Skip to main content
Log in

Recent lake acidification and recovery trends in southern Quebec, Canada

  • Published:
Water, Air, and Soil Pollution Aims and scope Submit manuscript

Abstract

A total of 51 lakes in southern Quebec, Canada, were sampled between 1985 and 1993 to study changes in water chemistry following reductions in SO2 emissions (main precursor of acid precipitation). Time series analysis of precipitation chemistry revealed significant reductions in concentrations and deposition of SO4 2− from 1981 to 1992 in southern Quebec as well as reductions in concentrations and deposition of base cations (Ca2+, Mg2+), NO3 and H+ in the western section of the study area. Reductions in atmospheric inputs inputs of SO4 2− have resulted in decreased lakewater SO4 2− concentrations in the majority of the lakes in our study, although only a small fraction (9 of 37 lakes used in the temporal analysis) have improved significantly in terms of acidity status (pH, acid neutralizing capacity — ANC). The main response of the lakes to decreased SO4 2− is a decrease in base cations (Ca2++Mg2+), which was observed in 17 of 37 lakes. Seventeen lakes also showed significant increases in dissolved organic carbon (DOC) over the period of study. The resulting increases in organic acidity as well as the decrease in base cations could both play a role in delaying the recovery of our lakes.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • Berryman, D., Bobée, B., Cluis, D. and Haemmerli, J.: 1988,Water Resources Bulletin 24, 545.

    CAS  Google Scholar 

  • Bobée, B., Lachance, M., Haemmerli, J., Tessier, A., Charette, J. Y. and Kramer, J.: 1983,Évaluation de la sensibilité à l'acidification des lacs du sud du Québec et incidences sur le réseau d'acquisition de données, Environment Canada, Inland Waters Directorate, Quebec Region, p. 203.

    Google Scholar 

  • Bouchard, A.: 1989,Caractérisation de la qualité de l'eau des lacs de la Côte-Nord et choix d'un scénario d'échantillonnage dans le cadre du Réseau TADPA-Québec, Environment Canada, Conservation and Protection, Quebec region. Quebec region.

    Google Scholar 

  • Bouchard, A. and Haemmerli, J.: 1992,Water, Air, and Soil Pollut. 62, 89.

    Article  CAS  Google Scholar 

  • Boulet, G. and Pinard, P.: 1991, Les précipitations acides au Québec: Bilan des années 1981 ù 1991, Presented at The Conference on Acid Rain and Ground Level Ozone (SMOG) held in Montreal, November 1991, pp. 9–27.

  • Canada/United States: 1994,Canada/United States Air Quality Agreement, Progress report.

  • Clair, T. A., Dillon, P. J., Ion, J., Jeffries, D. S., Papineau, M. and Vet, R.: 1995,Can. J. Fish. Aquat. Sci. 52, 197.

    CAS  Google Scholar 

  • Cluis, D. A., Laberge, C. and Houle, C.: 1988,Détection des tendances et dépassement de normes en qualité de l'eau, INRS-Eau.

  • Dillon, P. J. and Lazerte, B. D.: 1992,Environ. Pollut. 77, 211.

    Article  CAS  Google Scholar 

  • Dillon, P. J. and Molot, L. A.: 1990,Biogechemistry 11, 23.

    Google Scholar 

  • Dillon, P. J., Reid, R. A. and Girard, R.: 1986,Water, Air, and Soil Pollut. 31, 59.

    Article  CAS  Google Scholar 

  • Driscoll, C. T., Likens, G. E., Hedin, L. O., Eaton, J. S. and Bormann, F. H.: 1989,Environ. Sci. Technol. 23, 137.

    Article  CAS  Google Scholar 

  • Driscoll, C. T. and Van Dreason, R.: 1993,Water, Air, and Soil Pollut. 67, 319.

    Article  CAS  Google Scholar 

  • Dupont, J.: 1992a,Water; Air, and Soil Pollut. 61, 107.

    Article  CAS  Google Scholar 

  • Dupont, J.: 1992b,Water, Air, and Soil Pollut. 61, 125.

    Article  CAS  Google Scholar 

  • Dupont, J.: 1992c,Effets des réductions des étnissions de SO 2 sur la qualité de l'eau des lacs de la région de Rouyn-Noranda, Quebec Ministry of Environment, Report no. QEN/PA-43/1.

  • Dupont, J. and Grimard, Y.: 1986,Water, Air, and Soil Pollut. 31, 223.

    Article  CAS  Google Scholar 

  • Environment Canada.: 1994,Annual report on the Federal-Provincial agreements for the Eastern Canada Acid Rain Program: 1993, Environment Canada, Conservation and Protection.

  • Hedin, L. O., Granat, L., Likens, G. E., Buishand, T. A., Galloway, J. N., Butler, T. J. and Rodhe, H.: 1994,Nature 367, 351.

    Article  CAS  Google Scholar 

  • Hedin, L. O., Likens, G. E., Postek, K. M. and Driscoll, C. T.: 1990,Nature 345, 798.

    Article  CAS  Google Scholar 

  • Henriksen, A. and Brakke, D. F.: 1988,Water, Air, and Soil Pollut. 42, 183.

    Article  CAS  Google Scholar 

  • Herlihy, A. T., Landers, D. H., Cusimano, R. F., Overton, W. S., Wigington, P. J. Jr., Pollack, A. K. and Mitchell-Hall, T. E.: 1990,Temporal variability in lakewater chemistry in the North-eastern United States: Results of phase 11 of the Eastern Lake Survey, NSI Technology Services Corp., prepared for Corvallis Environmental Research Lab., Or.

  • Hirsch, R. M., Slack, J. R. and Smith, R. A.: 1982,Water Resour. Res. 18, 107.

    Google Scholar 

  • Hirsch, R. M. and Slack, J. R.: 1984,Water Resour. Res. 20, 727.

    Google Scholar 

  • Holtze, K. E. and Hutchinson, N. J.: 1989,Can. J. Fish. Aquat. Sci. 46, 1188.

    Article  CAS  Google Scholar 

  • Kahl, J. S., Haines, T. A., Norton, S. A. and Davis, R. B.: 1993,Water, Air, and Soil Pollut. 67, 281.

    Article  CAS  Google Scholar 

  • Keller, W., Pitblado, J. R. and Carbone, J.: 1992,Can. J. Fish. Aquat. Sci. 49, 23.

    Article  Google Scholar 

  • Kelso, J. R. M. and Jeffries, D. S.: 1988,Can. J. Fish. Aquat. Sci. 45, 1905.

    CAS  Google Scholar 

  • Lettenmaier, D. P.: 1976,Water Resour. Res. 12, 1037.

    Article  Google Scholar 

  • Matuszek, J. E. and Beggs, G. L.: 1988,Can. J. Fish. Aquat. Sci. 45, 1931.

    Article  Google Scholar 

  • Murdoch, P. S. and Stoddard, J. L.: 1992,Water Resourc. Res. 28, 2707.

    Article  CAS  Google Scholar 

  • Murdoch, P. S. and Stoddard, J. L.: 1993,Water, Air, and Soil Pollut. 67, 367.

    Article  CAS  Google Scholar 

  • Newell, A. D.: 1993,Water, Air, and Soil Pollut. 67, 257.

    Article  CAS  Google Scholar 

  • Oliver, B. G., Thurman, E. M. and Malcolm, R. L.: 1983,Geochimica et Cosmochimica Acta 47, 2031.

    Article  CAS  Google Scholar 

  • Paul, E. A. and Clark, F. E.: 1989,Soil Microbiology and Biochemistry, Academic Press, San Diego, CA., p. 271.

    Google Scholar 

  • RMCC.: 1990,The 1990 Canadian Long-Range Transport of Air Pollutants and Acid Deposition Assessment Report: Part 4 Aquatic effects, Federal/Provincial Research and Monitoring Coordinating Committee.

  • Sirois, A.: 1993,Atmospheric Environment 27A, 945.

    CAS  Google Scholar 

  • Stoddard, J. L. and Kellogg, J. H.: 1993,Water, Air, and Soil Pollut. 67, 301.

    Article  CAS  Google Scholar 

  • Tremblay, S. and Richard, Y.: 1993,Water, Air, and Soil Pollut. 66, 315.

    CAS  Google Scholar 

  • Wilkinson, K. J., Jones, H. G., Campbell, P. G. C. and Lachance, M.: 1992,Water, Air, and Soil Pollut. 61, 57.

    Article  CAS  Google Scholar 

  • Wright, R. F.: 1989,Water, Air, And Soil Pollut. 46, 251.

    CAS  Google Scholar 

  • Wright, R. F. and Haus, M.: 1991,Proceedings of the Royal Society of Edinburgh 97B, 169.

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Rights and permissions

Reprints and permissions

About this article

Cite this article

Bouchard, A. Recent lake acidification and recovery trends in southern Quebec, Canada. Water Air Soil Pollut 94, 225–245 (1997). https://doi.org/10.1007/BF02406060

Download citation

  • Received:

  • Accepted:

  • Issue Date:

  • DOI: https://doi.org/10.1007/BF02406060

Key words

Navigation