Abstract
Multivariate regression analysis was used to determine the major emission sources contributing to suspended particulates in air collected over a small mixed land use watershed. Aerosol samples were collected at 5 different land use types in 1976 and 1977 and analyzed for 10 elements. Aerosol composition was then compared to emission source composition to obtain the relative contribution by each emission source. Two examples of source reconciliation by multivariate regression analysis for typical samples are given. An industrial land use type clearly shows increased contributions from anthropogenic activity when compared to a rural site only 15 km distant in a crosswind direction. Differences in calculated and measured ambient aerosol concentrations can lead to specific interpretations about emission sources. The implications of errors in concentration data are discussed. A weighting technique can aid in correcting problems caused by incomplete or inaccurate data for 1 or 2 elements.
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Andren, A. W. and Lindberg, S. E.: 1977, Water, Air, Soil Pollut. 8, 199.
Andren, A. W. and Strand, J. W.: 1981, ‘Atmospheric Deposition of Particulate Organic Carbon and Polyaromatic Hydrocarbons to Lake Michigan’, in S. Eisenreich (ed.), Atmospheric Pollutants in Natural Waters, Ann Arbor Science, Inc., Chapter 23.
Friedlander, S. K.: 1971, Conference ‘Science in the Control of Smog’, Pasadena, CA.
Friedlander, S. K.: 1973, Environ. Sci. Technol. 7, 235.
Gartrell, G., Jr. and Friedlander, S. K.: 1975, Atmos. Environ. 9, 279.
Gatz, D. F.: 1975, Atmos. Environ. 9, 1.
Greenberg, R. R., Gordon, G. E., and Zoller, W. H.: 1978, Environ. Sci. Technol. 12, 1329.
Hopke, P. K.: 1980, Ann. N. Y. Acad. Sci. 338, 103.
Klein, D. H., Andren, A. W., Carter, J. A., Emery, J. F., Feldman, C., Fulkerson, W., Lyon, W. S., Ogle, J. C., Talmi, Y., Van Hook, R. L, and Bolton, N.: 1975, Environ. Sci. Technol. 9, 973.
Kleinman, M. T., Pasternack, B. S., Eisenbud, M., and Kneip, T. J.: 1980, Environ. Sci. Technol. 14, 62.
Mayrsohn, H. and Crabtree, J. H.: 1976, Atmos. Environ. 10, 137.
Miller, M. S., Friedlander, S. K., and Hidy, G. M.: 1972, J. Colloid Interface Sci. 39, 165.
Murphy, T. J.: 1974, Sources of Phosphorus Inputs from the Atmosphere and their Significance to Oligotrophic Lakes, Research Report No. 92, Water Resources Center, University of Illinois, Urbana, Illinois.
Stolzenburg, T. S.: 1979, Metallic Composition ofAerosols over the Menomonee River Watershed, Ph.D Thesis, University of Wisconsin, Madison, Wisconsin.
Stolzenburg, T. S. and Andren, A. W.: 1980, Anal. Chim. Acta 118, 377.
Stolzenburg, T. S. and Andren, A. W.: 1981, Water, Air, Soil Pollut. 15, 243.
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Stolzenburg, T.R., Andren, A.W. & Stolzenburg, M.R. Source reconciliation of atmospheric aerosols. Water Air Soil Pollut 17, 75–85 (1982). https://doi.org/10.1007/BF00164093
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DOI: https://doi.org/10.1007/BF00164093