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Ba(Zr0.3Ti0.7)O3 doping to enhance the dielectric and energy discharging performances of a 0.65Bi0.5Na0.5TiO3–0.35Sr0.7Bi0.2TiO3 lead-free ceramic

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Abstract

A group of lead-free (1 − x)(0.65Bi0.5Na0.5TiO3–0.35Sr0.7Bi0.2TiO3)–x[Ba(Zr0.3Ti0.7) O3] [(1 − x)BNT–SBT–xBZT] ternary ceramics is prepared through the traditional solid-phase sintering reaction. The introduction of relaxor dielectric ceramic Ba (Zr0.3Ti0.7)O3 (BZT) can reduce the grain size, form a typical “ferroelectric + relaxor ferroelectric” lead-free system, and refine the hysteresis loops and improve η through site doping. As such, the dielectric anomaly peaks gradually shift to lower temperature and show a diffusion phase transition behavior over a wide temperature range, resulting in an active relaxation with the increase of doping BZT. Remarkably, the high energy density performance (Wrec and η are 1.00 J cm−3 and 87%, respectively) is obtained in this 0.86BNT-SBT-0.14BZT ceramic at relatively low electric field of 80 kV cm−1. This work is an appropriate reference to promote the energy storage performance of BNT-based ceramics by introducing BZT, providing an approach for lead-free dielectric materials.

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References

  1. G. Wang, Z.L. Lu, Y. Li, L.H. Li, H.F. Ji, A. Feteira, D. Zhou, D.W. Wang, S.J. Zhang, I.M. Reaney, Chem. Rev. 121, 6124 (2021)

    Article  CAS  Google Scholar 

  2. J.L. Li, Z.H. Shen, X.H. Chen, S. Yang, W.L. Zhou, M.W. Wang, L.H. Wang, Q.W. Kou, Y.C. Liu, Q. Li, Z. Xu, Y.F. Chang, S.J. Zhang, F. Li, Nat. Mater. 19, 9 (2020)

    Article  CAS  Google Scholar 

  3. N.N. Luo, K. Han, M.J. Cabral, X.Z. Liao, S.J. Zhang, C.Z. Liao, G.Z. Zhang, X.Y. Chen, Q. Feng, J.F. Li, Y.Z. Wei, Nat. Commun. 11, 4824 (2020)

    Article  CAS  Google Scholar 

  4. L.T. Yang, X. Kong, F. Li, H. Hao, Z.X. Cheng, H.X. Liu, J.-F. Li, S.J. Zhang, Prog. Mater. Sci. 102, 72 (2019)

    Article  CAS  Google Scholar 

  5. H. Palneedi, M. Peddigari, G.T. Hwang, D.Y. Jeong, J. Ryu, Adv. Funct. Mater. 28, 1803665 (2018)

    Article  CAS  Google Scholar 

  6. H.T. Wang, J.H. Liu, J.W. Zhai, B. Shen, J. Am. Ceram. Soc. 99, 2909 (2016)

    Article  CAS  Google Scholar 

  7. Z.T. Yang, H.L. Du, S.B. Qu, Y.D. Hou, H. Ma, J.F. Wang, J. Wang, X.Y. Wei, Z. Xu, J. Mater. Chem. C 4, 13778 (2016)

    CAS  Google Scholar 

  8. H.B. Zhang, T. Wei, Q. Zhang, W.G. Ma, P.Y.D. Salamon, S.T. Zhang, B. Nan, H. Tan, Z.G. Ye, J. Mater. Chem. C 8, 16648 (2021)

    Article  Google Scholar 

  9. T. Wei, K. Liu, P.Y. Fan, D.J. Lu, B.H. Ye, C.R. Zhou, H.B. Yang, H. Tan, D. Salamon, B. Nan, H.B. Zhang, Ceram. Int. 47, 3713 (2021)

    Article  CAS  Google Scholar 

  10. G.Z. Zhang, D.Y. Zhu, X.S. Zhang, L. Zhang, J.Q. Yi, B. Xie, Y.K. Zeng, Q. Li, Q. Wang, S.L. Jiang, J. Am. Ceram. Soc. 98, 1175 (2015)

    Article  CAS  Google Scholar 

  11. Q. Xu, J. Xie, Z.C. He, L. Zhang, M.H. Cao, X.D.M.T. Huang,Lanagan, H. Hao, Z.H. Yao, H.X. Liu, J. Eur. Ceram. Soc. 37, 99 (2017)

    Article  CAS  Google Scholar 

  12. Y.P. Pu, M.T. Yao, L. Zhang, P.P. Jing, J. Alloys Compd. 687, 689 (2016)

    Article  CAS  Google Scholar 

  13. X.M. Fan, P. Li, J.A. Du, C. Chen, P. Fu, J.G. Hao, Z.X. Yue, W. Li, J. Mater. Sci. 31, 9974 (2020)

    CAS  Google Scholar 

  14. J. Suchanicz, K. Kluczewska-Chmielarz, D. Sitko, G. Jaglo, J. Adv. Ceram. 10, 152 (2021)

    Article  CAS  Google Scholar 

  15. G.A. Smolenskii, V.A. Isupov, A.I. Agranovskaya, N.N. Krainik, Phys. Solid State 2, 2651 (1961)

    Google Scholar 

  16. Y.P. Pu, L. Zhang, Y.F. Cui, M. Chen, ACS Sustain. Chem. Eng. 6, 6102 (2018)

    Article  CAS  Google Scholar 

  17. M.K. Zhu, H.C. Hu, N. Lei, Y.D. Hou, H. Yan, Appl. Phys. Lett. 94, 182901 (2009)

    Article  CAS  Google Scholar 

  18. Q. Xu, H.X. Liu, L. Zhang, J. Xie, H. Hao, M.H. Cao, Z.H. Yao, M.T. Lanagan, RSC Adv. 6, 59280 (2016)

    Article  CAS  Google Scholar 

  19. Q. Xu, M. Chen, W. Chen, H.X. Liu, B.H. Kim, B.K. Ahn, Acta Mater. 56, 642 (2008)

    Article  CAS  Google Scholar 

  20. Q. Xu, T.M. Li, H. Hao, S.J. Zhang, Z.J. Wang, M.H. Cao, Z.H. Yao, H.X. Liu, J. Eur. Ceram. Soc. 35, 545 (2015)

    Article  CAS  Google Scholar 

  21. H.B. Yang, P.F. Liu, F. Yan, Y. Lin, T. Wang, J. Alloys Compd. 773, 244 (2018)

    Article  CAS  Google Scholar 

  22. Y. Lin, D. Li, M. Zhang, H.B. Yang, J. Mater. Chem. C 8, 2258 (2020)

    Article  CAS  Google Scholar 

  23. W.G. Ma, Y.W. Zhu, M.A. Marwat, P.Y. Fan, B. Xie, D. Salamon, Z.G. Ye, H.B. Zhang, J. Mater. Chem. C 7, 281 (2019)

    Article  CAS  Google Scholar 

  24. X.F. Zhou, H. Qi, Z.N. Yan, G.L. Xue, H. Luo, D. Zhang, ACS Appl. Mater. Inter 11, 43107 (2019)

    Article  CAS  Google Scholar 

  25. P. Butnoi, S. Manotham, P. Jaita, C. Randorn, G. Rujijanagul, J. Eur. Ceram. Soc. 3, 3822 (2018)

    Article  CAS  Google Scholar 

  26. F. Li, K. Yang, X. Liu, J. Zou, J.W. Zhai, B. Shen, P. Li, J. Shen, B.H. Liu, P. Chen, K.Y. Zhao, H.R. Zeng, Scr. Mater. 141, 15 (2017)

    Article  CAS  Google Scholar 

  27. J.L. Li, F. Li, Z. Xu, S.J. Zhang, Adv. Mater. 30, 1802155 (2018)

    Article  CAS  Google Scholar 

  28. K.Y. Wu, H. Wang, Z. Miao, S.X. Ding, Y.X. Qi, Y. Ming, W.J. Ding, H. Yuan, Q.J. Zheng, D.M. Lin, Ceram. Int. 46, 13159 (2020)

    Article  CAS  Google Scholar 

  29. J.U. Rahman, A. Hussain, A. Maqbool, G.H. Ryu, T.K. Song, W.J. Kim, M.H. Kim, J. Alloys Compd. 593, 97 (2014)

    Article  CAS  Google Scholar 

  30. F. Li, X. Hou, J. Wang, H.R. Zeng, B. Shen, J.W. Zhai, J. Eur. Ceram. Soc. 39, 2889 (2019)

    Article  CAS  Google Scholar 

  31. P. Zhao, B. Tang, F. Si, C.T. Yang, H. Li, S.R. Zhang, J. Eur. Ceram. Soc. 40, 1938 (2020)

    Article  CAS  Google Scholar 

  32. X.S. Qiao, F.D. Zhang, D. Wu, B. Chen, X.M. Zhao, Z.H. Peng, X.D. Ren, P.F. Liang, X.L. Chao, Z.P. Yang, Chem. Eng. J. 388, 124158 (2020)

    Article  CAS  Google Scholar 

  33. N.S. Zhao, H.Q. Fan, L. Ning, J.W. Ma, Y.Y. Zhou, J. Am. Ceram. Soc. 101, 5578 (2018)

    Article  CAS  Google Scholar 

  34. E. Birks, M. Dunce, R. Ignatans, A. Kuzmin, A. Plaude, M. Antonova, K. Kundzins, A. Sternberg, J. Appl. Phys. 119, 074102 (2016)

    Article  CAS  Google Scholar 

  35. W. Jo, S. Schaab, E. Sapper, L.A. Schmitt, H.-J. Kleebe, A.J. Bell, J. Rodel, J. Appl. Phys. 110, 074106 (2011)

    Article  CAS  Google Scholar 

  36. H. Qi, R.Z. Zuo, J. Mater. Chem. A 7, 3971 (2019)

    Article  CAS  Google Scholar 

  37. Y.F. Wang, Z.L. Lv, H. Xie, J. Cao, Ceram. Int. 40, 4323 (2014)

    Article  CAS  Google Scholar 

  38. T. Wang, L. Jin, C.C. Li, Q.Y. Hu, X.Y. Wei, J. Am. Ceram. Soc. 98, 559 (2015)

    Article  CAS  Google Scholar 

  39. W.P. Cao, W.L. Li, X.F. Dai, T.D. Zhang, J. Sheng, Y.F. Hou, W.D. Fei, J. Eur. Ceram. Soc. 36, 593 (2016)

    Article  CAS  Google Scholar 

  40. Q.N. Li, C.R. Zhou, J.W. Xu, L. Yang, X. Zhang, W.D. Zeng, C.L. Yuan, G.H. Chen, G.H. Rao, J. Electron. Mater. 45, 5146 (2016)

    Article  CAS  Google Scholar 

  41. G.Z. Dong, H.Q. Fan, Y.X. Jia, H. Liu, J. Mater. Sci. Mater. Electron. 31, 13620 (2020)

    Article  CAS  Google Scholar 

  42. M. Chandrasekhar, P. Sonia, Kumar, Phys. B 497, 59 (2016)

    Article  CAS  Google Scholar 

  43. Z.L. Yu, L.F. Liu, M.Y. Shen, H. Qian, F.F. Li, Y.N. Lyu, Ceram. Int. 43, 7653 (2017)

    Article  CAS  Google Scholar 

  44. F. Yan, H.B. Yang, Y. Lin, T. Wang, Inorg. Chem. 56, 13510 (2017)

    Article  CAS  Google Scholar 

  45. S.J. Pang, L. Yang, J.Y. Qin, H. Qin, H. Xie, H. Wang, C.R. Zhou, J.W. Xu, Appl. Phys. A 125, 119 (2019)

    Article  CAS  Google Scholar 

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Acknowledgments

This work was supported in part by National Natural Science Foundation of China (NSFC 51773168 and 92066204), NSFC of Shaanxi province (2020JM-465), and by the Shaanxi project of Education Department (21JY031).

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The authors declare that no funds, grants, or other support were received during the preparation of this manuscript.

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Authors and Affiliations

  1. College of Printing, Packaging, and Digital Media Technology, Xi’an University of Technology, Xi’an, 710054, Shaanxi, China

    Mengjie Zhao, Weimin Xia, Yannan Liang, Danfeng Lu & Yan Feng

  2. College of Material Science and Engineering, Xi’an University of Technology, Xi’an, 710048, Shaanxi, China

    Weimin Xia & Xiaofang Zhang

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  1. Mengjie Zhao
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Contributions

Material preparation, data collection and analysis were performed by MZ and YL. The study conception and design were performed by WX,YF and XZ. The first draft of the manuscript was written by MZ and DL. And all authors commented on previous version of the manuscript. All authors read and approved the final manuscript.

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Correspondence to Weimin Xia.

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Zhao, M., Xia, W., Liang, Y. et al. Ba(Zr0.3Ti0.7)O3 doping to enhance the dielectric and energy discharging performances of a 0.65Bi0.5Na0.5TiO3–0.35Sr0.7Bi0.2TiO3 lead-free ceramic. J Mater Sci: Mater Electron 33, 21702–21712 (2022). https://doi.org/10.1007/s10854-022-08958-4

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