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Formation of metal nanostructures under X-ray radiation in films of interpolyelectrolyte complexes with different silver ion content

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Abstract

The specific features of the formation of metal nanoparticles under X-ray radiation in interpolyelectrolyte complex (IPEC) films based on polyacrylic acid and polyethyleneimine with different silver ion content were studied. IPEC films were irradiated in aqueous-alcoholic medium. Electron microscopy demonstrated that the formation of silver nanoparticles occurred in zones regularly located by film thickness. It was found that nanoparticle size and spatial distribution in IPEC films depended on the initial concentration of silver ions within the sample and on the absorbed dose of radiation. The obtained film nanocomposites are promising objects for application as antibacterial and catalytic materials.

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References

  1. J. Dai, M. L. Bruening, Nano Lett., 2002, 2, 497; DOI: https://doi.org/10.1021/nl025547l.

    Article  CAS  Google Scholar 

  2. M. L. Bruening, D. M. Dotzauer, P. Jain, L. G. Ouyang, L. Baker, Langmuir, 2008, 24, 7663; DOI: https://doi.org/10.1021/la800179z.

    Article  CAS  Google Scholar 

  3. D. M. Dotzauer, A. Abusaloua, S. Miachon, J.-A. Dalmon, M. L. Bruening, Appl. Catal. BEnviron., 2009, 91, 180; DOI: https://doi.org/10.1016/j.apcatb.2009.05.022.

    Article  CAS  Google Scholar 

  4. A. A. Zezin, D. I. Klimov, E. A. Zezina, K. V. Mkrtchyan, V. I. Feldman, Radiat. Phys. Chem., 2020, 169, 108076; DOI: https://doi.org/10.1016/j.radphyschem.2018.11.030.

    Article  CAS  Google Scholar 

  5. D. V. Pergushov, A. A. Zezin, A. B. Zezin, A. H. E. Müller, Adv. Polym. Sci., 2014, 255, 173; DOI: https://doi.org/10.1007/12_2012_182.

    Article  CAS  Google Scholar 

  6. N. L. Rosi, C. A. Mirkin, Chem. Rev., 2005, 105, 1547; DOI: https://doi.org/10.1021/cr030067f.

    Article  CAS  Google Scholar 

  7. S. Fathalipour, S. Ahunbar, Polym. Sci., Ser. B, 2019, 61, 663; DOI: https://doi.org/10.1134/s1560090419050038.

    Article  Google Scholar 

  8. N. A. Samoilova, M. A. Krayukhina, O. V. Vyshivannaya, I. V. Blagodatskikh, D. A. Popov, N. M. Anuchina, I. A. Yamskov, Russ. Chem. Bull., 2018, 67, 1010; DOI: https://doi.org/10.1007/s11172-018-2172-x.

    Article  CAS  Google Scholar 

  9. D. I. Klimov, E. A. Zezina, V. C. Lipik, S. S. Abramchuk, A. A. Yaroslavov, V. I. Feldman, A. A. Zezin, Radiat. Phys. Chem., 2019, 162, 23; DOI: https://doi.org/10.1016/j.radphyschem.2019.04.027.

    Article  CAS  Google Scholar 

  10. A. A. Zezin, Polym. Sci., Ser. C, 2016, 58, 118; DOI: https://doi.org/10.1134/S1811238216010136.

    Article  CAS  Google Scholar 

  11. J. Belloni, Catal. Today, 2006, 113, 141; DOI: https://doi.org/10.1016/j.cattod.2005.11.082.

    Article  CAS  Google Scholar 

  12. V. A. Aleksandrova, L. N. Shirokova, Polym. Sci., Ser. B, 2018, 60, 727; DOI: https://doi.org/10.1134/s1560090418060027.

    Article  CAS  Google Scholar 

  13. A. A. Zezin, Polym. Sci., Ser. A, 2019, 61, 754; DOI: https://doi.org/10.1134/S0965545X19060154.

    Article  CAS  Google Scholar 

  14. F. Schacher, E. Betthausen, A. Walther, H. Schmalz, D. V. Pergushov, A. H. E. Müller, ACS Nano, 2009, 3, 2095; DOI: https://doi.org/10.1021/nn900110s.

    Article  CAS  Google Scholar 

  15. F. H. Schacher, T. Rudolph, M. Drechsler, A. H. E. Müller, Nanoscale, 2011, 3, 288; DOI: https://doi.org/10.1039/c0nr00649a.

    Article  CAS  Google Scholar 

  16. Z. Lei, X. Wei, L. Zhang, S. Bi, Colloids Surf. A: Physicochem. Eng. Asp., 2008, 317, 705; DOI: https://doi.org/10.1016/j.colsurfa.2007.12.006.

    Article  CAS  Google Scholar 

  17. V. Demchenko, S. Riabov, V. Shtompel’, Nanoscale Res. Lett., 2017, 12, 235; DOI: https://doi.org/10.1186/s11671-017-1967-2.

    Article  Google Scholar 

  18. V. Demchenko, V. Shtompel’, S. Riabov, Eur. Polym. J., 2016, 75, 310; DOI: https://doi.org/10.1016/j.eurpolymj.2016.01.004.

    Article  CAS  Google Scholar 

  19. A. A. Zezin, V. I. Feldman, S. S. Abramchuk, V. K. Ivanchenko, E. A. Zezina, N. A. Shmakova, V. I. Schvedunov, Polym. Sci., Ser. C, 2011, 53, 61; DOI: https://doi.org/10.1134/S1811238211060038.

    Article  CAS  Google Scholar 

  20. V. I. Feldman, A. A. Zezin, S. S. Abramchuk, E. A. Zezina, J. Phys. Chem. C, 2013, 117, 7286; DOI: https://doi.org/10.1021/jp3090765.

    Article  CAS  Google Scholar 

  21. A. G. Chmielewski, D. K. Chmielewska, J. Michalik, M. H. Sampa, Nucl. Instrum. Methods Phys. Res. B, 2007, 265, 339; DOI: https://doi.org/10.1016/j.nimb.2007.08.069.

    Article  CAS  Google Scholar 

  22. W. Abidi, H. Remita, Recent Pat. Eng., 2010, 4, 170; DOI: https://doi.org/10.2174/187221210794578556.

    Article  CAS  Google Scholar 

  23. R. Yoksan, S. Chirachanchai, Mater. Chem. Phys., 2009, 115, 296; DOI: https://doi.org/10.1016/j.matchemphys.2008.12.001.

    Article  CAS  Google Scholar 

  24. B. G. Ershov, E. V. Abkhalimov, Colloid J., 2006, 68, 417; DOI: https://doi.org/10.1134/s1061933x06040041.

    Article  CAS  Google Scholar 

  25. D. I. Klimov, E. A. Zezina, S. B. Zezin, M. Yang, F. Wang, V. I. Shvedunov, A. A. Zezin, Radiat. Phys. Chem., 2018, 142, 65; DOI: https://doi.org/10.1016/j.radphyschem.2017.02.034.

    Article  CAS  Google Scholar 

  26. A. A. Zezin, V. I. Feldman, A. V. Dudnikov, S. B. Zezin, S. S. Abramchuk, S. I. Belopushkin, High Energy Chem., 2009, 43, 100; DOI: https://doi.org/10.1134/S0018143909020064.

    Article  CAS  Google Scholar 

  27. A. A. Zezin, V. I. Feldman, E. A. Zezina, S. I. Belopushkin, E. V. Tsybina, S. S. Abramchuk, S. B. Zezin, High Energy Chem., 2011, 45, 99; DOI: https://doi.org/10.1134/S0018143911020147.

    Article  CAS  Google Scholar 

  28. A. S. Pozdnyakov, G. F. Prozorova, S. S. Abramchuk, V. I. Feldman, A. A. Zezin, E. A. Zezina, A. I. Emel’yanov, Radiat. Phys. Chem., 2019, 158, 115; DOI: https://doi.org/10.1016/j.radphyschem.2019.01.019.

    Article  Google Scholar 

  29. J. H. Hubbel, S. M. Seltzer, Radiat. Phys. Division, PML, NIST, 1995; DOI: https://dx.doi.org/10.18434/T4D01F.

  30. J. D. Hanawalt, H. W. Rinn, L. K. Frevel, Industr. Eng. Chem. Anal. Ed., 1938, 10, 457; DOI: https://doi.org/10.1021/ac50125a001.

    Article  CAS  Google Scholar 

  31. P. Wardman, J. Phys. Chem. Ref. Data, 1989, 18, 1637; DOI: https://doi.org/10.1063/1.555843.

    Article  CAS  Google Scholar 

  32. B. G. Ershov, E. Janata, A. Henglein, J. Phys. Chem., 1993, 97, 339; DOI: https://doi.org/10.1021/j100104a013.

    Article  CAS  Google Scholar 

  33. M. Mostafavi, N. Keghouche, M.-O. Delcourt, J. Belloni, Chem. Phys. Lett., 1990, 167, 193; DOI: https://doi.org/10.1016/0009-2614(90)85004-v.

    Article  CAS  Google Scholar 

  34. M. Mostafavi, N. Keghouche, M.-O. Delcourt, Chem. Phys. Lett., 1990, 169, 81; DOI: https://doi.org/10.1016/0009-2614(90)85169-d.

    Article  CAS  Google Scholar 

  35. B. G. Ershov, J. Phys. Chem., 1998, 102, 10663; DOI: https://doi.org/10.1021/jp981906i.

    Article  CAS  Google Scholar 

  36. M. Anbar, M. Bambenek, A. B. Ross, Selected Specific Rates of Reactions of Transients from Water in Aqueous Solution, I. Hydrated Electron, NSRDS-NBS 43, National Bureau of Standards, U.S. Department of Commerce, Washington, 1973; DOI: https://doi.org/10.2172/4445489.

    Book  Google Scholar 

  37. B. G. Ershov, Russ. Chem. Bull., 1994, 43, 16; DOI: https://doi.org/10.1007/bf00699128.

    Article  Google Scholar 

Download references

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Authors and Affiliations

  1. N. S. Enikolopov Institute of Synthetic Polymeric Materials, Russian Academy of Sciences, 70 ul. Profsoyuznaya, 117393, Moscow, Russian Federation

    K. V. Mkrtchyan & A. A. Zezin

  2. Department of Chemistry, Lomonosov Moscow State University, Build. 11, 1 Leninskie Gory, 119991, Moscow, Russian Federation

    A. A. Zezin, E. A. Zezina & I. A. Baranova

  3. A. N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, 28 ul. Vavilova, 119334, Moscow, Russian Federation

    S. S. Abramchuk

Authors
  1. K. V. Mkrtchyan
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  2. A. A. Zezin
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  3. E. A. Zezina
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  4. S. S. Abramchuk
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  5. I. A. Baranova
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Correspondence to A. A. Zezin.

Additional information

Based on the materials of the XXI Mendeleev Congress on General and Applied Chemistry (September 9–13, 2019, St. Petersburg, Russia).

Published in Russian in Izvestiya Akademii Nauk. Seriya Khimicheskaya, No. 9, pp. pp. 1731–1739, September, 2020.

This work was financially supported by the Russian Foundation for Basic Research (Project No. 18-03-00608).

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Mkrtchyan, K.V., Zezin, A.A., Zezina, E.A. et al. Formation of metal nanostructures under X-ray radiation in films of interpolyelectrolyte complexes with different silver ion content. Russ Chem Bull 69, 1731–1739 (2020). https://doi.org/10.1007/s11172-020-2956-7

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  • DOI: https://doi.org/10.1007/s11172-020-2956-7

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