Skip to main content
Log in

Fog Water, Throughfall, and Bulk Precipitation Chemistry and a Newly Developed Methodology for the Estimation of Fog Water Deposition

  • Published:
Water, Air, & Soil Pollution Aims and scope Submit manuscript

Abstract

Fog water, throughfall, and bulk precipitation were collected at the site neighboring to coastal and urbanized area in Japan. Fog water was collected by using string type passive fog collector. Fog water was strongly influenced by the sea salt components presumably due to drizzle. Furthermore, fog water would be acidified by acid-related nitrate species like HNO3 gas in ambient air; however, fog water was neutralized well as shown below. Throughfall selectively included non-sea salt chloride (nss-Cl) among the three media: fog water, throughfall, and bulk precipitation, likely due to a dry deposition of nss-Cl species on canopy. The pH values for fog water, throughfall, and bulk precipitation, were 5.28, 5.97, and 5.73, respectively. Those were typically higher compared with other previous observations, meaning that all media were neutralized well. In particular, fog water was dominantly neutralized by nss-Mg2+ and nss-Ca2+. The supply of nitrogen (NO3-N + NH4+-N) via throughfall showed the seasonality, higher in winter and summer. We considered a new and simple methodology to evaluate/estimate the deposition amount of fog water. We applied our new methodology to our present observation and obtained a good agreement with the result heretofore used.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7

Similar content being viewed by others

Data Availability

Not applicable.

Code Availability

Not applicable.

References 

  • Aikawa, M., Hiraki, T., Shoga, M., & Tamaki, M. (2001). Fog and precipitation chemistry at Mt. Rokko in Kobe, April 1997-March 1998. Water, Air and Soil Pollution, 130, 1517–1522.

    Article  Google Scholar 

  • Aikawa, M., Hiraki, T., Shoga, M., & Tamaki, M. (2004). Spatial variations and trends in acid deposition in Japan within a 100 km x 100 km region from 1986 to 1999. Water, Air and Soil Pollution, 157, 225–244.

    Article  CAS  Google Scholar 

  • Aikawa, M., Hiraki, T., Shoga, M., & Tamaki, M. (2005). Chemistry of fog water collected in the Mt. Rokko area (Kobe City, Japan) between April 1997 and March 2001. Water, Air and Soil Pollution, 160, 373–393.

    Article  CAS  Google Scholar 

  • Aikawa, M., Hiraki, T., & Tamaki, M. (2005). Characteristics in concentration of chemical species in ambient air based on three-year monitoring by filter pack method. Water, Air and Soil Pollution, 161, 335–352.

    Article  CAS  Google Scholar 

  • Aikawa, M., Hiraki, T., & Tamaki, M. (2006). Comparative field study on precipitation, throughfall, stemflow, fog water, and atmospheric aerosol and gases at urban and rural sites in Japan. Science of the Total Environment, 366, 275–285. https://doi.org/10.1016/j.scitotenv.2005.06.027

    Article  CAS  Google Scholar 

  • Aikawa, M., Hiraki, T., Shoga, M., Tamaki, M., & Sumitomo, S. (2007). Seven-year trend of the time and seasonal dependence of fog water collected near an industrialized area in Japan. Atmospheric Research, 83, 1–9. https://doi.org/10.1016/j.atmosres.2006.01.011

    Article  CAS  Google Scholar 

  • Aikawa, M., Hiraki, T., Suzuki, M., Tamaki, M., & Kasahara, M. (2007). Separate chemical characterizations of fog water, aerosol, and gas before, during, and after fog events near an industrialized area in Japan. Atmospheric Environment, 41, 1950–1959. https://doi.org/10.1016/j.atmosenv2006.10.049

    Article  CAS  Google Scholar 

  • Aikawa, M., Ohara, T., Hiraki, T., Oishi, O., Tsuji, A., Yamagami, M., Murano, K., & Mukai, H. (2010). Significant geographic gradients in particulate sulfate over Japan determined from multiple site measurements and a chemical transport model: Impacts of transboundary pollution from the Asian continent. Atmospheric Environment, 44, 381–391. https://doi.org/10.1016/j.atmosenv.2009.10.025

    Article  CAS  Google Scholar 

  • Balestrini, R., & Tagliaferri, A. (2001). Atmospheric deposition and canopy exchange processes in alpine forest ecosystems (northern Italy). Atmospheric Environment, 35, 6421–6433. https://doi.org/10.1016/j.atmosenv2006.10.049

    Article  CAS  Google Scholar 

  • EANET, 2010, Technical manual for wet deposition monitoring in East Asia -2010, https://www.eanet.asia/wp-content/uploads/2019/04/techwet.pdf (last access: July 6th, 2021)

  • Geospatial information authority of Japan, 2021, https://www.gsi.go.jp/index.html (last access 2021/11/23)

  • Hattori, S., Chikaarashi, H., & Takeuchi, N. (1982). Measurement of the rainfall interception and its micrometeorological analysis in a Hinoki stand. Bulletin of the Forestry and Forest Products Research Institute, 318, 79–102.

    Google Scholar 

  • Igawa, M., Tsutsumi, Y., Mori, T., & Okochi, H. (1998). Fogwater chemistry at a mountainside forest and the estimation of the air pollutant Deposition via fog droplets based on the atmospheric quality at the mountain base. Environmental Science and Technology, 32, 1566–1572.

    Article  CAS  Google Scholar 

  • Igawa, M., Kojima, K., Yoshimoto, O., & Nanzai, B. (2015). Air pollutant deposition at declining forest sites of the Tanzawa Mountains, Japan. Atmospheric Research, 151, 93–100. https://doi.org/10.1016/j.atmosres.2014.03.017

    Article  CAS  Google Scholar 

  • Igawa, M., Kamijo, K., Nanzai, B., & Matsumoto, K. (2017). Chemical composition of polluted mist droplets. Atmospheric Environment, 171, 230–236. https://doi.org/10.1016/j.atmosenv.2017.10.029

    Article  CAS  Google Scholar 

  • Kobayashi, T., Nakagawa, Y., Tamaki, M., Hiraki, T., & Aikawa, M. (2001). Cloud water deposition to forest canopies of Cryptomeria japonica at Mt. Rokko, Kobe, Japan. Water, Air and Soil Pollution, 130, 601–606.

    Article  Google Scholar 

  • Kobayashi, T., Nakagawa, Y., Tamaki, M., Hiraki, T., & Aikawa, M. (2002). Temporal variation of cloud water deposition to Cryptomeria canopies - Fog drip observed in the coniferous forest stands at Mt. Rokko in Kobe -. Environmental Science, 15(3), 151–161. (in Japanese with English abstract).

    Google Scholar 

  • Lange, C. A., Matschullat, J., Zimmermann, F., Sterzik, G., & Wienhaus, O. (2003). Fog frequency and chemical composition of fog water—a relevant contribution to atmospheric deposition in the eastern Erzgebirge, Germany. Atmospheric Environment, 37, 3731–3739. https://doi.org/10.1016/S1352-2310(03)00350-9

  • Lovett, G. M., & Lindberg, S. E. (1984). Dry deposition and canopy exchange in a mixed oak forest as determined by analysis of throughfall. Journal of Applied Ecology, 21, 1013–1027.

    Article  Google Scholar 

  • Lovett, G. M., Reiners, W. A., & Olson, R. K. (1982). Cloud droplet deposition in subalpine balsam fir forests: Hydrological and chemical inputs. Science, 218, 1303–1304.

    Article  CAS  Google Scholar 

  • Ministry of the Environment, Japan (2019). Report on acid deposition and air pollution in Japan (Fiscal year 2013–2017). http://www.env.go.jp/air/acidrain/monitoring/rep4/1_2syou.pdf (last access: July 4th, 2021) (in Japanese)

  • Peng, Y., Suzuki, M., Nguyen, K. L., Zhang, X., & Aikawa, M. (2021). Presence and source attribution of airborne anthropogenic/non-sea-salt inorganic chloride determined by filter-pack method at eastern edge in East Asia. Water, Air and Soil Pollution., 232, 238.

    Article  CAS  Google Scholar 

  • Sanada, M., Ohta, S., Ootomo, R., & Sanada, E. (1991). Stemflow and throughfall in the plantation of Abies sachalinensis and Picea jezoensis in the suburbs of Sapporo. Japanese Journal of Forest Environment, 33(1), 8–15. (in Japanese with English summary).

    Google Scholar 

  • Seinfeld, J. H., & Pandis, S. N. (2016). Atmospheric chemistry and physics from air pollution to climate change (p. 30). Wiley.

    Google Scholar 

  • Selma Isil, M. S., Collett, J., Jr., Lynch, J., Weiss-Penzias, P., & Rogers, C. M. (2022). Cloud and fog deposition: Monitoring in high elevation and coastal ecosystems The past, present, and future. Atmospheric Environment, 274, 118997. https://doi.org/10.1016/j.atmosenv.2022.118997

    Article  CAS  Google Scholar 

  • Tamaki, M., Hiraki, T., & Aikawa, M. (2000). Progress in acid deposition monitoring technology in Japan. Global Environmental Research, 4(1), 25–38.

    CAS  Google Scholar 

  • Wang, Y., Okochi, H., & Igawa, M. (2021). Characteristics of fog and fog collection with passive collector at Mt. Oyama in Japan. Water, Air and Soil Pollution., 232, 260. https://doi.org/10.1007/s11270-021-05205-0

    Article  CAS  Google Scholar 

  • Zhang, S., Fan, S., Wang, Y., Ge, P., Hu, C., Zhu, D., & Zhang, H. (2021). Chemical characteristics of size-resolved fog water at an urban site in Nanjing and the summit of Mt. Lu. East China. Atmospheric Environment, 263, 118667. https://doi.org/10.1016/j.atmosenv.2021.118667

    Article  CAS  Google Scholar 

  • Zhang, X., Murakami, T., Wang, J., & Aikawa, M. (2021). Sources, species and secondary formation of atmospheric aerosols and gaseous precursors in the suburb of Kitakyushu Japan. Science of the Total Environment, 763(2021), 143001. https://doi.org/10.1016/j.scitotenv.2020.143001

    Article  CAS  Google Scholar 

  • Zhang, X., Eto, Y., Wang, J., & Aikawa, M. (2021). Risk assessment and management of PM2.5-bound heavy metals in the urban area of Kitakyushu Japan. Science of the Total Environment, 795, 148748. https://doi.org/10.1016/j.scitotenv.2021.148748

    Article  CAS  Google Scholar 

Download references

Acknowledgements

This work was supported by JSPS KAKENHI Grant Numbers JP19H00955. The collection of samples was carried out under the supports by City of Kitakyushu and Sarakurayama visitor center. We sincerely appreciate the cooperation for the sample collection.

Funding

This work was supported by JSPS KAKENHI Grant Numbers JP19H00955.

Author information

Authors and Affiliations

Authors

Contributions

Momoko Abe: setup of survey site, sample collection, chemical analysis, statistical analysis, visualization, writing of draft manuscript.

Sho Oniwa: setup of the survey site, sample collection.

Hiroshi Okochi: design of the study, funding, reviewing of the final manuscript.

Masahide Aikawa: design, conceptualization, organization, creation and supervision of the study, writing of the final manuscript.

Corresponding author

Correspondence to Masahide Aikawa.

Ethics declarations

Ethics Approval

Not applicable.

Consent to Participate

Not applicable.

Consent to Publication

Not applicable.

Competing Interests

The authors declare no competing interests.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Abe, M., Oniwa, S., Okochi, H. et al. Fog Water, Throughfall, and Bulk Precipitation Chemistry and a Newly Developed Methodology for the Estimation of Fog Water Deposition. Water Air Soil Pollut 233, 474 (2022). https://doi.org/10.1007/s11270-022-05939-5

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1007/s11270-022-05939-5

Keywords

Navigation