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Research progress on selective catalytic reduction of NOx by NH3 over copper zeolite catalysts at low temperature: reaction mechanism and catalyst deactivation

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Abstract

Selective catalytic reduction (SCR) system is considered to be the most effective control method for reducing NOx in exhaust gas post-treatment of the diesel engine. Catalysts are the main factors affecting de-NOx efficiency in SCR reactions. In recent years, due to the excellent characteristics of copper zeolite catalysts, they have been widely studied as low-temperature NH3-SCR catalysts. However, the development of low-temperature SCR catalysts with high removal efficiency still faces severe challenges. This paper reviewed the latest research progress with copper zeolite catalysts at low temperature and compared the action mechanism of various copper zeolite catalysts in NH3-SCR reactions. Copper zeolite catalysts were studied from the aspects of catalytic performance, preparation strategy, broadening the operating temperature window, hydrothermal deactivation and resistance to H2O and SO2. Several solutions to the problems existing in low-temperature NH3-SCR reactions were discussed. In addition, this paper also puts forward some views on the future research direction of copper zeolite catalysts. Finally, the summaries and prospects of the development of low-temperature SCR copper zeolite catalysts were presented. Hopefully, more researchers can understand the current research status of copper zeolite catalysts and obtain better research achievements from copper zeolite catalysts in the future. This review could pave the way for similar studies to enable a wider variety of copper zeolite catalysts to be commercially available.

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Funding

This work is funded by the National Nature Science Foundation of China under the research grant of No. 52165055. This research is also funded by the Guangxi University of Science and Technology Doctoral Fund under the research grant of 13Z10.

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Authors and Affiliations

  1. School of Mechanical and Automotive Engineering, Guangxi University of Science and Technology, Liuzhou, 545006, China

    Jianbin Luo, Hongxiang Xu, Xiguang Liang, Shizhuo Wu, Zhonghang Liu, Yuanhao Tie, Mingsen Li & Dayong Yang

  2. Institute of the New Energy and Energy-Saving and Emission-Reduction, Guangxi University of Science and Technology, Liuzhou, 545006, China

    Jianbin Luo, Hongxiang Xu, Xiguang Liang, Shizhuo Wu, Zhonghang Liu, Yuanhao Tie & Mingsen Li

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  1. Jianbin Luo
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Contributions

JL contributed to method, funding acquisition, conceptualization, and writing—review and editing. HX contributed to resources, project administration, method, software, data curation, writing—original draft, and writing—review and editing. XL contributed to project administration and method. SW contributed to investigation and method. ZL contributed to software and formal analysis. YT contributed to project administration and writing—review and editing. ML performed data curation and writing—review and editing. DY contributed to conceptualization, methodology, resources, and writing—original draft.

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Correspondence to Jianbin Luo.

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Luo, J., Xu, H., Liang, X. et al. Research progress on selective catalytic reduction of NOx by NH3 over copper zeolite catalysts at low temperature: reaction mechanism and catalyst deactivation. Res Chem Intermed 49, 2321–2357 (2023). https://doi.org/10.1007/s11164-022-04938-9

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