PAC study on¹¹¹Cd in antiferromagnetic CuO

Abstract

400 keV¹¹¹In⁺ ions were implanted into CuO powder. After annealing at 570 K, more than 50% of the implants were found on substitutional sites in the monoclinic CuO lattice. PAC-spectra taken below the Néel temperatureT _N≈230 K revealed a broadening of the quadrupole spectrum and additional satellite frequencies caused by combined electric and magnetic hyperfine interaction. Assuming that the orientation of the electric field gradient is given by the point charge model and taking the 〈010〉 direction of the supertransferred fieldB _tr in CuO from neutron diffraction, we find a Larmor frequency of ω_L≈40 MHz corresponding toB _tr≈2.7 T at 60 K.