Abstract
A two-dimensional free boundary transmission problem arising in the modeling of an electrostatically actuated plate is considered and a representation formula for the derivative of the associated electrostatic energy with respect to the deflection of the plate is derived. The latter paves the way for the construction of energy minimizers and also provides the Euler–Lagrange equation satisfied by these minimizers. A by-product is the monotonicity of the electrostatic energy with respect to the deflection.
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1 Introduction
We consider a model for a microelectromechanical system (MEMS) featuring an elastic, electrostatically actuated plate with positive thickness as introduced in [3]. More precisely, given a finite interval \(D:=(-L,L)\) with \(L>0\), let the function \(u\in C({\bar{D}},[-H,\infty ))\) with \(u(\pm L)=0\) measure the deflection from rest of the lower part of an elastic plate with thickness \(d>0\), clamped at its boundaries and suspended above a fixed ground plate, the latter being located at \(z=-H\) with \(H>0\) and represented by \(D\times \{-H\}\) (see Fig. 1). The deflected elastic plate is then
while the region between the ground plate and the deflected elastic plate is
The two regions are separated by the interface
and the subdomain of \(D\times (-H,\infty )\) spanned by the MEMS device is
The deflection of the plate being triggered by electrostatic actuation, the total energy of the device is
with mechanical energy \(E_\textrm{m}(u)\) and electrostatic energy \(E_\textrm{e}(u)\). The former is given by
with \(\beta >0\) and \(a, \tau \ge 0\), taking into account bending and external stretching effects of the elastic plate. The electrostatic energy
involves the electrostatic potential \(\psi _u\) in the domain \(\Omega (u)\) with \(\psi _u\) being the solution to the transmission problem
where \(\llbracket \cdot \rrbracket \) denotes the (possible) jump across the interface \(\Sigma (u)\); that is,
whenever meaningful for a function \(f:\Omega (u)\rightarrow {\mathbb {R}}\). Moreover,
involves the material dependent constant permittivities \(\sigma _2,\sigma _1>0\). The unit normal vector field to \(\Sigma (u)\) (pointing into \(\Omega _2(u)\)) is
As for the boundary values in (1.2c) we assume the particular form
where
with \(V>0\). For instance, \(\zeta (r):=V\min \{1,(r-1)^m/d^m\}\) for \(r>1\) and \(m>2\) and \(\zeta \equiv 0\) on \((-\infty ,1]\) is a possible choice. Note that
that is, the ground plate and the top of the elastic plate are kept at different constant potentials. Let us emphasize that we explicitly allow that the elastic plate touches upon the ground plate when u reaches the value \(-H\) somewhere, a situation corresponding to a non-empty coincidence set
as depicted in Fig. 2. In this case, the region \(\Omega _1(u)\) is not connected and its boundary features cusps, so that its connected components are not Lipschitz domains.
In this research we shall be interested in minimizers of the total energy E which correspond to stationary states of the MEMS device. More precisely, we shall show the existence of minimizers and derive the corresponding Euler–Lagrange equation they satisfy, which, due to the nature of the problem, is a variational inequality. Obviously, the main difficulty in this regard is related to the electrostatic energy \(E_\textrm{e}\) and the associated transmission problem (1.2) for the electrostatic potential. The latter was investigated in [5] for deflections belonging to the set
with \(\llbracket \sigma \rrbracket =\sigma _1-\sigma _2 \). More precisely, the following result is shown in [5].
Theorem 1.1
[5, Theorem 1.1] Suppose (1.4).
-
(a)
For each \(u\in \bar{{\mathcal {S}}}\), there is a unique variational solution \(\psi _u \in h_{u}+H_{0}^1(\Omega (u))\) to (1.2). Moreover,
$$\begin{aligned} \psi _{u,1}:= \psi _{u}|_{\Omega _1(u)} \in H^2(\Omega _1(u))\,\textrm{and}\,\, \psi _{u,2} := \psi _{u}|_{\Omega _2(u)} \in H^2(\Omega _2(u)), \end{aligned}$$and \(\psi _{u}\) is a strong solution to the transmission problem (1.2).
-
(b)
Given \(\kappa >0\), there is \(c(\kappa )>0\) such that \(\psi _u\) satisfies
$$\begin{aligned} \Vert \psi _u\Vert _{H^1(\Omega (u))} + \Vert \psi _{u,1}\Vert _{H^2(\Omega _1(u))} + \Vert \psi _{u,2}\Vert _{H^2(\Omega _2(u))} \le c(\kappa ) \end{aligned}$$for every \(u\in \bar{{\mathcal {S}}}\) with \(\Vert u\Vert _{H^2(D)}\le \kappa \).
The \(H^2\)-regularity of the electrostatic potential \(\psi _u\) provided by Theorem 1.1 is then the basis for deriving the existence of minimizers of the total energy E. We shall look for minimizers with clamped boundary conditions; that is, minimizers in the closed convex subset
of \(H^2(D)\). We denote by \(\partial {\mathbb {I}}_{\bar{{\mathcal {S}}}_0}\) the subdifferential of the indicator function \({\mathbb {I}}_{\bar{{\mathcal {S}}}_0}\). Our main result then reads:
Theorem 1.2
Assume \(a>0\) or \(\llbracket \sigma \rrbracket <0\), and let (1.4) be satisfied. Then, the total energy E has at least one minimizer in \(\bar{{\mathcal {S}}}_0\). Moreover, any minimizer \(u_*\in \bar{{\mathcal {S}}}_0\) of E in \(\bar{{\mathcal {S}}}_0\) with
is an \(H^2\)-weak solution to the variational inequality
that is,
for all \(w\in {\bar{{\mathcal {S}}}_0}\). For \(u\in \bar{{\mathcal {S}}}_0\), the function \(g(u)\in L_2(D)\) is given by
Finally, if \(\llbracket \sigma \rrbracket <0\), then \(u_*\le 0\) in D.
Even though the total energy E consists of two competing terms with different signs, it is not difficult to see that it is \(H^2\)-coercive if \(a>0\) in (1.1b), see [4], and the existence of a minimizer for E in \(\bar{{\mathcal {S}}}_0\) follows directly. When \(a=0\), the coercivity of E is no longer obvious without additional assumptions. In fact, we are not able to prove directly that E is bounded below and thus have to proceed differently. In this case, the coercivity of the functional can be enforced by adding a penalty term which vanishes when u is bounded, an idea already used in [2]. The minimizers of the penalized energy functional on \(\bar{{\mathcal {S}}}_0\) then satisfy the Euler–Lagrange equation (1.7) with an additional term. The assumption \(\llbracket \sigma \rrbracket <0\) now guarantees that \(g(u)\ge 0\) in D according to (1.8) which, in turn, yields an a priori bound on the minimizers by a comparison argument. This then implies that the minimizers of the penalized energy actually minimize the total energy E. It is worth emphasizing that the non-negative sign of g(u) — read off from the explicit formula (1.8) when \(\llbracket \sigma \rrbracket <0\) — is essential for this approach.
The main motivation of this research is thus the derivation of an explicit formula for the electrostatic force g(u) as the (directional) derivative of the electrostatic energy \(E_\textrm{e}(u)\). By definition of \(E_\textrm{e}(u)\), such a computation corresponds to that of a shape derivative and thus follows the guidelines of classical results [1, 6, 7]. In fact, a computation in the same spirit is performed in [4] for a related MEMS model but with a flat transmission interface. As we shall see in Sect. 2, the non-flat transmission interface \(\Sigma (u)\) in (1.2b) leads to additional terms in the electrostatic force, making the computation of the latter noticeably more involved. We first establish in Sect. 2 differentiability properties of the electrostatic potential \(\psi _u\) with respect to u which then ensure the Fréchet differentiability of the electrostatic energy \(E_\textrm{e}\) on \({\mathcal {S}_0}\). The subsequent identification of g(u) as the (directional) derivative of the electrostatic energy \(E_\textrm{e}(u)\) is the main contribution of Sect. 2. It is worth already pointing out here that the derivation of the explicit formula (1.8) of g(u) does not require the explicit computation of the derivative of the electrostatic potential \(\psi _u\) with respect to u. Once the formula (1.8) is established, the existence of minimizers of E in \(\bar{{\mathcal {S}}}_0\) follows along the lines of [2] as described above.
As already pointed out, the electrostatic force g(u) has a sign if one assumes that \(\llbracket \sigma \rrbracket <0\); that is, if \(\sigma _2> \sigma _1\). For instance, this is a natural assumption when the region between the two plates is vacuumed or filled with air. We also point out that this assumption implies the monotonicity of the electrostatic energy \(E_\textrm{e}\) as stated explicitly in Corollary 2.7.
Remark 1.3
The total energy E can also be minimized in \(\bar{{\mathcal {S}}}\) leading then to weak solutions to (1.7) with \({\mathbb {I}}_{\bar{{\mathcal {S}}}}\) instead of \({\mathbb {I}}_{\bar{{\mathcal {S}}}_0}\) which satisfy pinned boundary conditions \(u(\pm L) = \partial _x^2 u(\pm L)=0\) instead of the clamped boundary conditions involved in \(\bar{{\mathcal {S}}}_0\). In this case, however, one has to be slightly more careful when computing the shape derivative of the electrostatic energy \(E_\textrm{e}\) due to the different constraints on the boundary.
2 Shape derivative of the electrostatic energy
The heart of the proof of Theorem 1.2 is the differentiability of the electrostatic energy \(E_\textrm{e}\) and, in particular, the identification of g(u) as its derivative at \(u\in \bar{{\mathcal {S}}}_0\). On a formal level, this derivative is computed in [3] (in a three-dimensional setting). Here we provide a rigorous proof. Actually, we shall show that the electrostatic energy \(E_\textrm{e}\) is Fréchet differentiable on
i.e., for points with empty coincidence set, while it admits a directional derivative at \(u\in \bar{{\mathcal {S}}}_0\) in the directions \(-u+{\mathcal {S}}_0\). Here and in the following, \({\mathcal {S}}_0\) and \(\bar{{\mathcal {S}}}_0\) are endowed with the \(H^2(D)\)-topology. The precise result reads as follows:
Theorem 2.1
Assume (1.4). The electrostatic energy \(E_\textrm{e}: {{\mathcal {S}}_0}\rightarrow {\mathbb {R}}\) is continuously Fréchet differentiable with
for \(u\in {\mathcal {S}}_0\) and \(\vartheta \in H^2(D)\cap H_0^1(D)\), where g(u) is defined in (1.8). Moreover, if \(u\in \bar{{\mathcal {S}}}_0\) and \(w\in {\mathcal {S}}_0\), then
The function \(g:\bar{{\mathcal {S}}}_0\rightarrow L_p(D)\) is continuous for each \(p\in [1,\infty )\).
The proof of Theorem 2.1 follows from Proposition 2.5 and Corollary 2.7 below. We will need the following result which is contained in [5].
Proposition 2.2
[5, Theorem 1.3, Proposition 3.3] Assume (1.4). Let \(u\in \bar{{\mathcal {S}}}_0\) and consider a bounded sequence \((u_n)_{n\ge 1}\) in \(\bar{{\mathcal {S}}}_0\) such that
Then, for any \(p\in [1,\infty )\),
Moreover,
Finally, setting
one has
The first step of the proof of Theorem 2.1 is to show that the electrostatic energy \(E_\textrm{e}\) is Fréchet differentiable on \({\mathcal {S}}_0\). The next lemma is adapted from [1, Theorem 5.3.2], see also [4, Lemma 4.1]. We include the proof for the reader’s ease.
Lemma 2.3
Assume (1.4). Let \(u\in {\mathcal {S}}_0\) be fixed and define, for \(v\in {\mathcal {S}}_0\), the transformation
by
Then there exists a neighborhood \({\mathcal {U}}\) of u in \({\mathcal {S}}_0\) such that the mapping
is continuously differentiable, recalling that \({\mathcal {S}}_0\) and thus also \({\mathcal {U}}\) are endowed with the \(H^2(D)\)-topology.
Remark 2.4
Lemma 2.3 is only an intermediate step in the computation of the Fréchet derivative of the electrostatic energy \(E_\textrm{e}\). As we shall see later in the proof of Proposition 2.5, the computation does not require an explicit formula for the derivative of \(v\mapsto \xi _v\). Moreover, we do not strive for optimal assumptions (e.g., the topology of \({\mathcal {S}}_0\) can be weakened, as long as it is stronger than that of \(W_\infty ^1(D)\)).
Proof of Lemma 2.3
The differentiability property relies on a classical approach: we shall first identify a suitable \(C^1\)-function
which vanishes at \((v,\xi _v)\) whenever \(v\in {\mathcal {S}}_0\). We then show that the implicit function theorem applies to \({\mathcal {F}}\) near \((u,\xi _u)\).
To this end, set \(\chi _v:=\psi _v-h_v\) for \(v\in {\mathcal {S}}_0\). Owing to Theorem 1.1, the function \(\chi _v\) belongs to \(H_0^1(\Omega (v))\) and satisfies the integral identity
which we next shall write as integrals over \(\Omega (u)\). To this end, we first note that, due to \(\Theta _{u,u}=\textrm{id}\),
where
and
For \(\phi \in H_0^1(\Omega (u))\) we set
and note that
Performing the change of variables \(({{\bar{x}}},\bar{z})=\Theta _{u,v}(x,z)\) in (2.5) with \(\theta =\phi _v\) and using (1.3) give
where the Jacobian \(J_v:=\vert \textrm{det}(D\Theta _{u,v})\vert \) is given by
Introducing the notations
and
we define the function
and observe that (2.7) is equivalent to
We then shall use the implicit function theorem to show that \(\xi _v\) depends smoothly on v. For that purpose, let us first show that \({\mathcal {F}}\) is Fréchet differentiable in \({\mathcal {S}}_0\times H_0^1(\Omega (u))\). Indeed, by (1.4), it is readily checked that
is linear in v, so that its Fréchet derivative with respect to v is
for \(\vartheta \in H^2(D)\cap H_0^1(D)\). Thus,
Moreover, \(v\mapsto J_v\) and \(v\mapsto (D\Theta _{u,v})^{-1}\) are continuously differentiable from \({\mathcal {S}}_0\) to \(L_\infty (\Omega (u))\) and \(L_\infty (\Omega (u),{\mathbb {R}}^{2\times 2})\), respectively, and we conclude that
is continuously differentiable from \({\mathcal {S}}_0\) to \(L_2(\Omega (u),{\mathbb {R}}^{2})\). Hence
The \(C^1\)-smoothness of \((v,\xi )\mapsto \textrm{div}(A(v)\nabla \xi )\) is proven as in [1, Theorem 5.3.2] and we have thus established that
The Lax–Milgram theorem and the open mapping theorem imply that the mapping
is an isomorphism from \(H_0^1(\Omega (u))\) to \(H^{-1}(\Omega (u))\). Consequently, by the implicit function theorem there is a neighborhood \({\mathcal {W}}\) of \((u,\xi _u)\) in \({\mathcal {S}}_0\times H_0^1(\Omega (u))\), a neighborhood \({\mathcal {U}}\) of u in \({\mathcal {S}}_0\), and a function \(\Xi \in C^1({\mathcal {U}},H_0^1(\Omega (u)))\) with \(\Xi (u)=\xi _u\) such that
By (2.3), we may assume that \((v,\xi _v)\in {\mathcal {W}}\) for \(v\in {\mathcal {U}}\). Hence, \(\xi _v=\Xi (v)\) for \(v\in {\mathcal {U}}\) and the proof is complete. \(\square \)
We next compute the Fréchet derivative of the electrostatic energy on \({\mathcal {S}}_0\) and thereby provide a proof of the first part of Theorem 2.1. This computation follows the classical approach developed in [1, 6, 7] for shape derivatives and is performed in a similar way in [4] for a geometry with a flat interface instead of \(\Sigma (u)\). It is worth pointing out that the non-flat transmission interface considered herein leads to additional terms. The concise formula (1.8) that we derive for the derivative g(u) of \(E_\textrm{e}(u)\) reveals the importance of these contributions to the electrostatic force, as it involves terms that counteract the contributions from the top of the elastic plate when \(\llbracket \sigma \rrbracket >0\). As the identification of these additional terms and the derivation of the concise formula (1.8) do not seem to be straightforward, we give a detailed proof (see also Remark 2.6 below).
Proposition 2.5
Assume (1.4). The electrostatic energy \(E_\textrm{e}: {\mathcal {S}}_0\rightarrow {\mathbb {R}}\) is continuously Fréchet differentiable with
for \(u\in {\mathcal {S}}_0\) and \(\vartheta \in H^2(D)\cap H_0^1(D)\), where g(u) is defined in (1.8).
Proof
The proof is quite technical and basically includes three steps. As a starting point, we shall use Lemma 2.3 which guarantees the differentiability of \(E_\textrm{e}\) and yields an abstract formula for its derivative, see (2.11) below. Computing then this derivative explicitly, we first derive in (2.20) an expression involving only the trace of the gradient of \(\psi _u\) on the top of the elastic plate and the jumps of \(\sigma \) and the partial derivatives of \(\psi _u\) on the interface. Finally, we write the interface integrals in terms of \(\psi _{u,2}\) only and thus obtain the desired formula (1.8).
To be more precise, we fix \(u\in {\mathcal {S}}_0\) and use the notation introduced in Lemma 2.3. Recall that, according to Lemma 2.3, there is a neighborhood \({\mathcal {U}}\) of u in \({\mathcal {S}}_0\) such that the mapping
belongs to \(C^1({\mathcal {U}},H_0^1(\Omega (u)))\), the transformation \(\Theta _{u,v}:\Omega (u)\rightarrow \Omega (v)\) being defined in (2.4). Now, for \(v\in {\mathcal {U}}\), we use (2.6), the relation \(\chi _v=\psi _v-h_v\), and the change of variable \((\bar{x},{{\bar{z}}})=\Theta _{u,v}(x,z)\) in the integral defining \(E_\textrm{e}(v)\) to obtain
where
Owing to the differentiability of \(v\mapsto \xi _v\) in \({\mathcal {U}}\), we deduce that the Fréchet derivative of \(E_\textrm{e}\) at u applied to some \(\vartheta \in H^2(D)\cap H_0^1(D)\) is given by
Taking the identity \(j(u) =\nabla \chi _u + \nabla h_u=\nabla \psi _u\) into account, we infer from (2.8) that
We next use that \(\Theta _{u,u}\) is the identity on \(\Omega (u)\) and that \(\xi _u=\chi _u\) to compute from the definition of j(v) that
Now, \(\chi _{u,1}=\psi _{u,1}\) in \(\Omega _1(u)\) due to (1.4), so that
while
Also note that
Consequently, gathering (2.11)–(2.15) and recalling (2.10) lead us to
where
and
We are left with simplifying these three integrals and begin with \(I_0(u)[\vartheta ]\). We use Gauß’ theorem and (1.2a) to get
Now, recall that \(\partial _v \xi _v[\vartheta ]\big \vert _{v=u}\) belongs to \(H_0^1(\Omega (u))\) according to Lemma 2.3. On the one hand, this entails that \(\partial _v \xi _v[\vartheta ]\big \vert _{v=u}\) vanishes on \(\partial \Omega (u)\), so that the first integral on the right-hand side of the above identity is zero. On the other hand, the \(H^1\)-regularity of \(\partial _v \xi _v[\vartheta ]\big \vert _{v=u}\) also implies that \(\llbracket \partial _v \xi _v[\vartheta ]\big \vert _{v=u} \rrbracket =0\) on \(\Sigma (u)\), so that
due to (1.2b). Therefore,
We next deal with \(I_1(u)[\vartheta ]\). Since \(\sigma _1 \Delta \psi _{u,1} = \textrm{div}(\sigma \nabla \psi _u) = 0\) in \(\Omega _1(u)\) by (1.2a), it follows from Gauß’ theorem that
Recalling that \(\vartheta \in H_0^1(D)\) and noticing that
we further obtain
Hence,
Finally, using (1.4a), \(\chi _u=\psi _u-h_u\), and \(\vartheta \in H_0^1(D)\), it follows from Green’s formula that
Owing to (1.2a), we have \(\sigma _2 \partial _x^2\psi _{u,2} = -\sigma _2 \partial _z^2\psi _{u,2}\) in \(\Omega _2(u)\) from which we deduce that
Consequently,
We finally note that
since \(\psi _{u,2}(x,u(x)+d)=V\) owing to (1.2c) and (1.4b). This identity allows us to simplify further the formula for \(I_2(u)[\vartheta ]\), so that we end up with
Collecting (2.16), (2.17), (2.18), and (2.19) gives
Finally, we shall write (2.20) only in terms of \(\psi _{u,2}\). To this end, we set
and observe that differentiating the transmission condition \(\llbracket \psi _u \rrbracket = 0\) on \(\Sigma (u)\), along with the second transmission condition in (1.2b), ensures that
These properties in turn imply that
Guided by (2.22), we next express the jump terms in (2.20) using \(F_u\) and \(G_u\). Since
we compute
Therefore, by (2.22),
Consequently, plugging this formula into (2.20) and recalling (2.21) yield
that is,
for \(u\in {\mathcal {S}}_0\) and \(\vartheta \in H^2(D)\cap H_0^1(D)\) with g(u) being defined in (1.8). It then readily follows from (2.1) that
is continuous. \(\square \)
Remark 2.6
Compared to the proof of [4, Proposition 4.2], the main difference in the proof of Proposition 2.5 is the term \(I_1({u})\) stemming from the non-flatness of the interface \(\Sigma ({u})\). Additionally, even though the terms \(I_0({u})\) and \(I_2({u})\) already appear in the flat geometry considered in [4, Proposition 4.2], they give herein different contributions to g(u) due to the specific choice (1.4) of the boundary values (1.2c).
The final step of the proof of Theorem 2.1 is to show that the electrostatic energy \(E_\textrm{e}\) admits directional derivatives in the directions \(-u+{\mathcal {S}}_0\).
Corollary 2.7
Assume (1.4). Let \(u_0\in \bar{{\mathcal {S}}}_0\) and \(u_1\in {\mathcal {S}}_0\). Then
Moreover, the function \(g:\bar{{\mathcal {S}}}_0\rightarrow L_p(D)\) is continuous for each \(p\in [1,\infty )\).
Proof
The stated continuity of g is a straightforward consequence of (2.1). Next, given \(u_0\in \bar{{\mathcal {S}}}_0\) and \(u_1\in {\mathcal {S}}_0\), we set
Since \(u_s\in {\mathcal {S}}_0\) for \(s\in (0,1]\), we deduce from Proposition 2.5 that
Therefore, letting \(s\rightarrow 0\), the continuity of g entails
Now (2.2) guarantees that \(E_\textrm{e}(u_s) \rightarrow E_\textrm{e}(u_0)\) as \(s\rightarrow 0\), so that
and we conclude from (2.24) that
as claimed. \(\square \)
If \(\llbracket \sigma \rrbracket <0\), then an obvious consequence of (1.8) is that g is non-negative on \(\bar{{\mathcal {S}}}_0\). This yields the monotonicity of the electrostatic energy \(E_\textrm{e}\).
Corollary 2.8
Assume \(\llbracket \sigma \rrbracket <0\) and (1.4). If \(u_0\in \bar{{\mathcal {S}}}_0\) and \(u_1\in {\mathcal {S}}_0\) are such that \(u_0\le u_1\) in D, then \(E_\textrm{e}(u_0)\le E_\textrm{e}(u_1)\).
Proof
The assumption \(\llbracket \sigma \rrbracket <0\) implies that \(g(u_s)\ge 0\) for \(s\in (0,1]\) according to (1.8), where \(u_s= (1-s) u_0 + s u_1\) as in the proof of Corollary 2.7. Hence, (2.23) and (2.25) with \(t=1\) imply the assertion. \(\square \)
3 Proof of Theorem 1.2
The proof of Theorem 1.2 now follows from Theorem 2.1 as in [2]. Indeed, Theorem 2.1 guarantees that any minimizer of the total energy E on \(\bar{{\mathcal {S}}}_0\) satisfies the Euler–Lagrange equation (1.7). In case that \(a>0\), the total energy E is coercive and thus the existence of a minimizer of E in \(\bar{{\mathcal {S}}}_0\) can be shown as in [2, Section 7]. In the more complex case \(a=0\), the total energy E need not be coercive. But, as pointed out in the introduction, one may enforce its coercivity by adding a penalizing term and proceed along the lines of [2, Section 6], recalling that the assumption \(\llbracket \sigma \rrbracket <0\) guarantees that \(g(u)\ge 0\) in D, which is essential in this case (see, in particular, [2, Equation (6.4)]).
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Acknowledgements
Part of this work was done while PhL enjoyed the hospitality and support of the Institut für Angewandte Mathematik, Leibniz Universität Hannover. We express our gratitude to the anonymous referees for their helpful comments.
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Laurençot, P., Walker, C. Stationary states to a free boundary transmission problem for an electrostatically actuated plate. Nonlinear Differ. Equ. Appl. 30, 2 (2023). https://doi.org/10.1007/s00030-022-00809-9
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DOI: https://doi.org/10.1007/s00030-022-00809-9