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Generation of disinfection by-products (DBPs) at two advanced water treatment plants

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Abstract

A sampling program was conducted to investigate the formation of disinfection by-products (DBPs) and dissolved organic carbon (DOC) at two advanced water treatment plants in Kaohsiung City, Taiwan. The results in this study can be used as a reference for the operational control of water treatment plants and the setting of regulations in Taiwan. Samples of drinking water were collected from two advanced water treatment plants from June 2007 to April 2008. Changes in the concentration of dissolved organic carbon, the trihalomethane formation potential, and the haloacetic acids formation potential were measured in raw water samples. Variations in the concentrations of trihalomethanes (THMs) and haloacetic acids (HAA5) in finished drinking water were evaluated. The major species of HAA5 were in the order of dichloroacetic acid and trichloroacetic acid and the THM was of trichloromethane. DOC was strongly related to DBPs in raw water. In this investigation, the removal efficiency of DBPs in Plant A (ultrafiltration/reverse osmosis system) exceeded that in Plant B (ozonation/biological activated carbon system). Both advanced water treatment plants greatly improved the quality of drinking water.

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References

  • Arora, H., LeChevallier, M. W., & Dixon, K. L. (1997). DBP occurrence survey. Journal–American Water Works Association, 89(6), 61–68.

    Google Scholar 

  • Cedergren, M. I., Selbing, A. J., Löfman, O., & Bengt, A. J. (2002). Chlorination by products and nitrate in drinking water and risk for congenital cardiac defects. Environmental Research, 89(2), 124–130. doi:10.1006/enrs.2001.4362.

    Article  CAS  Google Scholar 

  • Chang, E. E., Lin, Y. P., & Chiang, P. C. (2001). Effects of bromide on the formation of THMs and HAAs. Chemosphere, 43(8), 1029–1034. doi:10.1016/S0045-6535(00)00210-1.

    Article  CAS  Google Scholar 

  • Cho, D. H., Kong, S. H., & Seong, G. O. (2003). Analysis of trihalomethanes in drinking water using headspace-SPME technique with gas chromatography. Water Research, 37, 402–408. doi:10.1016/S0043-1354(02)00285-3.

    Article  CAS  Google Scholar 

  • Guary, C., Rodriquez, M., & Serodes, J. (2005). Using ozonation and chloramination to reduce the formation of trihalomethanes and haloacetic acids in drinking water. Desalination, 176, 229–240. doi:10.1016/j.desal.2004.10.015.

    Article  CAS  Google Scholar 

  • Ivancev, V. T., Dalmacijam, B., Tamas, Z., & Karlovic, E. (1999). The effect of different drinking water treatment processes on the rate of chloroform formation in the reactions of natural organic matter with hypochlorite. Water Research, 33(18), 3715–3722. doi:10.1016/S0043-1354(99)00070-6.

    Article  Google Scholar 

  • Kanokkantapong, V., Marhaba, T. F., Pavasant, P., & Panyapinyophol, B. (2006). Characterization of haloacetic acid precursors in source water. Journal of Environmental Management, 80(3), 214–421. doi:10.1016/j.jenvman.2005.09.006.

    Article  CAS  Google Scholar 

  • Kim, H. C., Yu, M. J., & Han, I. (2006). Multi-method study of the characteristic chemical nature of aquatic humic substances isolated from the Han River, Korea. Applied Geochemistry, 21(7), 1226–1239. doi:10.1016/j.apgeochem.2006.03.011.

    Article  CAS  Google Scholar 

  • Lin, T. F., & Hoang, S. W. (2000). Inhalation exposure to THMs from drinking water in south Taiwan. The Science of the Total Environment, 246(1), 41–49. doi:10.1016/S0048-9697(99)00420-9.

    Article  CAS  Google Scholar 

  • Lou, J. C., & Kao, C. M. (2005). The investigation of drinking water quality in Kaohsiung City (2nd). Project Report of Taiwan Water Supply Corp.

  • Miltner, J., Shukairt, M., & Summers, R. (1992). Disinfection by-product formation and control by ozonation and biotreatment. Journal–American Water Works Association, 84(11), 53–62.

    CAS  Google Scholar 

  • NIEA W101.54A (2002). Standard methods for water quality analysis. Taiwan Environmental Protection Agency.

  • Roberts, M. G., Singer, P. C., & Obolensky, A. (2002). Comparing total HAA and total THM concentrations using ICR data. Journal–American Water Works Association, 94(1), 103–114.

    CAS  Google Scholar 

  • Servais, P., Billen, G., Bouillot, P., & Benezet, M. (1992). A pilot study of biological GAC filtration in drinking water treatment. Journal of Water Supply: Research & Technology–Aqua, 41(3), 163–168.

    CAS  Google Scholar 

  • Siddiqui, M. S., Amy, G. L., & Murphy, B. D. (1997). Ozone enhanced removal of natural organic matter from drinking water sources. Water Research, 31(12), 3098–3169. doi:10.1016/S0043-1354(97)00130-9.

    Article  CAS  Google Scholar 

  • Siverns, S. (2006). Membrane using ultrafiltration as a pre-treatment before RO. Ultrapure Water, May/June.

  • Snoeyink, V. L., Kirisits, M. J., & Pelekani, C. (1999). Adsorption of disinfection by-product precursors. In P. C. Singer (Ed.), Formation and control of disin fection by-products in drinking water (pp. 259–284). Denver: American Water Works Association.

    Google Scholar 

  • Teuschler, L. K., & Simmons, J. E. (2003). Approaching DBP toxicity as a mixtures problem. Journal–American Water Works Association, 96(6), 131–138.

    Google Scholar 

  • Tokmak, B., Capar, G., Dilek, F., & Yetis, U. (2004). Trihalomethanes and associated potential cancer risks in the water supply in Ankara, Turkey. Environmental Research, 96(3), 345–352. doi:10.1016/j.envres.2003.11.005.

    Article  CAS  Google Scholar 

  • Tung, H., Unz, R. F., & Xie, Y. F. (2006). Haloacetic acid removal by granular activated carbon adsorption. Journal–American Water Works Association, 98(6), 107–112.

    CAS  Google Scholar 

  • USEPA (2003a). National primary drinking water regulations: Stage 2 disinfectants and disinfection byproducts (D/DBP). Final rule, 68–159.

  • USEPA (2003b). Method 552.3. Determination of haloacetic acids and dalapon in drinking water by liquid-liquid microextraction, derivatization and gas chromatography with electron-capture detection., Technical Support Center, Office of Groundwater and Drinking Water. Cincinnati, Ohio, US Environmental Protection Agency.

  • Wang, G., Chang, H., & Hsieh, S. (2005). HAA formation in water treatment processes: Case study in Taiwan. In Proceedings 1st IWA-ASPIRE conference, Singapore.

  • World Health Organization (1994). Guidelines for drinking water quality. Recommendations (2nd ed., Vol. 1). WHO: Geneva.

    Google Scholar 

  • Yang, C. Y., Cheng, B. H., Tsai, S. S., Wu, T. N., Lin, M. C., & Lin, K. C. (2000). Association between chlorination of drinking water and adverse pregnancy outcome in Taiwan. Environmental Health Perspectives, 108(8), 765–768. doi:10.2307/3434730.

    Article  CAS  Google Scholar 

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Lou, JC., Huang, CE., Han, JY. et al. Generation of disinfection by-products (DBPs) at two advanced water treatment plants. Environ Monit Assess 162, 365–375 (2010). https://doi.org/10.1007/s10661-009-0802-3

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  • DOI: https://doi.org/10.1007/s10661-009-0802-3

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