Abstract
The typical characteristic of a thin porous layer is that its thickness is much smaller than its in-plane dimensions. This often leads to physical behaviors that are different from three-dimensional porous media. The classical Richards equation is insufficient to simulate many flow conditions in thin porous media. Here, we have provided an alternative approach by accounting for the dynamic capillarity effect. In this study, we have presented a set of one-dimensional in-plane imbibition and subsequent drainage experiments in a thin fibrous layer. The X-ray transmission method was used to measure saturation distributions along the fibrous sample. We simulated the experimental results using Richards equation either with classical capillary equation or with a so-called dynamic capillarity term. We have found that the standard Richards equation was not able to simulate the experimental results, and the dynamic capillarity effect should be taken into account in order to model the spontaneous imbibition. The experimental data presented here may also be used by other researchers to validate their models.
Article Highlights
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We have presented a set of one-dimensional in-plane imbibition and subsequent drainage experiments in a thin fibrous layer.
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The experimental data were simulated using the Richards equation either with classical capillary equation or with a so-call dynamic capillarity term.
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The dynamic capillarity effect should be taken into account in order to model the spontaneous imbibition.
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Data Availability
The data are available by contacting the corresponding author.
References
Abidoye, L.K., Das, D.B.: Scale dependent dynamic capillary pressure effect for two-phase flow in porous media. Adv. Water Resour. 74, 212–230 (2014)
Ashari, A., Vahedi Tafreshi, H.: A two-scale modeling of motion-induced fluid release from thin fibrous porous media. Chem. Eng. Sci. 64, 2067–2075 (2009)
Ashari, A., Bucher, T.M., Vahedi Tafreshi, H.: A semi-analytical model for simulating fluid transport in multi-layered fibrous sheets made up of solid and porous fibers. Comput. Mater. Sci. 50, 378–390 (2010)
Ashari, A., Bucher, T.M., Tafreshi, H.V.: Modeling motion-induced fluid release from partially saturated fibrous media onto surfaces with different hydrophilicity. Int. J. Heat Fluid Flow. 32, 1076–1081 (2011)
Aslannejad, H., Hassanizadeh, S.M., Raoof, A., de Winter, D.A.M., Tomozeiu, N., van Genuchten, M.T.: Characterizing the hydraulic properties of paper coating layer using FIB-SEM tomography and 3D pore-scale modeling. Chem. Eng. Sci. 160, 275–280 (2017)
Barenblatt, G.I.: Filtration of two nonmixing fluids in a homogeneous porous medium. Fluid Dyn 6, 857–864 (1971)
Bottero, S., Hassanizadeh, S.M., Kleingeld, P.J., Heimovaara, T.J.: Nonequilibrium capillarity effects in two-phase flow through porous media at different scales. Water Resour. Res. 47, W10505 (2011)
COMSOL: COMSOL multiphysics 5.0. COMSOL Inc., Burlington, MA (2014)
Dane, J.H., Hopmans, J.W.: Water retention and storage: laboratory. In: Dane, J.H., Topp, G. (eds.), Methods of Soil Analysis: Part 4 Physical Methods, Soil Sci. Soc. of Am., Madison, pp. 675–720 (2002)
Diamantopoulos, E., Durner, W.: Dynamic nonequilibrium of water flow in porous media: a review. Vadose Zone J 11, vzj2011-0197 (2012)
DiCarlo, D.A.: Modeling observed saturation overshoot with continuum additions to standard unsaturated theory. Adv. Water Resour. 28, 1021–1027 (2005)
Giuespie, T., Chemical, T.D.: The capillary rise of a liquid in a vertical strip of filter paper. J. Colloid Sci. 1, 123–130 (1959)
Goel, G., Abidoye, L.K., Chahar, B.R., Das, D.B.: Scale dependency of dynamic relative permeability-satuartion curves in relation with fluid viscosity and dynamic capillary pressure effect. Environ. Fluid Mech. 16, 945–963 (2016)
Hassanizadeh, S.M., Gray, W.G.: Mechanics and thermodynamics of multiphase flow in porous media including interphase boundaries. Adv. Water Resour. 13, 169–186 (1990)
Hassanizadeh, S.M., Gray, W.G.: Thermodynamic basis of capillary-pressure in porous-media. Water Resour. Res. 29, 3389–3405 (1993)
Hassanizadeh, S.M., Celia, M.A., Dahle, H.K.: Dynamic effect in the capillary pressure–saturation relationship and its impacts on unsaturated flow. Vadose Zone J. 1, 38–57 (2002)
Joekar-Niasar, V., Majid Hassanizadeh, S.: Effect of fluids properties on non-equilibrium capillarity effects: dynamic pore-network modeling. Int. J. Multiph. Flow. 37, 198–214 (2011)
Juanes, R.: Nonequilibrium effects in models of three-phase flow in porous media. Adv. Water Resour. 31, 661–673 (2009)
Landeryou, M., Eames, I., Cottenden, A.: Infiltration into inclined fibrous sheets. J. Fluid Mech. 529, 173–193 (2005)
Manthey, S., Hassanizadeh, S.M., Helmig, R., Hilfer, R.: Dimensional analysis of two-phase flow including a rate-dependent capillary pressure–saturation relationship. Adv. Water Resour. 31, 1137–1150 (2008)
Marmur, A., Cohen, R.D.: Characterization of porous media by the kinetics of liquid penetration: the vertical capillaries model. J. Colloid Interface Sci. 189, 299–304 (1997)
Melciu, I.C., Pascovici, M.D.: Imbibition of liquids in fibrous porous media. In: IOP Conference Series: Materials Science and Engineering, vol. 147, p. 012041 (2016)
Mualem, Y.: A new model for predicting the hydraulic conductivity of unsaturated porous media. Water Resour. Res. 12, 513–522 (1976)
O’Carroll, D.M., Phelan, T.J., Abriola, L.M.: Exploring dynamic effects in capillary pressure in multistep outflow experiments. Water Resour. Res. 41, 1–14 (2005)
Prat, M., Agaësse, T.: Thin porous media. In: Kambiz, V. (ed.), Handbook of Porous Media, Taylor&Francis, London, p. 959 (2015)
Qin, C.Z., Hassanizadeh, S.M.: Multiphase flow through multilayers of thin porous media: general balance equations and constitutive relationships for a solid–gas–liquid three-phase system. Int. J. Heat Mass Transf. 70, 693–708 (2014)
Qin, C.Z., Hassanizadeh, S.M.: A new approach to modelling water flooding in a polymer electrolyte fuel cell. Int. J. Hydrogen Energy. 40, 3348–3358 (2015)
Reza, M., Pillai, K.M.: Darcy’s law-based model for wicking in paper-like swelling porous media. AIChE J. 56, 2257–2267 (2010)
Richards, L.A.: Capillary conduction of liquids through porous mediums. Physics 1, 318–333 (1931)
Smiles, D.E., Vachaud, G., Vauclin, M.: A test of the uniqueness of the soil moisture characteristic during transient, nonhysteretic flow of water in a rigid soil1. Soil Sci. Soc. Am. J. 35, 534–539 (1971)
Tavangarrad, A.H., Mohebbi, B., Hassanizadeh, S.M., Rosati, R., Claussen, J., Blümich, B.: Continuum-scale modeling of liquid redistribution in a stack of thin hydrophilic fibrous layers. Transp. Porous Media. 122, 203–219 (2018)
Tavangarrad, A.H., Hassanizadeh, S.M., Rosati, R., Digirolamo, L., van Genuchten, M.T.: Capillary pressure–saturation curves of thin hydrophilic fibrous layers: effects of overburden pressure, number of layers, and multiple imbibition–drainage cycles. Text. Res. J. 89, 4906–4915 (2019a)
Tavangarrad, A.H., Mohebbi, B., Qin, C., Hassanizadeh, S.M., Rosati, R., Claussen, J., Blümich, B.: Continuum-scale modeling of water infiltration into a stack of two thin fibrous layers and their inter-layer space. Chem. Eng. Sci. 207, 769–779 (2019b)
Testoni, G.A., Kim, S., Pisupati, A., Park, C.H.: Modeling of the capillary wicking of flax fibers by considering the effects of fiber swelling and liquid absorption. J. Colloid Interface Sci. 525, 166–176 (2018)
Topp, G., Peters, A.: Comparison of water content-pressure head data obtained by equilibrium, steady-state, and unsteady-state methods1. Soil Sci. Soc. Am. J. 31, 312–314 (1967)
van Genuchten, M.T.: A closed-form equation for predicting the hydraulic conductivity of unsaturated soils. Soil Sci. Soc. Am. J. 44, 892–898 (1980)
van Duijn, C.J., Mitra, K., Pop, I.S.: Travelling wave solutions for the Richards equation incorporating non-equilibrium effects in the capillarity pressure. Nonlinear Anal. Real World Appl. 41, 232–268 (2018)
Washburn, E.W.: The dynamics of capillary flow. Phys. Rev. XVII, 273–283 (1921)
Zhuang, L., Hassanizadeh, S.M., van Genuchten, MTh., Leijnse, A., Raoof, A., Qin, C.: Modelling of horizontal water redistribution in an unsaturated soil. Vadose Zone J. 15, 3 (2016)
Zhuang, L., Hassanizadeh, S.M., Kleingeld, P., van Genuchten, M.: Revisiting the horizontal redistribution of water in soils; experiments and numerical modeling. Water Resour. Res. 53, 7576–7589 (2017a)
Zhuang, L., Hassanizadeh, S.M., Qin, C.-Z., de Waal, A.: Experimental investigation of hysteretic dynamic capillarity effect in unsaturated flow. Water Resour. Res. 53, 9078–9088 (2017b)
Zhuang, L., van Duijn, C.J., Hassanizadeh, S.M.: The effect of dynamic capillarity in modeling saturation overshoot during infiltration. Vadose Zone J. 18, 180133 (2019)
Acknowledgements
We gratefully acknowledge Ioannis Zarikos and Hamed Aslannejad of Utrecht University for technical support in using the confocal microscope. This work was supported by Kimberly-Clark Corporation and carried out in collaboration with the Darcy Center. The first author received funding from the National Natural Science Foundation of China (Grant No. 42007165). The second author received funding from the European Research Council under the European Union’s Seventh Framework Program (FP/2007-2013)/ERC Grant Agreement No. 341225.
Funding
This work was supported by Kimberly-Clark Corporation and carried out in collaboration with the Darcy Center. The first author received funding from the National Natural Science Foundation of China (Grant No. 42007165). The second author received funding from the European Research Council under the European Union’s Seventh Framework Program (FP/2007–2013)/ERC Grant Agreement No. 341225.
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LZ was involved in the methodology, software, validation, and writing–original draft; SMH was involved in the conceptualization, supervision, writing—review and editing, and funding acquisition; DB contributed to the methodology and supervision; CJD contributed to the data analysis and supervision.
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Appendices
Appendix 1: Including Evaporation Effect During Imbibition
The evaporation rate r was measured experimentally. In the experiment, a fully saturated fibrous layer was placed on a stainless-steel porous plate. The temporal changes of weight were recorded using a three-digit precision balance (Kern & Sohn GmbH, Germany). Figure
7 shows the saturation changes in the fibrous layer as a function of time. An evaporation rate of r = 0.165 h−1 was obtained by fitting the data linearly. We performed a set of simulations including evaporation during spontaneous imbibition process. The governing equations were modified by adding the evaporation term, − φr, to the right-hand side of Eq. (4). They are almost identical to the ones shown in Fig. 3a; this indicates that the influence of evaporation is negligible during spontaneous imbibition process here. This is to be expected as the time scale of evaporation was much larger than the one for our experiments (Fig.
8).
Appendix 2: Simulations Obtained by Adjusting Intrinsic and/or Relative Permeabilities
Figure
9a shows the simulation results obtained using the classical Richards equation with the intrinsic permeability value reduced by a factor of 9.2/4.2 = 2.19 compared to the value used in Simulations I–III. In an additional set of simulations, the relative permeability was also reduced by increasing the value of parameter l in Eq. (3) from 0.5 to 1.0. Results are shown in Fig. 9a, b, respectively. It is evident that reducing the intrinsic permeability was capable of decelerating the imbibition process, similarly to decreasing the relative permeability. However, the shape of saturation profiles and saturation value at x = 1 cm were unchanged. Clearly, the classical Richards equation was not capable of modeling the spontaneous imbibition process despite adjusting values of intrinsic and/or relative permeabilities.
Appendix 3: Simulations Obtained with Different τ–S Functions
Based on the studies of dynamic capillarity in soils (Zhuang et al. 2019), we have chosen five typical functional forms for the dynamic capillarity coefficient τ. The functions are shown in Table
3. The constant τ0 in each function was optimized and may vary in different functional forms. The simulation results using the quadratic power function τ4 are shown in Fig. 3. The selected simulation results obtained using the remaining four τ–S functions are shown in Fig.
10. Obviously, regardless of τ–S functional forms, including the dynamic capillarity term always improved the agreement with the wetted length of the layer at different times. Specifically, as shown in Fig. 10a, b, for τ1 and τ2, the saturation profiles were relatively steep with unchanged saturation at x = 1 cm. These simulations curves are not anywhere close to the measured values. The simulations using τ3 (linear) and τ5 (cubic power) gave a better agreement with the observations (see Fig. 10c, d). However, these results still showed either faster or slower temporal saturation changes at x = 0. The function τ4 (quadratic power function), therefore, was chosen as the best form for modeling dynamic capillarity in this work.
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Zhuang, L., Hassanizadeh, S.M., Bhatt, D. et al. Spontaneous Imbibition and Drainage of Water in a Thin Porous Layer: Experiments and Modeling. Transp Porous Med 139, 381–396 (2021). https://doi.org/10.1007/s11242-021-01670-7
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DOI: https://doi.org/10.1007/s11242-021-01670-7