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Temperature-programmed Studies of Coke Resistant Ni Catalyst for Carbon Dioxide Reforming of Methane

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Abstract

Argon glow discharge plasma was applied for drying the impregnated Ni/SiO2 catalyst instead of the drying thermally. Such plasma treated catalyst significantly inhibits the coke formation from methane decomposition. The methane-derived carbon shows an improved reactivity against CO2. This can result in a better balance of coke formation and gasification by CO2 when the plasma-treated Ni/SiO2 catalyst is used for the CO2 reforming of methane.

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Acknowledgments

The support from the National Natural Science Foundation of China (under contract 20490203) is greatly appreciated. The instruments supplied by ABB Switzerland and the support from the Program for Changjiang Scholars and Innovative Research Team from the Ministry of Education of China are also appreciated.

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Authors and Affiliations

  1. Key Laboratory for Green Chemical Technology of Ministry of Education, School of Chemical Engineering and Technology, Tianjin University, Tianjin, 300072, P.R. China

    Yun-Xiang Pan & Chang-Jun Liu

  2. Analysis Center, Tianjin University, Tianjin, 300072, P.R. China

    Lan Cui

Authors
  1. Yun-Xiang Pan
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  2. Chang-Jun Liu
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  3. Lan Cui
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Correspondence to Chang-Jun Liu.

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Pan, YX., Liu, CJ. & Cui, L. Temperature-programmed Studies of Coke Resistant Ni Catalyst for Carbon Dioxide Reforming of Methane. Catal Lett 123, 96–101 (2008). https://doi.org/10.1007/s10562-008-9400-1

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  • DOI: https://doi.org/10.1007/s10562-008-9400-1

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