Abstract
In this study, a comprehensive model for the numerical simulation of electrical and optical characteristics of multilayer organic light-emitting devices (OLED) is presented. The model consists of three parts: charge carrier transport model, exciton model, and a post-processing part for calculating luminance. The defect states in the organic layers are modeled and are introduced into the equations. For demonstrating the rule of the defect states in such devices, a multilayer OLED is considered consisting of a host–guest emissive layer sandwiched between electron and hole transport layers. The current density and luminance results of the analyzed device are compared with the experimental data. We have found that by considering the defect states, there is good accordance between the simulation results and the experimental data.
Similar content being viewed by others
References
Al-Sadi, M., Jaiser, F., Bagnich, S., Unger, T., Blakesley, J., Wilke, A., Neher, D.: Electrical and optical simulations of a polymer-based phosphorescent organic light-emitting diode with high efficiency. J. Polym. Sci. Part b Polym. Phys. 50, 1567–1576 (2012)
Arkhipov, V.I., Heremans, P., Emelianova, E.V., Adriaenssens, G.J., Bässler, H.: Charge carrier mobility in doped semiconducting polymers. Appl. Phys. Lett. 82, 3245–3247 (2003)
Arkhipov, V.I., Heremans, P., Emelianova, E.V., Adriaenssens, G.J., Bässler, H.: Charge carrier mobility in doped disordered organic semiconductors. J. Non. Cryst. Solids. 338, 603–606 (2004)
Ayobi, A., Mirnia, S.N., Roknabadi, M.R., Bahari, A.: Investigation of charge trapping induced by DCM–TPA dopant in organic light emitting devices composed of (NPB: Alq 3): DCM–TPA mixed host-doped emitting layer. Trans. Electr. Electron. Mater. 20, 240–251 (2019)
Bulovic, V., Bulović, V., Shoustikov, A., Baldo, M.A., Bose, E., Kozlov, V.G., Thompson, M.E., Forrest, S.R.: Bright, saturated, red-to-yellow organic light-emitting devices based on polarization-induced spectral shifts. Chem. Phys. Lett. 287, 455–460 (1998)
Chang, Y., Liu, S., Chen, C., Yuan, C., Liu, L., Chen, Y., Su, W., Lee, K., Wu, C., Lee, C.: A new model for optimization of organic light-emitting device by concurrent incorporation of electrical and optical simulations. J. Appl. Phys. 084507, 1–9 (2012)
Cheon, K.O., Shinar, J.: Electroluminescence spikes, turn-off dynamics, and charge traps in organic light-emitting devices. Phys. Rev. B. 69, 201306 (2004)
Davids, P.S., Campbell, I.H., Smith, D.L.: Device model for single carrier organic diodes. J. Appl. Phys. 82, 6319–6325 (1997)
Duke, C.B.: Tunneling in Solids. Academic Press, Amsterdam (1969)
Fishchuk, I.I., Kadashchuk, A.K., Bässler, H., Weiss, D.S.: Nondispersive charge-carrier transport in disordered organic materials containing traps. Phys. Rev. B. 66, 205208 (2002)
Förster, T.: Transfer mechanisms of electronic excitation. Discuss. Faraday Soc. 27, 7–17 (1959)
Gao, W.B., Sun, J.X., Yang, K.X., Liu, H.Y., Zhao, J.H., Liu, S.Y.: Improved performances of the organic light-emitting devices by doping in the mixed layer. Opt. Quantum Electron. 35, 1149–1155 (2003)
Gusso, A., Ma, D., Hümmelgen, I.A., Da Luz, M.G.E.: Modeling of organic light-emitting diodes with graded concentration in the emissive multilayer. J. Appl. Phys. 95, 2056–2062 (2004)
Heeger, A.J.: Semiconducting and metallic polymers: the fourth generation of polymeric materials. Angewandte Chem Int 40, 2591–2611 (2001)
Jeong, H., Shin, H., Lee, J., Kim, B., Park, Y.-I., Yook, K.S., An, B.-K., Park, J.: Recent progress in the use of fluorescent and phosphorescent organic compounds for organic light-emitting diode lighting. J. Photonics Energy. 5, 57608 (2015)
Jurchescu, O.D., Baas, J., Palstra, T.T.M.: Effect of impurities on the mobility of single crystal pentacene. Appl. Phys. Lett. 84, 3061–3063 (2004)
Kalyani, N.T., Swart, H., Dhoble, S.J.: Principles and Applications of Organic Light Emitting Diodes (OLEDs). Elsevier Science (2017)
Karg, S., Steiger, J., Von Seggern, H.: Determination of trap energies in Alq3 and TPD. Synth. Met. 111, 277–280 (2000)
Kawamura, Y., Brooks, J., Brown, J.J., Sasabe, H., Adachi, C.: Intermolecular interaction and a concentration-quenching mechanism of phosphorescent Ir (III) complexes in a solid film. Phys. Rev. Lett. 96, 17404 (2006)
Kido, J.: Organic displays. Phys. World. 12, 27 (1999)
Knapp, E., Ruhstaller, B.: Numerical analysis of steady-state and transient charge transport in organic semiconductor devices. Opt. Quantum Electron. 42, 667–677 (2011)
Kozlov, V.G., Bulovic, V., Burrows, P.E., Baldo, M., Khalfin, V.B., Parthasarathy, G., Forrest, S.R., You, Y., Thompson, M.E.: Study of lasing action based on Förster energy transfer in optically pumped organic semiconductor thin films. J. Appl. Phys. 84, 4096–4108 (1998)
Lee, C.-C., Chang, M.-Y., Huang, P., Chen, Y.C., Chang, Y., Liu, S.-W.: Electrical and optical simulation of organic light-emitting devices with fluorescent dopant in the emitting layer. J. Appl. Phys. 101, 114501 (2007)
Lee, C.-C., Jong, Y.-D., Huang, P.-T., Chen, Y.C., Hu, P.-J., Chang, Y.: Numerical simulation of electrical model for organic light-emitting devices with fluorescent dopant in the emitting layer. Jpn. J. Appl. Phys. 44, 8147 (2005)
Lee, C., Jong, Y., Huang, P., Hsu, S., Laskar, I.R., Chen, T., Zhi-jun, W., Shu-fen, C.: Numerical simulation of electrical and optical characteristics of multilayer organic light-emitting devices. Jpn. J. Appl. Phys. 43, 7560–7565 (2004)
Luhman, W.A., Holmes, R.J.: Investigation of energy transfer in organic photovoltaic cells and impact on exciton diffusion length measurements. Adv. Funct. Mater. 21, 764–771 (2011)
Nguyen, T.-P.: Defects in organic electronic devices. Phys. Status Solidi. 205, 162–166 (2008)
Park, J., Kawakami, Y., Park, S.-H.: Numerical analysis of multilayer organic light-emitting diodes. J. Light. Technol. 25, 2828–2836 (2007)
Pope, M., Swenberg, C.E.: Electronic Processes in Organic Crystals and Polymers. Oxford University Press, New York (1999)
Pourjavad, M.A., Farjamtalab, I., Sabbaghi-Nadooshan, R.: Influence of doped Alq3 layer on performance of MEH-PPV, MDMO-PPV, and P3HT polymer light-emitting diodes. Opt. Quantum Electron. 48, 421 (2016)
Ruhstaller, B., Beierlein, T., Riel, H., Karg, S., Scott, J.C., Riess, W.: Simulating electronic and optical processes in multilayer organic light-emitting devices. IEEE J. Sel. Top. Quantum Electron. 9, 723–731 (2003)
Ruhstaller, B., Carter, S.A., Barth, S., Riel, H., Riess, W., Scott, J.C.: Transient and steady-state behavior of space charges in multilayer organic light-emitting diodes. J. Appl. Phys. 89, 4575–4586 (2001)
Scharfetter, D.L., Gummel, H.K.: Large-signal analysis of a silicon read diode oscillator. IEEE Trans. Electron Devices. 16, 64–77 (1969)
Scott, J.C., Malliaras, G.G.: Charge injection and recombination at the metal–organic interface. Chem. Phys. Lett. 299, 115–119 (1999)
Shen, J., Yang, J.: Physical mechanisms in double-carrier trap-charge limited transport processes in organic electroluminescent devices: a numerical study. J. Appl. Phys. 83, 7706–7714 (1998)
Shinar, J.: Organic Light-Emitting Devices: A Survey. Springer, New York (2013)
Staudigel, J., Stößel, M., Steuber, F., Simmerer, J.: A quantitative numerical model of multilayer vapor-deposited organic light emitting diodes. J. Appl. Phys. 3895, 3895–3910 (1999)
Steiger, J., Schmechel, R., Von Seggern, H.: Energetic trap distributions in organic semiconductors. Synth. Met. 129, 1–7 (2002)
Stoessel, M., Wittmann, G., Staudigel, J., Steuber, F., Blässing, J., Roth, W., Klausmann, H., Rogler, W., Simmerer, J., Winnacker, A.: Cathode-induced luminescence quenching in polyfluorenes. J. Appl. Phys. 87, 4467–4475 (2000)
Sze, S.: Physics of Semiconductor Devices. Wiley, New York (1981)
Walker, A.B., Kambili, A., Martin, S.J.: Electrical transport modelling in organic electroluminescent devices. J. Phys. Condens. Matter. 14, 9825–9876 (2002)
Yang, K., East, J.R., Haddad, G.I.: Numerical modeling of abrupt heterojunctions using a thermionic-field emission boundary condition. Solid. State. Electron. 36, 321–330 (1993)
Author information
Authors and Affiliations
Corresponding author
Additional information
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
About this article
Cite this article
Sheykholeslami Nasab, P., Davoudi Darareh, M., Yousefi, M.H. et al. Numerical simulation of multilayer organic light-emitting diodes with host–guest emissive layer: the role of defect states. Opt Quant Electron 52, 271 (2020). https://doi.org/10.1007/s11082-020-02387-5
Received:
Accepted:
Published:
DOI: https://doi.org/10.1007/s11082-020-02387-5