Abstract
Neutron-deficient isotopes of radium have been produced in the reactions35Cl+175Lu,40Ar+170,171Yb, and36Ar+170,171Yb and separated in-flight with a gas-filled recoil separator. The activities have been identified on the basis of correlated alpha decay chains. The alpha particle energy Eα and the half-life T1/2 of an isomeric state of the new isotope,203mRa, have been determined to be (7615±20) keV and (33 +22−10 ) ms, respectively. An assignment of another decay with Eα = (7577±20) keV and T1/2=(1.1 +5.0−0.5 ) ms to203gRa is made on the basis of one observed three-decay chain. Tentative evidence for the production of the new isotope202Ra is also given. The values Eα = (7860±60) keV and T1/2=(0.7 +3.3−0.3 ) ms were measured. Improved decay data have been obtained for204Ra. The results are Eα = (7484±10) keV and T1/2=(59 +12−9 ) ms. Earlier findings concerning the decay of two states in205Ra and an isomer in207Ra have been confirmed. Approximate values for cross sections have been determined for202Ra, produced using the36Ar+170Yb reaction and for203Ra,204Ra, and205Ra using the35Cl+175Lu reaction. The results are 2 nb (202Ra), 4 nb (203Ra), 40 nb (204Ra), and 800 nb (205Ra).
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Communicated by B. Povh
This work was supported by the Academy of Finland.