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Heterogeneous Catalysis on Liquid Organic Hydrogen Carriers

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Abstract

Hydrogen is recognized as an ideal substitute for conventional energy sources due to its exceptional merits. However, the lack of inexpensive and efficient hydrogen storage approaches is the main obstacle for the “Hydrogen Economy”. Liquid organic hydrogen carriers (LOHCs) are attractive due to the decoupling of energy generation and usage in both space and time. Herein, we surveyed the recent advances of heterogeneous catalysts for different LOHCs, including methanol, ethanol, formic acid, formate salts, toluene, dibenzyl-toluene, and heterocycles. This review categorizes the catalysts by other metal species and discusses their catalytic mechanisms on hydrogenation and dehydrogenation. The challenges associated with the development of nanoscale heterogeneous catalysts and the possible solutions are also discussed. Finally, the future research directions for developing next-generation heterogeneous catalysts are outlined.

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Copyright© 2021, The American Association for the Advancement of Science

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Copyright© 2021, Elsevier

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Copyright© 2021, Elsevier

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Adapted from Ref. [67] with the permission of American Chemical Society. Copyright© 2011, American Chemical Society

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Copyright© 2021, Elsevier

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Copyright© 2017, American Chemical Society

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Copyright© 2021, Elsevier

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Copyright© 2021, Elsevier

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Adapted from Ref. [101] with the permission of Elsevier. Copyright© 2021, Elsevier

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Copyright© 2021, Elsevier

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Copyright© 2021, Elsevier

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Copyright© 2015, American Chemical Society

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Copyright© 2012, Royal Society of Chemistry

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Copyright© 2013, American Chemical Society

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Copyright© 2018, Jo Nakayama et al.

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Copyright© 2010, Royal Society of Chemistry

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Copyright© 2019, American Chemical Society

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Copyright© 2018, American Chemical Society

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Copyright© 2020, American Chemical Society

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Copyright© 2015, Royal Society of Chemistry

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Copyright© 2019, American Chemical Society

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Acknowledgements

The authors thank for the support from the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office (Award No. DE-EE0008826). The authors also thank Katarzyna Grubel, Kriston Brooks, Tom Autrey (Pacific Northwest National Laboratory collaborators), and Shaoqu Xie (Washington State University) for the fruitful discussion.

Funding

Funding was provided by Office of Energy Efficiency and Renewable Energy (Grant No. DE-EE0008826)

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  1. The Gene and Linda Voiland School of Chemical Engineering and Bioengineering, Washington State University, Pullman, USA

    Zhun Dong, Ahmad Mukhtar & Hongfei Lin

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  1. Zhun Dong
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  2. Ahmad Mukhtar
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  3. Hongfei Lin
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Correspondence to Hongfei Lin.

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Dong, Z., Mukhtar, A. & Lin, H. Heterogeneous Catalysis on Liquid Organic Hydrogen Carriers. Top Catal 64, 481–508 (2021). https://doi.org/10.1007/s11244-021-01458-5

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