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Effect of BaO–2B2O3 sintering aid on the structural and electrical properties of high temperature piezoelectric ceramic Bi3TiNbO9

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Abstract

High temperature piezoelectric ceramic Bi3TiNbO9 with the addition of BaO–2B2O3 as sintering aid was prepared by a solid-state reaction method. The addition of BaO–2B2O3 can promote the growth of grains and increase the density of the samples. Both the ferroelectric and piezoelectric properties of Bi3TiNbO9 with the addition of BaO–2B2O3 increase remarkably compared with Bi3TiNbO9. The maximum remanent polarization and piezoelectric coefficient of the sample with the addition of 2 wt% BaO–2B2O3 can reach 8.67 µC/cm2 of 14 pC/N, which is about 4 and 7 times as large as the corresponding values of Bi3TiNbO9. The increased electrical properties can be ascribed to the dense morphology, the increased structural distortion, and the reduced concentration of oxygen vacancies. This study is useful for the preparation of high-temperature piezoelectric ceramic Bi3TiNbO9 with reasonable electrical properties.

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Funding

This work was supported by the National Key Research and Development Program of China (2017YFA0403502) and the Joint Funds of the National Natural Science Foundation of China and the Chinese Academy of Sciences’ Large-Scale Scientific Facility (Grant No. U1832115).

Author information

Authors and Affiliations

  1. Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, 230031, People’s Republic of China

    M. Tao, C. B. Pan, L. H. Yin, W. H. Song, X. B. Zhu, J. Yang & Y. P. Sun

  2. University of Science and Technology of China, Hefei, 230026, People’s Republic of China

    M. Tao & C. B. Pan

  3. High Magnetic Field Laboratory, Chinese Academy of Sciences, Hefei, 230031, People’s Republic of China

    Y. P. Sun

  4. Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, People’s Republic of China

    Y. P. Sun

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  1. M. Tao
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  3. L. H. Yin
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  4. W. H. Song
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  6. J. Yang
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Contributions

MT and JY: contributed to writing of the original draft. MT and CP: contributed to material preparation and data collection. LY, WS, XZ, and YS: contributed to data analysis and manuscript preparation. JY: also contributed to the conception of the study, project administration, and funding acquisition.

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Correspondence to J. Yang.

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Tao, M., Pan, C.B., Yin, L.H. et al. Effect of BaO–2B2O3 sintering aid on the structural and electrical properties of high temperature piezoelectric ceramic Bi3TiNbO9. J Mater Sci: Mater Electron 34, 535 (2023). https://doi.org/10.1007/s10854-023-09946-y

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  • DOI: https://doi.org/10.1007/s10854-023-09946-y

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