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Exploring the potential of Cu-LDHs composite for efficient Coomassie brilliant blue dye removal: evaluating adsorption isotherms and antibacterial activity

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Abstract

This study presents the synthesis and characterization of a copper-based layered double hydroxide (Cu-LDH) composite via the coprecipitation method. The composite material aimed to effectively remove the anionic dye “Coomassie Brilliant Blue” (CBB) and exhibit antibacterial properties against both gram-positive and gram-negative bacteria. The synthesized nanocomposites were characterized using various techniques. The adsorption of CBB dye was investigated by studying various physicochemical variables, including contact time, pH of the dye solution, and initial dye concentration. The optimal dosage and contact time for efficient CBB dye removal were determined as 0.07 g and 10 min, respectively. The results showed that Cu-LDHs exhibited a high adsorption capacity for CBB dye, with a maximum removal efficiency of 85% which could be achieved within 10  min, and the Cu-LDHs improved an experimental adsorption capacity at equilibrium qmax = 80 mg/g. The adsorption process followed a pseudo-second-order kinetic model. The Langmuir isotherm model provided a good fit to the equilibrium data, indicating monolayer adsorption. Furthermore, the antibacterial activity of Cu-LDHs was assessed against various bacterial strains using a diffusion method. The results demonstrated the inhibitory effects of Cu-LDHs and CBB-Cu-LDHs on bacterial growth at a dosage of 10 mg, indicating the potential of Cu-LDHs as antibacterial agents. The underlying mechanisms responsible for dye adsorption and antibacterial activity were discussed.

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Acknowledgements

I would like to thank Mr Abdelkader Tabti for his assistance and support throughout all aspects of our study.

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Authors and Affiliations

  1. Laboratory of Excellence in Applied Organic Synthesis, Faculty of Exact and Applied Sciences, University Oran1 Ahmed Ben Bella, BP 1524 El M’Naouer, 31000, Oran, Algeria

    Hadja Alia Tabti, Abdelkader Ammam, Bouthaina Doumi, Rafik Abdelkrim Boudia & Mehdi Adjdir

  2. Faculty of Science and Technology, Ahmed Ben Yahia El Wancharissi University, 38000, Tissemsilt, Algeria

    Hadja Alia Tabti

  3. Biotoxicology Pharmacognosy and Biological Valorization of Plants Laboratory, Department of Biology, Faculty of Science, University of Dr. Tahar Moulay, 20000, Saida, Algeria

    Abdelkader Ammam

  4. Laboratory of Separation and Purification Technology, Department of Chemistry, Faculty of Science, University of Abou Bekr Belkaid, 13000, Tlemcen, Algeria

    Brahim Guezzen

  5. Department of Engineering Process, Faculty of Technology, University of Dr. Tahar Moulay, 20000, Saida, Algeria

    Mohamed Boudinar & Abdelkader Kadeche

  6. Laboratory of Elaboration and Spectroscopic Characterizations of Structural and Electronic Properties of Materials, Faculty of Technology, University of Dr.Tahar Moulay, 20000, Saida, Algeria

    Mohamed Boudinar, Amina Ramdani & Mehdi Adjdir

  7. Laboratory of Materials and Catalysis, Faculty of Sciences, Site I BP 89 Djillali Liabès’s University, 22000, Sidi-Abbès, Algeria

    Amina Ramdani

  8. Faculty of Sciences and Technology, University Belhadj Bouchaib, BP 284, 46000, Ain-Temouchent, Algeria

    Abdelkader Nebatti Ech-Chergui

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We wish to draw the attention of the Editor that all authors "Hadja Alia Tabti, Abdelkader Ammam, Brahim Guezzen, Mohamed Boudinar, Abdelkader Kadeche, Amina Ramdani, Bouthaina Doumi, Abdelkader Nebatti Ech-Chergui, Rafik Abdelkrim Boudia, Mehdi Adjdir” participated in contributing the text manuscript, and all authors have accepted responsibility for the entire content of this manuscript and approved its submission

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Tabti, H.A., Ammam, A., Guezzen, B. et al. Exploring the potential of Cu-LDHs composite for efficient Coomassie brilliant blue dye removal: evaluating adsorption isotherms and antibacterial activity. Res Chem Intermed (2024). https://doi.org/10.1007/s11164-024-05288-4

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