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Application of carbon materials in catalytic systems for the hydrogenation—dehydrogenation of liquid organic hydrogen carriers

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Russian Chemical Bulletin Aims and scope

Abstract

Carbon materials with different textural characteristics (active carbon, carbon nanotubes, and Sibunite) for the purposes of hydrogen generation and storage and its evolution in processes using liquid organic hydrogen carriers are compared. A combination of structural and physicochemical characteristics (surface functionalization, controlled metal—carbon interaction, and relative chemical inertness) provides advantages of the modern carbon materials over oxides as catalyst carriers, since they allow the accumulation (hydrogenation) and evolution (dehydrogenation) of hydrogen to occur without cracking product formation. The prospects of the Sibunite-based Pt catalysts in these reactions are shown.

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Funding

This work was carried out in the framework of the state assignment of the N. D. Zelinsky Institute of Organic Chemistry of the Russian Academy of Sciences (FFZZ-2022-0005) and financially supported by the Russian Science Foundation (Project No. 23-73-30007).

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Authors and Affiliations

  1. Department of Chemistry, M. V. Lomonosov Moscow State University, 1/3 Leninskie Gory, 119991, Moscow, Russian Federation

    A. N. Kalenchuk, V. I. Bogdan, S. F. Dunaev & L. M. Kustov

  2. N. D. Zelinsky Institute of Organic Chemistry, Russian Academy of Sciences, 47 Leninsky prop., 119991, Moscow, Russian Federation

    A. N. Kalenchuk, V. I. Bogdan & L. M. Kustov

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  1. A. N. Kalenchuk
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  2. V. I. Bogdan
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  3. S. F. Dunaev
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  4. L. M. Kustov
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Correspondence to L. M. Kustov.

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The authors declare no competing interests.

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Dedicated to Academician of the Russian Academy of Sciences M. P. Egorov on the occasion of his 70th birthday.

Published in Russian in Izvestiya Akademii Nauk. Seriya Khimicheskaya, Vol. 73, No. 1, pp. 1–13, January, 2024.

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Kalenchuk, A.N., Bogdan, V.I., Dunaev, S.F. et al. Application of carbon materials in catalytic systems for the hydrogenation—dehydrogenation of liquid organic hydrogen carriers. Russ Chem Bull 73, 1–13 (2024). https://doi.org/10.1007/s11172-024-4118-9

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  • DOI: https://doi.org/10.1007/s11172-024-4118-9

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