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Broadening the dielectric stability temperature range of BNBST relaxor ferroelectric ceramics by rare earth Ce doping for energy storage

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Abstract

(Bi0.5Na0.5)0.65(Ba0.3Sr0.7)0.35Ti1-XCeXO3 (abbreviated as BNBSTC100x, x = 0, 0.01, 0.02, 0.03, 0.04, 0.05, 0.06, 0.07, 0.08) ceramics were prepared by a solid-state reaction method. The effect of rare earth Ce-doping content on the phase structure, microstructure, dielectric properties and energy storage characteristics of ceramics was investigated. All BNBSTC100x ceramics had a single pseudocubic perovskite structure with high bulk density. With the increase of Ce-doping content, the dielectric peak of BNBSTC100x ceramics was gradually suppressed and flattened, which effectively broadened the dielectric stability temperature range. Meanwhile, the P-E hysteresis loop of the ceramics gradually changed to slim with Ce content, and the optimized energy storage properties were achieved in BNBSTC4 ceramics with recoverable energy storage density Wrec = 1.15 J/cm3 and efficiency η = 81% under a relatively low electric field of 100 kV/cm. Furthermore, the BNBSTC4 ceramics also exhibited good temperature, frequency and fatigue cycle stability, which should be a good candidate ceramic material for pulse power capacitors used in a wider temperature range.

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The datasets generated during and/or analyzed during the current work are available from the corresponding author on reasonable request.

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Acknowledgements

This work was supported by National Natural Science Foundation of China (52267002), Natural Science Foundation of Jiangxi Province (20212ACB204010), and Science & Technology Research Project of Jiangxi Provincial Education Department (GJJ211301).

Funding

This work was supported by National Natural Science Foundation of China (52267002), Natural Science Foundation of Jiangxi Province (20212ACB204010), and Science & Technology Research Project of Jiangxi Provincial Education Department (GJJ211301).

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Author notes

  1. Wen Zhu and Wei Deng have contributed equally to this work.

Authors and Affiliations

  1. China National Light Industry Key Laboratory of Functional Ceramic Materials, Energy Storage and Conversion Ceramic Materials Engineering Laboratory of Jiangxi Province, Advanced Ceramic Materials Research Institute, School of Materials Science and Engineering, Jingdezhen Ceramic University, Jingdezhen, 333403, China

    Wen Zhu, Wei Deng, Zhipeng Li, Zong-Yang Shen, Xuhai Shi, Fusheng Song, Wenqin Luo, Zhumei Wang & Yueming Li

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  1. Wen Zhu
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  2. Wei Deng
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Contributions

WZ and WD: conceptualization, methodology, writing, contributed equally to the manuscript. ZL: methodology and manuscript revision. Z-YS: project administration, conceptualization, methodology and manuscript revision. XS: assist in data handling. FS: assist in data handling. WL: language organization and editing. ZW: assist in data handling. YL: assist in data handling.

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Correspondence to Zong-Yang Shen.

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Zhu, W., Deng, W., Li, Z. et al. Broadening the dielectric stability temperature range of BNBST relaxor ferroelectric ceramics by rare earth Ce doping for energy storage. J Mater Sci: Mater Electron 33, 26861–26869 (2022). https://doi.org/10.1007/s10854-022-09351-x

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