Abstract
Recently, there have been considerable interests in strain sensors that are flexible and stretchable, due to their potential for use in wearable electronics applications. Herein, a facile approach has been employed to produce synergistic strain sensor, taking advantage of the salient properties of hybrid conductive inks produced from graphene and silver nanoparticles (AgNPs). The hybrid ink was inkjet-printed on a polyvinyl alcohol (PVA) substrate. The effect of factors such as amount of graphene, annealing time and printing cycle on the performance of the hybrid conductive ink was investigated. The results showed that an increase in the amount of graphene from 0.1 to 0.5 wt% produced about 90% enhancement in the electrical conductivity of the hybrid ink. However, the change in electrical conductivity values of the hybrid ink at 0.5 wt% and 0.7 wt% graphene content is negligible. On the other hand, it was observed that the electrical conductivity was notably influenced by the number of printing cycle, as well as the annealing time. Significantly, the sensitivity performance of the printed hybrid graphene/AgNPs strain sensor is higher than that of individual graphene and AgNPs printed strain sensors under the strain range up to 20%.
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References
J. Wang, W. Zhang, Q. Yin, B. Yin, H. Jia, Highly sensitive and flexible strain sensors based on natural rubber/graphene foam composites: the role of pore sizes of graphene foam. J. Mater. Sci.: Mater. Electron. 31(1), 125–133 (2020)
X.M. Zhang, X.L. Yang, K.Y. Wang, Conductive graphene/polydimethylsiloxane nanocomposites for flexible strain sensors. J. Mater. Sci.: Mater. Electron. 30(21), 19319–19324 (2019)
C. Deng, L. Pan, R. Cui, C. Li, J. Qin, Wearable strain sensor made of carbonized cotton cloth. J. Mater. Sci.: Mater. Electron. 28(4), 3535–3541 (2017)
A.M. Gaikwad, D.A. Steingart, T.N. Nga, D.E. Schwartz, G.L. Whiting, A flexible high potential printed battery for powering printed electronics . Appl Phys. Lett. 102(23), 104–101 (2013)
S.H. Eom, S. Lim, RF stretchable sensor using flexible substrate and eutectic gallium-indium. In Proceedings of the Antennas and Propagation (ISAP), International Symposium on IEEE, pp. 996–997 (2016)
H. Dai, E.T. Thostenson, T. Schumacher, Processing and characterization of a novel distributed strain sensor using carbon nanotube-based nonwoven composite. Sensors 15(7), 17728–17747 (2015)
K. Karimi, E. Jabari, E. Toyserkani, P. Lee-Sullivan, Highly conductive graphene paper for flexible electronics applications. J. Mater. Sci.: Mater. Electron. 29(3), 2537–2549 (2018)
M. Goosey, A short introduction to graphene and its potential interconnect applications. Circuit World 38(2), 83–86 (2012)
Z. Zhong, X. Gong, L. Wang, G. Bai, H. Wei, W. Yang, A facile way for fabrication of silver nanoparticle decorated graphene composites. Mater. Chem. Phys. 241, 122344 (2020)
D. Deng, S. Feng, M. Shi, C. Huang, In situ preparation of silver nanoparticles decorated graphene conductive ink for inkjet printing. J. Mater. Sci.: Mater. Electron. 28(20), 15411–15417 (2017)
F. Miao, S. Majee, M. Song, J. Zhao, S.L. Zhang, S. L, Z.B. Zhang, Inkjet printing of electrochemically-exfoliated graphene nano-platelets. Synth. Met. 220, 318–322 (2016)
T.S. Tran, N.K. Dutta, C.N. R, Graphene inks for printed flexible electronics: Graphene dispersions, ink formulations, printing techniques and applications. Adv Colloid Interfac 261, 41–61 (2018)
M.R. Ammar, G. Legeay, A. Bulou, J.F. Bardeau, Physical and chemical treatments of surface for improved adhesion of PVA Coating. In Proceedings of the Le Congrès National de la Recherche des IUT, pp. 1–6 (2008)
Y. Wan, Y. Wang, C.F. Guo, Recent progresses on flexible tactile sensors. Mater. Today Phy. 1, 61–73 (2017)
Y.Z.N. Htwe, W.S. Chow, Y. Suda, A.A. Thant, M. Mariatti, Effect of electrolytes and sonication times on the formation of graphene using an electrochemical exfoliation process. Appl. Surf. Sci. 469, 951–961 (2019)
Y.Z.N. Htwe, W.S. Chow, Y. Suda, A.A. Thant, M. Mariatti, Properties enhancement of graphene and chemical reduction silver nanoparticles conductive inks printed on polyvinyl alcohol (PVA) substrate. Synth. Met. 256, 116–120 (2019)
W. Zhang, E. Bi, M. Li, L. Gao, Synthesis of Ag/RGO composite as effective conductive ink filler for flexible inkjet printing electronics. Colloids Surf. A 490, 232–240 (2016)
A. Kamyshny, J. Steinke, S. Magdassi, Metal-based inkjet inks for printed electronics. J. Appl. Phys. 4(1), 19–36 (2011)
D.S. Saidina, S.A. Zubir, S. Fontana, C. Hérold, M. Mariatti, Synthesis and characterization of graphene-based inks for spray-coating applications. J. Electron. Mater. 48, 5757–5770 (2019)
A. Denneulin, J. Bras, A. Blayo, B. Khelifi, F. Roussel-Dherbey, C. Neuman, The influence of carbon nanotubes in inkjet printing of conductive polymer suspensions. Nanotechnology 20(38), 385–701 (2009)
G. Suriati, M. Mariatti, A. Azizan, A effects of filler shape and size on the properties of silver filled epoxy composite for electronic applications. J. Mater. Sci.: Mater. Electron. 22(1), 56–63 (2009)
A.J. Marsden, D.G. Papageorgiou, C. Vallés, A. Liscio, V. Palermo, M.A. Bissett, I.A. Kinloch, Electrical percolation in graphene–polymer composites. 2D Mater. 5(3), 032003 (2018)
Y. Gao, W. Shi, W. Wang, Y. Leng, Y. Zhao, Inkjet printing patterns of highly conductive pristine graphene on flexible substrates. Ind. Eng. Chem. Res. 53(43), 16777–16784 (2014)
J. Li, X. Zhang, X. Liu, Q. Liang, G. Liao, Z. Tang, T. Shi, Conductivity and foldability enhancement of Ag patterns formed by PVAc modified Ag complex inks with low-temperature and rapid sintering. Mater. Des. 185, 108255 (2020)
N. Karim, S. Afroj, S. Tan, K.S. Novoselov, S.G. Yeates, All inkjet-printed graphene-silver composite ink on textiles for highly conductive wearable electronics applications. Sci. Rep. 9(1), 1–10 (2019)
S. Shengbo, L. Lihua, J. Aoqun, D. Qianqian, J. Jianlong, Z. Qiang, Z. Wendong, Highly sensitive wearable strain sensor based on silver nanowires and nanoparticles. Nanotechnology 29(25), 255–202 (2018)
H. Lee, B. Seong, H. Moon, D. Byun, Directly printed stretchable strain sensor based on ring and diamond shaped silver nanowire electrodes. RSC Adv. 5(36), 28379–28384 (2015)
S. Chun, Y. Choi, W. Park, All-graphene strain sensor on soft substrate. Carbon 116, 753–759 (2017)
M. Amjadi, A. Pichitpajongkit, S. Lee, S. Ryu, S.I. Park, Highly stretchable and sensitive strain sensor based on silver nanowire–elastomer nanocomposite. ACS Nano 8(5), 5154–5163 (2014)
Y. Liu, D. Zhang, K. Wang, Y. Liu, Y. Shang, A novel strain sensor based on graphene composite films with layered structure. Compos. Part A Appl. Sci. Manuf. 80, 95–103 (2016)
S. Zhang, H. Zhang, G. Yao, F. Liao, M. Gao, Z. Huang, Y. Lin, Highly stretchable, sensitive, and flexible strain sensors based on silver nanoparticles/carbon nanotubes composites. J. Alloys Compd. 652, 48–54 (2015)
Acknowledgements
This study was supported by ASEAN University Network for Science and Engineering Education Development Network (AUN/SEED-Net) Project. Similarly, the authors appreciate the support from Japan International Cooperation Agency (JICA). In addition, the authors appreciate the Malaysian Ministry of Education for the grant provided (FRGS MRSA Grant No. 6071385). Furthermore, the first author would like to thank Universiti Sains Malaysia for the USM fellowship scheme.
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Htwe, Y.Z.N., Hidayah, I.N. & Mariatti, M. Performance of inkjet-printed strain sensor based on graphene/silver nanoparticles hybrid conductive inks on polyvinyl alcohol substrate. J Mater Sci: Mater Electron 31, 15361–15371 (2020). https://doi.org/10.1007/s10854-020-04100-4
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DOI: https://doi.org/10.1007/s10854-020-04100-4