Skip to main content
Log in

Performance of inkjet-printed strain sensor based on graphene/silver nanoparticles hybrid conductive inks on polyvinyl alcohol substrate

  • Published:
Journal of Materials Science: Materials in Electronics Aims and scope Submit manuscript

Abstract

Recently, there have been considerable interests in strain sensors that are flexible and stretchable, due to their potential for use in wearable electronics applications. Herein, a facile approach has been employed to produce synergistic strain sensor, taking advantage of the salient properties of hybrid conductive inks produced from graphene and silver nanoparticles (AgNPs). The hybrid ink was inkjet-printed on a polyvinyl alcohol (PVA) substrate. The effect of factors such as amount of graphene, annealing time and printing cycle on the performance of the hybrid conductive ink was investigated. The results showed that an increase in the amount of graphene from 0.1 to 0.5 wt% produced about 90% enhancement in the electrical conductivity of the hybrid ink. However, the change in electrical conductivity values of the hybrid ink at 0.5 wt% and 0.7 wt% graphene content is negligible. On the other hand, it was observed that the electrical conductivity was notably influenced by the number of printing cycle, as well as the annealing time. Significantly, the sensitivity performance of the printed hybrid graphene/AgNPs strain sensor is higher than that of individual graphene and AgNPs printed strain sensors under the strain range up to 20%.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8
Fig. 9
Fig. 10
Fig. 11

Similar content being viewed by others

References

  1. J. Wang, W. Zhang, Q. Yin, B. Yin, H. Jia, Highly sensitive and flexible strain sensors based on natural rubber/graphene foam composites: the role of pore sizes of graphene foam. J. Mater. Sci.: Mater. Electron. 31(1), 125–133 (2020)

    CAS  Google Scholar 

  2. X.M. Zhang, X.L. Yang, K.Y. Wang, Conductive graphene/polydimethylsiloxane nanocomposites for flexible strain sensors. J. Mater. Sci.: Mater. Electron. 30(21), 19319–19324 (2019)

    CAS  Google Scholar 

  3. C. Deng, L. Pan, R. Cui, C. Li, J. Qin, Wearable strain sensor made of carbonized cotton cloth. J. Mater. Sci.: Mater. Electron. 28(4), 3535–3541 (2017)

    CAS  Google Scholar 

  4. A.M. Gaikwad, D.A. Steingart, T.N. Nga, D.E. Schwartz, G.L. Whiting, A flexible high potential printed battery for powering printed electronics . Appl Phys. Lett. 102(23), 104–101 (2013)

    Google Scholar 

  5. S.H. Eom, S. Lim, RF stretchable sensor using flexible substrate and eutectic gallium-indium. In Proceedings of the Antennas and Propagation (ISAP), International Symposium on IEEE, pp. 996–997 (2016)

  6. H. Dai, E.T. Thostenson, T. Schumacher, Processing and characterization of a novel distributed strain sensor using carbon nanotube-based nonwoven composite. Sensors 15(7), 17728–17747 (2015)

    Google Scholar 

  7. K. Karimi, E. Jabari, E. Toyserkani, P. Lee-Sullivan, Highly conductive graphene paper for flexible electronics applications. J. Mater. Sci.: Mater. Electron. 29(3), 2537–2549 (2018)

    CAS  Google Scholar 

  8. M. Goosey, A short introduction to graphene and its potential interconnect applications. Circuit World 38(2), 83–86 (2012)

    CAS  Google Scholar 

  9. Z. Zhong, X. Gong, L. Wang, G. Bai, H. Wei, W. Yang, A facile way for fabrication of silver nanoparticle decorated graphene composites. Mater. Chem. Phys. 241, 122344 (2020)

    CAS  Google Scholar 

  10. D. Deng, S. Feng, M. Shi, C. Huang, In situ preparation of silver nanoparticles decorated graphene conductive ink for inkjet printing. J. Mater. Sci.: Mater. Electron. 28(20), 15411–15417 (2017)

    CAS  Google Scholar 

  11. F. Miao, S. Majee, M. Song, J. Zhao, S.L. Zhang, S. L, Z.B. Zhang, Inkjet printing of electrochemically-exfoliated graphene nano-platelets. Synth. Met. 220, 318–322 (2016)

    CAS  Google Scholar 

  12. T.S. Tran, N.K. Dutta, C.N. R, Graphene inks for printed flexible electronics: Graphene dispersions, ink formulations, printing techniques and applications. Adv Colloid Interfac 261, 41–61 (2018)

    CAS  Google Scholar 

  13. M.R. Ammar, G. Legeay, A. Bulou, J.F. Bardeau, Physical and chemical treatments of surface for improved adhesion of PVA Coating. In Proceedings of the Le Congrès National de la Recherche des IUT, pp. 1–6 (2008)

  14. Y. Wan, Y. Wang, C.F. Guo, Recent progresses on flexible tactile sensors. Mater. Today Phy. 1, 61–73 (2017)

    Google Scholar 

  15. Y.Z.N. Htwe, W.S. Chow, Y. Suda, A.A. Thant, M. Mariatti, Effect of electrolytes and sonication times on the formation of graphene using an electrochemical exfoliation process. Appl. Surf. Sci. 469, 951–961 (2019)

    CAS  Google Scholar 

  16. Y.Z.N. Htwe, W.S. Chow, Y. Suda, A.A. Thant, M. Mariatti, Properties enhancement of graphene and chemical reduction silver nanoparticles conductive inks printed on polyvinyl alcohol (PVA) substrate. Synth. Met. 256, 116–120 (2019)

    Google Scholar 

  17. W. Zhang, E. Bi, M. Li, L. Gao, Synthesis of Ag/RGO composite as effective conductive ink filler for flexible inkjet printing electronics. Colloids Surf. A 490, 232–240 (2016)

    CAS  Google Scholar 

  18. A. Kamyshny, J. Steinke, S. Magdassi, Metal-based inkjet inks for printed electronics. J. Appl. Phys. 4(1), 19–36 (2011)

    CAS  Google Scholar 

  19. D.S. Saidina, S.A. Zubir, S. Fontana, C. Hérold, M. Mariatti, Synthesis and characterization of graphene-based inks for spray-coating applications. J. Electron. Mater. 48, 5757–5770 (2019)

    CAS  Google Scholar 

  20. A. Denneulin, J. Bras, A. Blayo, B. Khelifi, F. Roussel-Dherbey, C. Neuman, The influence of carbon nanotubes in inkjet printing of conductive polymer suspensions. Nanotechnology 20(38), 385–701 (2009)

    Google Scholar 

  21. G. Suriati, M. Mariatti, A. Azizan, A effects of filler shape and size on the properties of silver filled epoxy composite for electronic applications. J. Mater. Sci.: Mater. Electron. 22(1), 56–63 (2009)

    Google Scholar 

  22. A.J. Marsden, D.G. Papageorgiou, C. Vallés, A. Liscio, V. Palermo, M.A. Bissett, I.A. Kinloch, Electrical percolation in graphene–polymer composites. 2D Mater. 5(3), 032003 (2018)

    Google Scholar 

  23. Y. Gao, W. Shi, W. Wang, Y. Leng, Y. Zhao, Inkjet printing patterns of highly conductive pristine graphene on flexible substrates. Ind. Eng. Chem. Res. 53(43), 16777–16784 (2014)

    CAS  Google Scholar 

  24. J. Li, X. Zhang, X. Liu, Q. Liang, G. Liao, Z. Tang, T. Shi, Conductivity and foldability enhancement of Ag patterns formed by PVAc modified Ag complex inks with low-temperature and rapid sintering. Mater. Des. 185, 108255 (2020)

    CAS  Google Scholar 

  25. N. Karim, S. Afroj, S. Tan, K.S. Novoselov, S.G. Yeates, All inkjet-printed graphene-silver composite ink on textiles for highly conductive wearable electronics applications. Sci. Rep. 9(1), 1–10 (2019)

    Google Scholar 

  26. S. Shengbo, L. Lihua, J. Aoqun, D. Qianqian, J. Jianlong, Z. Qiang, Z. Wendong, Highly sensitive wearable strain sensor based on silver nanowires and nanoparticles. Nanotechnology 29(25), 255–202 (2018)

    Google Scholar 

  27. H. Lee, B. Seong, H. Moon, D. Byun, Directly printed stretchable strain sensor based on ring and diamond shaped silver nanowire electrodes. RSC Adv. 5(36), 28379–28384 (2015)

    CAS  Google Scholar 

  28. S. Chun, Y. Choi, W. Park, All-graphene strain sensor on soft substrate. Carbon 116, 753–759 (2017)

    CAS  Google Scholar 

  29. M. Amjadi, A. Pichitpajongkit, S. Lee, S. Ryu, S.I. Park, Highly stretchable and sensitive strain sensor based on silver nanowire–elastomer nanocomposite. ACS Nano 8(5), 5154–5163 (2014)

    CAS  Google Scholar 

  30. Y. Liu, D. Zhang, K. Wang, Y. Liu, Y. Shang, A novel strain sensor based on graphene composite films with layered structure. Compos. Part A Appl. Sci. Manuf. 80, 95–103 (2016)

    CAS  Google Scholar 

  31. S. Zhang, H. Zhang, G. Yao, F. Liao, M. Gao, Z. Huang, Y. Lin, Highly stretchable, sensitive, and flexible strain sensors based on silver nanoparticles/carbon nanotubes composites. J. Alloys Compd. 652, 48–54 (2015)

    CAS  Google Scholar 

Download references

Acknowledgements

This study was supported by ASEAN University Network for Science and Engineering Education Development Network (AUN/SEED-Net) Project. Similarly, the authors appreciate the support from Japan International Cooperation Agency (JICA). In addition, the authors appreciate the Malaysian Ministry of Education for the grant provided (FRGS MRSA Grant No. 6071385). Furthermore, the first author would like to thank Universiti Sains Malaysia for the USM fellowship scheme.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to M. Mariatti.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Htwe, Y.Z.N., Hidayah, I.N. & Mariatti, M. Performance of inkjet-printed strain sensor based on graphene/silver nanoparticles hybrid conductive inks on polyvinyl alcohol substrate. J Mater Sci: Mater Electron 31, 15361–15371 (2020). https://doi.org/10.1007/s10854-020-04100-4

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10854-020-04100-4

Navigation