based on various physical and chemical analyses, including x-ray absorption spectroscopy, x-ray photoelectron spectroscopy, and spectroscopic ellipsometry measurements.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. K. Nomura, H. Ohta, A. Takagi, T. Kamiya, M. Hirano, and H. Hosono, Nature 432, 488 (2004).

    Article  Google Scholar 

  2. J.S. Park, W.-J. Maeng, H.-S. Kim, and J.-S. Park, Thin Solid Films 520, 1679 (2012).

    Article  Google Scholar 

  3. A. Walsh, J.F. da Silva, and S.H. Wei, J. Phys.: Condens. Matter 23, 334210 (2011).

    Google Scholar 

  4. J.H. Noh, S.Y. Ryu, S.J. Jo, C.S. Kim, S.-W. Sohn, P.D. Rack, D.-J. Kim, and H.K. Baik, IEEE Electron Device Lett. 31, 567 (2010).

    Article  Google Scholar 

  5. W. Kim, J.-H. Bang, H.-S. Uhm, S.-H. Lee, and J.-S. Park, Thin Solid Films 519, 1573 (2010).

    Article  Google Scholar 

  6. C.J. Chiu, S.P. Chang, and S.J. Chang, IEEE Electron Device Lett. 31, 1245 (2010).

    Google Scholar 

  7. M. Dai, G. Wu, Y. Yang, J. Jiang, L. Li, and Q. Wan, Appl. Phys. Lett. 98, 093506 (2010).

    Article  Google Scholar 

  8. C.E. Kim and I. Yun, Appl. Phys. Lett. 100, 013501 (2012).

    Article  Google Scholar 

  9. S.Y. Park, K.H. Ji, H.Y. Jung, J.-I. Kim, R. Choi, K.S. Son, M.K. Ryu, S. Lee, and J.K. Jeong, Appl. Phys. Lett. 100, 162108 (2012).

    Article  Google Scholar 

  10. D.-H. Cho, S. Yang, C. Byun, J. Shin, M.K. Ryu, S.-H.K. Park, C.-S. Hwang, S.M. Chung, W.-S. Cheong, S.M. Yoon, and H.-Y. Chu, Appl. Phys. Lett. 93, 142111 (2008).

    Article  Google Scholar 

  11. T. Iwasaki, N. Itagaki, T. Den, H. Kumomi, K. Nomura, T. Kamiya, and H. Hosono, Appl. Phys. Lett. 90, 242114 (2007).

    Article  Google Scholar 

  12. C.-J. Kim, et al., Appl. Phys. Lett. 95, 252103 (2009).

    Article  Google Scholar 

  13. J.-S. Park, K.-S. Kim, Y.-G. Park, Y.-G. Mo, H.D. Kim, and J.K. Jeong, Adv. Mater. 21, 329 (2009).

    Article  Google Scholar 

  14. D.H. Kim, D.Y. Yoo, H.K. Jung, D.H. Kim, and S.Y. Lee, Appl. Phys. Lett. 99, 172106 (2011).

    Article  Google Scholar 

  15. S. Tomai, M. Nishimura, M. Itose, M. Matuura, M. Kasami, S. Matsuzaki, H. Kawashima, F. Utsuno, and K. Yano, Jpn. J. Appl. Phys. 51, 03CB01 (2012).

  16. S. Urakawa, S. Tomai, Y. Ueoka, H. Yamazaki, M. Kasami, K. Yano, D. Wang, M. Furuta, M. Horita, Y. Ishikawa, and Y. Uraoka, Appl. Phys. Lett. 102, 053506 (2013).

    Article  Google Scholar 

  17. K.-H. Lim, K. Kim, S. Kim, S.Y. Park, H. Kim, and Y.S. Kim, Adv. Mater. 25, 2994 (2013).

    Article  Google Scholar 

  18. J.H. Jeong, H.W. Yang, J.-S. Park, J.K. Jeong, Y.G. Mo, H.D. Kim, J.W. Song, and C.S. Hwang, Electrochem. Solid-State Lett. 11, 157 (2008).

    Article  Google Scholar 

  19. S.Y. Lee, D.H. Kim, E. Chong, Y.W. Jeon, and D.H. Kim, Appl. Phys. Lett. 98, 122105 (2011).

    Article  Google Scholar 

  20. R.B.M. Cross and M.M. De Souza, Appl. Phys. Lett. 89, 263513 (2006).

    Article  Google Scholar 

  21. K.B. Chung, J.P. Long, H. Seo, G. Lucovsky, and D. Nordlund, J. Appl. Phys. 106, 074102 (2009).

    Article  Google Scholar 

  22. C. McGuinness, C.B. Stagarescu, P.J. Ryan, J.E. Downes, D. Fu, and K.E. Smith, Phys. Rev. B 68, 165104 (2003).

    Article  Google Scholar 

  23. H.-M. Lee, S.-B. Kang, K.-B. Chung, and H.-K. Kim, Appl. Phys. Lett. 102, 021914 (2013).

    Article  Google Scholar 

  24. G. Lucovsky, D. Zeller, K. Wu, and J.L. Whitten, Microelectron. Eng. 88, 1537 (2011).

    Article  Google Scholar 

  25. B.D. Ahn, J.H. Lim, M.-H. Cho, J.-S. Park, and K.-B. Chung, J. Phys. D Appl. Phys. 45, 415307 (2012).

    Article  Google Scholar 

  26. D.E. Aspnes and A.A. Studna, Phys. Rev. B 27, 985 (1983).

    Article  Google Scholar 

  27. H.-W. Park, J.-S. Park, J.H. Lee, and K.-B. Chung, Electrochem. Solid-State Lett. 15, H133 (2012).

    Article  Google Scholar 

  28. H.-W. Park, B.-K. Kim, J.-S. Park, and K.-B. Chung, Appl. Phys. Lett. 102, 102102 (2013).

    Article  Google Scholar 

Download references

Acknowledgements

This research was partially supported by the Basic Science Research Program through the National Research Foundation of Korea (NRF), funded by the Ministry of Education, Science, and Technology (No. 2012011730 and NRF-2013R1A1A 2A10005186). This work was supported by the IT R&D program of MKE/KETI (Grant No. 10041416, The core technology development of light and space adaptable new mode display for energy saving on 7 in. and 2 W) and also by the Global Frontier R&D Program (2013-073298) of the Center for Hybrid Interface Materials (HIM) funded by the Ministry of Science, ICT, and Future Planning.

Author information

Authors and Affiliations

Authors

Corresponding authors

Correspondence to Kwun-Bum Chung or Jin-Seong Park.

Additional information

T.W. Seo and Hyun-Suk Kim have contributed equally to this work.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Seo, T.W., Kim, HS., Lee, KH. et al. High Mobility and Stability of Thin-Film Transistors Using Silicon-Doped Amorphous Indium Tin Oxide Semiconductors. J. Electron. Mater. 43, 3177–3183 (2014). https://doi.org/10.1007/s11664-014-3211-5

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11664-014-3211-5

Keywords

Navigation