Abstract
Field measurement of isotopic ratios may be used to fingerprint an element’s origin, be it from commercial power, industrial, medical or historical weapons fallout. Samples of samarium radionuclides were prepared by neutron activation for subsequent analysis using accelerator mass spectrometry (AMS). High purity samarium (III) oxide powder was irradiated in the University of Texas at Austin TRIGA reactor to a total neutron fluence of 5 × 1015 cm−2. An initial determination of the isotopic ratios was made using activation calculations with a BURN card in an MCNPX-based model of the TRIGA core. Experimental validation of the MCNP results was achieved by analyzing gamma spectra of the irradiated oxide powers after irradiation. Subsequent measurement of 151Sm will be conducted at the CAMS facility at LLNL demonstrating the first measurement of this isotope at this facility.
Similar content being viewed by others
References
Whitney SM, Biegalski S (2008) Nucl Sci Eng 157:200–209
Vogel JS et al (1995) Anal Chem 67:353–357
Kutschera W (2005) Int J Mass Spectrom 242:145–160
Bucholz BA et al (2010) Nucl Instr Meth B 268:773–775
Chart of Nuclides (2012) National Nuclear Data Center, Brookhaven National Laboratory. http://www.nndc.bnl.gov/chart/. Accessed 12 February 2012
MCNPX 2.6.0 Manual (2012) MCNPX Homepage. mcnpx.lanl.gov/docs/MCNPX_2.6.0_Manual.pdf. Accessed 1 January 2012
Acknowledgments
The authors would like to thank Department of Defense Threat Reduction Agency Grant #HDTRA1-08-1-0032 for support of this work. In addition, the authors appreciate the staff at the Nuclear Engineering Teaching Laboratory at the University of Texas at Austin for operational and experimental support. This work was performed in part under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Graham, J., Biegalski, S. & Bucholtz, B. Preparation of radio-Sm by neutron activation for accelerator mass spectrometry. J Radioanal Nucl Chem 296, 233–236 (2013). https://doi.org/10.1007/s10967-012-1953-1
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10967-012-1953-1