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Temperature-dependent magnetoelectric response of lead-free Na0.4K0.1Bi0.5TiO3/NiFe2O4-laminated composites

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Abstract

This study investigates the temperature-dependent quasi-static magnetoelectric (ME) response (αE) of electrically poled lead-free Na0.4K0.1Bi0.5TiO3–NiFe2O4 (NKBT–NFO)-laminated composites. The aim is to understand the temperature stability of ME-based sensors and devices. The relaxor ferroelectric nature of NKBT is confirmed through impedance and polarization–electric (PE) hysteresis loop studies, with a depolarization temperature (Td) of approximately 110 °C. Heating causes a decrease and disappearance of planar electromechanical coupling (Kp), charge coefficient (d31), and remnant polarization (Pr) above Td. The temperature rise to 125 °C also leads to a reduction in magnetostriction (λ) and magnetostriction coefficient (q = dλ/dH) of NFO by approximately 33% and 25%, respectively. At room temperature, the bilayer and trilayer configurations exhibit maximum ME responses of approximately 33 mV/cm·Oe and 80 mV/cm·Oe, respectively, under low magnetic field conditions (H ∼ 300–450 Oe). The ME response of NKBT/NFO is highly sensitive to temperature, decreasing with heating in accordance with the individual temperature-dependent properties of NKBT and NFO. This study demonstrates a temperature window for the effective utilization of NKBT/NFO-based laminated composite ME devices.

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The data generated and analyzed during the current study are available from the corresponding author upon reasonable request.

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Acknowledgements

The authors acknowledge the IRCC, IIT Bombay, for dielectric, impedance and PE loop measurements. NV & ARK acknowledge the Department of Science and Technology, India (Project Code No. RD/0118-DST000-020) for supporting this work. AA would like to extend his gratitude to the Science and Engineering Research Board of India, DST, India for providing the financial aid under Project No.: EMR/2015/001559. The funding received from the Institute of Eminence Research Initiative Project on Materials and Manufacturing for Futuristic Mobility (Project no. SB20210850MMMHRD008275) is gratefully acknowledged. AP acknowledges the Indian Institute of Bombay, Mumbai for the post-doctoral research fellowship.

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The authors declare that no funds, grants, or other support were received during the preparation of this manuscript.

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Authors and Affiliations

  1. Department of Metallurgical Engineering and Materials Science, Indian Institute of Technology Bombay, Mumbai, 400076, India

    Adityanarayan Pandey, Pravin Varade, K. Miriyala, Ajit R. Kulkarni & N. Venkataramani

  2. Department of Applied Mechanics, Indian Institute of Technology Madras, Chennai, 600036, India

    Amritesh Kumar & A. Arockiarajan

  3. Ceramic Technologies Group-Center of Excellence in Materials and Manufacturing for Futuristic Mobility, Indian Institute of Technology Madras, Chennai, 600036, India

    A. Arockiarajan

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  1. Adityanarayan Pandey
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  7. N. Venkataramani
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Contributions

All authors contributed to study conception and design. Material preparation, data collection and analysis were performed by AP, AK, PV, and KM. The first draft of the manuscript was written by AP and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.

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Correspondence to Adityanarayan Pandey or N. Venkataramani.

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Pandey, A., Kumar, A., Varade, P. et al. Temperature-dependent magnetoelectric response of lead-free Na0.4K0.1Bi0.5TiO3/NiFe2O4-laminated composites. Appl. Phys. A 129, 843 (2023). https://doi.org/10.1007/s00339-023-07125-8

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