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Dielectric and energy storage properties of Ba0.85Ca0.15Zr0.1Ti0.9O3 ceramics with different aging temperature during the sol–gel process

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Abstract

A series of Ba0.85Ca0.15Zr0.1Ti0.9O3 (referred to as BCZT) ceramics were fabricated by the sol–gel method with different aging temperatures. The structure, dielectric property, and the energy storage property were researched. Compared with the BCZT synthesized with the traditional solid-state reaction method, the samples prepared by the sol–gel method have obvious advantages in various performances. And a strong influence of aging temperature on the BCZT ceramics was observed. The suitable aging temperature can broaden the dielectric peak and decrease the Curie temperature. In addition, the optimal BCZT sample with the aging temperature of 60 °C exists a high permittivity (εr ~ 3141) and a low dielectric loss (tanδ ~ 0.012) at the frequency of 102 Hz. Moreover, the coercive field and remnant polarization of the BCZT were greatly decreased, contributing to slim hysteresis loops. Notably, the thinner P-E loop contributes a high energy storage efficiency (76.6%) at 40 kV/cm electric field which is much higher than the BCZT synthesized by the traditional solid-state reaction method. All measurements indicate the effect of aging temperature on ceramic properties is related to the grain size and the degree of diffusion.

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Data can be available from the corresponding author upon academic reasonable request.

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Acknowledgements

This work has been financially supported by the National Natural Science Foundation of China (Nos. 51402091,61901161), the Scientific Research Project in Henan Normal University (No. 20210376), Key Scientific Research Projects of Colleges and Universities in Henan Province (21A140014), and Young Backbone Teachers Training Plan of Colleges and Universities in Henan Province (2020GGJS060).

Funding

This article was funded by National Natural Science Foundation of China, Nos. 51402091, Shaoqian Yin,61901161,Shaoqian Yin, the Scientific Research Project in Henan Normal University, No. 20210376,Xianwei Wang, Key Scientific Research Projects of Colleges and Universities in Henan Province,21A140014,Yanchun Hu, Young Backbone Teachers Training Plan of Colleges and Universities in Henan Province,2020GGJS060,Yanchun Hu.

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Author notes

  1. S. T. Dang, L. L. Xue, L. F. He, Y. C. Shi have contributed equally to this work.

Authors and Affiliations

  1. National Demonstration Center for Experimental Physics Education, School of Physics, Henan Normal University, and Henan Key Laboratory of Photovoltaic Materials, Xinxiang, 453007, People’s Republic of China

    S. T. Dang, L. L. Xue, L. F. He, Y. C. Shi, H. N. Li, Y. C. Hu, J. Shang, S. Q. Yin & X. W. Wang

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  1. S. T. Dang
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  2. L. L. Xue
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  3. L. F. He
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  4. Y. C. Shi
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  5. H. N. Li
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  6. Y. C. Hu
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Contributions

All authors contributed to the study. Resources, funding acquisition and project administration are provided by Xianwei Wang, Yanchun Hu, Jun Shang and Shaoqin Yin. Material preparation was performed by Lulu Xue and Lifang He. Data collection and analysis were completed by Santan Dang, Yongchuang Shi, and Haonan Li. The first draft of the manuscript was written by Santan Dang and Lulu Xue. Review and Editing was completed by Xianwei Wang and Yanchun Hu. All authors commented on previous versions of the manuscript and read and approved the final manuscript.

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Correspondence to Y. C. Hu or X. W. Wang.

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Dang, S.T., Xue, L.L., He, L.F. et al. Dielectric and energy storage properties of Ba0.85Ca0.15Zr0.1Ti0.9O3 ceramics with different aging temperature during the sol–gel process. J Mater Sci: Mater Electron 33, 26100–26112 (2022). https://doi.org/10.1007/s10854-022-09297-0

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