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Simultaneously achievement of high recoverable energy density and efficiency in sodium niobate-based ceramics

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Abstract

Single lead-free Na0.73Bi0.09(Nb1 − xTax)O3 (x = 0, 0.10, 0.20, 0.30, and 0.40) ceramic phases were processed via a solid-state sintering route. The phase, microstructure, dielectric, and energy storage properties of the sintered ceramics were investigated. A high εr > 1000, a recoverable energy storage density (Wrec) ~ 0.92 J/cm3 along with ultra-high efficiency of 96.33% at 127 kV was obtained for x = 0 composition at room temperature. At x = 0.10, the value of Wrec increased to ~ 1.13 J/cm3 while the efficiency slightly decreased to ~ 95.7%. Furthermore, the discharging time of x = 0.10 composition was ~ 0.12 µs. These characteristics make the x = 0.10 composition a suitable candidate material for pulsed power applications.

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Data sharing not applicable to this article as no datasets were generated or analyzed during the current study.

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Funding

The financial support of the Higher Education Commission (HEC) Islamabad, Pakistan through the Local Challenge Fund (20-LCF-5/RGM/RF&D/HEC/2020) and National Research Program for Universities (7488/KPK/NRPU/R&D/HEC/2017) for this work is highly acknowledged.

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Authors and Affiliations

  1. Laboratory for Research in Advanced Materials, Department of Physics, University of Science & Technology, Bannu, 28100, Khyber Pakhtunkhwa, Pakistan

    Abdul Manan, Maqbool Ur Rehman & Murad Ali Khan

  2. Department of Chemsirty, Government Postgraduate College Bannu, University of Science & Technology, Bannu, 28100, Khyber Pakhtunkhwa, Pakistan

    Shah Faisal

  3. Center for Materials Science, Islamia College Peshawar, Peshawar, 25120, Khyber Pakhtunkhwa, Pakistan

    Atta Ullah, Arbab Safeer Ahmad & Muhammad Amer Khan

  4. National Center of Excelence in Physical Chemistry, University of Peshawar, Peshawar, 25120, Khyber Pakhtunkhwa, Pakistan

    Zahid Ali Ghazi

  5. Department of Physics, College of Science, Qassim University, Buraidah, Saudi Arabia

    Faisal Alresheedi

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  1. Abdul Manan
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  2. Maqbool Ur Rehman
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  4. Atta Ullah
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  9. Muhammad Amer Khan
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Contributions

AM: Writing—Original draft preparation, MUR: Dielectric properties Interpretation SF: P–E loop data analysis, AU: Sample preparations, ZAG: Sample preparation for XRD, ASA: Energy density calculation,, MAK: Sample preparation for SEM, FA: Dielectric data analysis.

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Correspondence to Abdul Manan.

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Manan, A., Rehman, M.U., Faisal, S. et al. Simultaneously achievement of high recoverable energy density and efficiency in sodium niobate-based ceramics. J Mater Sci: Mater Electron 33, 22208–22216 (2022). https://doi.org/10.1007/s10854-022-09000-3

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  • DOI: https://doi.org/10.1007/s10854-022-09000-3

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