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The production of no carrier added arsenic radioisotopes in nuclear reactors

Journal of Radioanalytical and Nuclear Chemistry volume 319, pages 175–184 (2019)Cite this article

Abstract

The comparative advantages and drawbacks of some reactor-produced arsenic radioisotopes having favourable characteristics for their use as tracers are discussed. The study comprises their preparation based on: (a) capture reactions on germanium; (b) threshold reactions on germanium, selenium and bromine; (c) secondary reactions on germanium, induced by recoil protons and tritons produced by the action of neutrons on lithium. The recommended options for the production of relatively short half-life radionuclides are 77As by capture on germanium or 76As via (n,α) reaction on bromine, while two different ways are applicable for the production of 74As, longer-lived radioisotope.

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Authors and Affiliations

  1. Centro de Tecnologías Químicas, Universidad Tecnológica Nacional, Facultad Regional Buenos Aires, Medrano 951, C1179AAQ, Ciudad Autónoma de Buenos Aires, República Argentina

    Sandra Siri, María Sol Segovia & Isaac Marcos Cohen

  2. Centro Atómico Ezeiza, Comisión Nacional de Energía Atómica, Presbítero González y Aragón 15, B1802AYA, Buenos Aires, Argentina

    Sandra Siri

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  1. Sandra Siri
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  2. María Sol Segovia
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Correspondence to Sandra Siri.

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Siri, S., Segovia, M.S. & Cohen, I.M. The production of no carrier added arsenic radioisotopes in nuclear reactors. J Radioanal Nucl Chem 319, 175–184 (2019). https://doi.org/10.1007/s10967-018-6278-2

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