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Revived BBFTO double perovskite with improved dielectric properties for some possible device applications

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A Correction to this article was published on 26 August 2023

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Abstract

A solid-state reaction procedure was followed to synthesize the BaBi1.4Fe0.6TiO6 ceramic. To compensate for the Bi3+ evaporation during the high-temperature sintering process, more Bi3+ content was so selected, further, it adds more promising ferroelectric and dielectric orders. The monoclinic crystal system formation was checked by the X-Ray Diffraction and Rietveld refinement methods. The average crystallite size is 37.46 nm, while the average grain size is 137.28 nm, which implies that a single grain might have contained some single-phase crystallites. The Energy-Dispersive X-Ray spectrum confirmed the sample’s elemental purity. The material belongs to a perovskite phase, which was supported by some appeared usual vibrational modes in the Fourier-Transform Infrared analysis. The UV–Visible absorbance property results cutoff wavelength of 590 nm and the optical direct bandgap Eg = 2.53 eV. The remanent magnetization of 2Pr = 0.782µC/cm2 supports the ferroelectric nature. The room temperature (RT) dielectric parameter at 100 Hz has a higher ɛr (1408) and lower tanδ (0.24) as well as a higher transition (Td > 350 °C) and Curie temperature (Tc > 485 °C). Deviation from the Debye-type relaxation process and semiconducting nature were observed in the sample. The conductivity nature is obedient to the Arrhenius law, which results in dc conductivity activation energy, Ea = 0.94 eV.

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Some of the data generated during this study are included in this article. The rest datasets generated during the current study are available from the corresponding author on reasonable request.

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Authors and Affiliations

  1. Department of Physics, Faculty of Engineering & Technology, Siksha O Anusandhan University (Deemed to be University), Khandagiri, Bhubaneswar, 751030, India

    Lutu Sahoo & R. K. Parida

  2. Department of Physics, Central Institute of Technology, Kokrajhar (Deemed to be University, MHRD, Govt. of India), BTC, Kokrajhar, Assam, 783370, India

    B. N. Parida

  3. Department of Chemistry, Faculty of Engineering & Technology, Siksha O Anusandhan University (Deemed to be University), Khandagiri, Bhubaneswar, 751030, India

    Nimai C. Nayak

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  1. Lutu Sahoo
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Contributions

LS: Performed the samples preparation, measurements and paper redaction. BNP: Performed the dielectric measurements and P-E measurement and contributed to the discussion of the dielectric P-E properties. NCN: Performed the UV measurements and contributed to the discussion of the UV properties. RKP: Contributed to the discussion of the structural and morphologic properties.

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Correspondence to B. N. Parida or R. K. Parida.

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Sahoo, L., Parida, B.N., Nayak, N.C. et al. Revived BBFTO double perovskite with improved dielectric properties for some possible device applications. J Mater Sci: Mater Electron 34, 1019 (2023). https://doi.org/10.1007/s10854-023-10434-6

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