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Magnetic properties of new (1−x)Bi1/2Na1/2TiO3+xBaNiO3−δ solid solution materials

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Abstract

New solid solution (1−x)Bi1/2Na1/2TiO3+xBaNiO3−δ materials were synthesized by a chemical method. The X-ray diffraction and Raman scattering structure studies confirmed that the BaNiO3−δ materials were well soluted in the host Bi1/2Na1/2TiO3 materials. The random incorporation of Ba and Ni into the host Bi1/2Na1/2TiO3 materials was displayed by the optical properties where the optical bandgap values were reduced, and the photoluminescence was suppressed. The complex magnetic properties of Bi1/2Na1/2TiO3 materials were obtained as a function of BaNiO3−δ amounts in the solid solutions. The role of co-modification of A- and B-sites via alkaline earth metals and transition metals as substitution and interstitially on magnetic properties of Bi1/2Na1/2TiO3 materials was experimentally proposed, which is further supported by first-principles density functional theory calculations. We expected that our work provided a new method to inject the ferromagnetic properties in lead-free ferroelectric materials for smart electronic applications.

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Acknowledgements

This research is funded by Vietnam National Foundation for Science and Technology Development Vietnam (NAFOSTED) under grant number 103.02-2019.366. This work is supported by the Incheon National University Research Grant No. 20180438. This research was partially supported by the Nippon Sheet Glass Foundation.

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Authors and Affiliations

  1. School of Engineering Physics and Multifunctional Ferroics Materials Lab., Ha Noi University of Science and Technology, 1 Dai Co Viet Road, Ha Noi, Viet Nam

    Dang Duc Dung, Nguyen Hoang Thoan, Nguyen Huu Lam, Vu Tien Lam & Pham Dinh Luong

  2. Faculty of Physics, Ha Noi National University of Education, 136 Xuan Thuy, Ha Noi, Viet Nam

    Phan Van Vinh & Duong Quoc Van

  3. Department of Physics, Incheon National University, Incheon, 22012, South Korea

    Dorj Odkhuu

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  1. Dang Duc Dung
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Dung, D.D., Thoan, N.H., Van Vinh, P. et al. Magnetic properties of new (1−x)Bi1/2Na1/2TiO3+xBaNiO3−δ solid solution materials. Appl. Phys. A 128, 168 (2022). https://doi.org/10.1007/s00339-022-05281-x

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