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Dose equivalent commitments from fallout radionuclides in the open waters of the Great Lakes. 1973–1981

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Abstract

The levels of 144Ce, 137Cs, 125Sb, and 90Sr in the open waters of the Great Lakes were measured over the period 1973–81. The levels were found to be very low. 144Ce was detected only up to 1975 after which it dropped below the detection limit. The data indicate that the concentrations of the remaining three radionuclides have decreased with time. 90Sr and 137Cs provide essentially all of the radiological dose from drinking Great Lakes water. The dose equivalant commitments have been calculated from these measurements and found to be well within the Great Lakes Water Quality Agreement's water quality objective for radioactivity.

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References

  • Argonne National Laboratory: 1973, ‘Radiological and Environmental Research Division Annual Report’, ANL-7960, Part III, January-December 1972.

  • Barry, P. J.: 1973, ‘Estimating Dose Commitments to Populations from Radioative Waste Disposals into Large Lakes’, in Environmental Behaviour of Radionuclides Released in the Nuclear Industry, IAEA-SM-172/43, Vienna, Austria, pp. 499–506.

  • Canada and the United States: 1972, ‘Great Lakes Water Quality Agreement’.

  • Canada and the United States: 1978, ‘Great Lakes Water Quality Agreement’, Annex 1, Section IV.

  • DurhamR. W.: 1974, Radionuclide Levels in the Great Lakes Waters-1973’, Scientific Series No. 48, Inland Waters Directorate, Canada Centre for Inland Waters, Burlington, Ontario.

    Google Scholar 

  • DurhamR. W. and JoshiS. R.: 1979, ‘Radionuclide Concentrations in Two Sewage Treatment Plants on Western Lake Ontario, Canada’, J. Radioanal. Chem. 54, 367–370.

    Google Scholar 

  • DurhamR. W. and JoshiS. R.: 1980b, ‘Recent Sedimentation Rates, 210Pb Fluxes, and Particle Settling Velocities in Lake Huron, Laurentian Great Lakes’, Chem. Geol. 31, 53–66.

    Google Scholar 

  • DurhamR. W. and JoshiS. R.: 1980b, ‘Investigation of Lake Ontario Water Quality Near Port Granby Radioactive Waste Management Site’, Water, Air, and Soil Pollut. 13, 17–26.

    Google Scholar 

  • EdgingtonD. N., WahlgrenM. A., and MarshallJ. S.: 1976, ‘The Behaviour of Plutonium in Aquatic Ecosystems: A Summary of Studies on the Great Lakes’, in M. W.Miller and J. N.Stannard (eds.), Environmental Toxicity of Aquatic Radionuclides: Models and Mechanisms, Ann Arbor Science, Ann Arbor, MI, pp. 45–80.

    Google Scholar 

  • FeelyH. W., VolchokH. L., HardyJr.E. P., and ToonkelL. E.: 1978, ‘Worldwide Deposition of 90Sr Through 1976’, Environ. Sci. & Tech. 12, 808–809.

    Google Scholar 

  • FrancisC. W. and BrinkleyF. S.: 1976, ‘Preferential Adsorption of 137Cs to Micaceous Minerals in Contamined Freshwater Sediment’, Nature 260, 511–513

    Google Scholar 

  • GregoryL. P.: 1972, ‘A Simplified Separation of Strontium, Radium, and Lead from Environmental Media by Precipitation Followed by Fractional Elution, Anal. Chem. 44, 2113–2115.

    Google Scholar 

  • International Commission on Radiological Protection: 1979, ‘Limits for Intake of Radionuclides for Workers’, Publication 30.

  • International Joint Commission, 1978: ‘Great Lakes Water Quality 1977’, Appendix D, Radioactivity Subcommittee Report.

  • KimuraT., KiyoshiI., IshimoriT., and HamadaT.: 1979, ‘Separation of Strontium-89 and-90 from Calcium in Milk with a Macrocyclic Ether’, Anal. Chem. 51, 1113–1116.

    Google Scholar 

  • LermanA.: 1972, ‘90Sr in the Great Lakes: Concentration-Time Model’, J. Geophys. Res. 77, 3256–3264.

    Google Scholar 

  • TracyB. L. and PrantlF. A.: 1983, ‘25 Years of Fission Product Input to Lakes Superior and Huron’, Water, Air, and Soil Pollut. 19, 15–27.

    Google Scholar 

  • WadeM. A. and SeimH. J.: 1961, ‘Ion Exchange Separation of Calcium and Strontium. Application to Determination of Total Strontium in Bone’, Anal. Chem. 33, 793–795.

    Google Scholar 

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Durham, R.W., Joshi, S.R. Dose equivalent commitments from fallout radionuclides in the open waters of the Great Lakes. 1973–1981. Environ Monit Assess 4, 405–417 (1984). https://doi.org/10.1007/BF00394178

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  • DOI: https://doi.org/10.1007/BF00394178

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