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Co-immobilization of Laccase and TEMPO onto Glycidyloxypropyl Functionalized Fibrous Phosphosilicate Nanoparticles for Fixing CO2 into β-Oxopropylcarbamatesin

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Abstract

TEMPO or Anchoring 2,2,6,6-tetra-methylpiperidine-1oxyl radical into the nanospaces a fibre of phosphosilicate with laccase compound causes an unheard potent to be producing which called bifunctional nanocatalyst (TEMPO@FPS-laccase). TEMPO@FPS-laccase indicated proper catalytic activity for synthesis of β-oxopropylcarbamates in aqueous medium without any pollutants through a multi component coupling of CO2, amines and propargyl alcohols in moderate condition. Free laccases may not be recovered but can be easily disabled in different environmental conditions. Enzyme immobilization is known as an expanding way to enhance resistor to extreme conditions and stability as well as recycled of laccase.

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Acknowledgements

The study was supported by “Natural Science Foundation of Shandong Province (Grant Nos. ZR201702200464, ZR2019QB013)” and “Science and Technology Development Plan Project of Zaozhuang City (Grant No. 2019GX07)”.

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Authors and Affiliations

  1. College of Chemistry, Chemical Engineering and Materials Science, Zaozhuang University, Zaozhuang, 277160, Shandong, China

    Liqun Fan, Jinhu Wang & Xianman Zhang

  2. Young Researchers and Elite Club, Neyshabur Branch, Islamic Azad University, Neyshabur, P.O. Box 97175-613, Iran

    Seyed Mohsen Sadeghzadeh, Rahele Zhiani, Mina Shahroudi & Fatemeh Amarloo

  3. New Materials Technology and Processing Research Center, Department of Chemistry, Neyshabur Branch, Islamic Azad University, Neyshabur, Iran

    Seyed Mohsen Sadeghzadeh, Rahele Zhiani, Mina Shahroudi & Fatemeh Amarloo

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  1. Liqun Fan
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  2. Jinhu Wang
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Correspondence to Jinhu Wang or Seyed Mohsen Sadeghzadeh.

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Fan, L., Wang, J., Zhang, X. et al. Co-immobilization of Laccase and TEMPO onto Glycidyloxypropyl Functionalized Fibrous Phosphosilicate Nanoparticles for Fixing CO2 into β-Oxopropylcarbamatesin. Catal Lett 149, 3465–3475 (2019). https://doi.org/10.1007/s10562-019-02894-5

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  • DOI: https://doi.org/10.1007/s10562-019-02894-5

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