Skip to main content
Log in

Increased saturation field as the origin of the giant electrocaloric effect in Ba0.8Sr0.2TiO3 thin films

  • Published:
Journal of the Korean Physical Society Aims and scope Submit manuscript

Abstract

We investigated the electrocaloric (EC) effects in epitaxial Ba0.8Sr0.2TiO3 (BSTO) thin films grown on LaAlO3 and MgO substrates and in BSTO sol-gel thin films grown on Si substrates. We compared the EC effects in two forms of BSTO to confirm whether the giant EC effect recently observed in the polycrystalline thin film is an intrinsic effect or an extrinsic effect exclusively occurring in polycrystalline thin films with nano-sized grains. The EC effect in our BSTO single crystals exhibited a moderate EC temperature change over a broad temperature range. On the other hand, the EC effect in the BSTO sol-gel film was observed over a narrow temperature range with a giant ΔT of about 14 °C. We claim that this giant EC effect is due to the increased saturation field related to the small grain size in the sol-gel thin film.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. B. A. Tuttle and D. A. Payne, Ferroelectrics 37, 603 (1981).

    Article  Google Scholar 

  2. P. D. Thacher, J. Appl. Phys. 39, 1996 (1968).

    Article  ADS  Google Scholar 

  3. E. Hegenbarth, Cryogenics 1, 242 (1961).

    Article  ADS  Google Scholar 

  4. W. N. Lawless, Phys. Rev. B 49, 433 (1977).

    Article  ADS  Google Scholar 

  5. A. S. Mischenko, Q. Zhang, J. F. Scott, R.W. Whatmore and N. D. Mathur, Science 311, 1270 (2006).

    Article  ADS  Google Scholar 

  6. A. S. Mischenko, Q. Zhang, R. W. Whatmore, J. F. Scott and N. D. Mathur, Appl. Phys. Lett. 89, 242912 (2006).

    Article  ADS  Google Scholar 

  7. O. Tegus, E. Brück, K. H. J. Buschow and F. R. D. Boer, Nature 415, 150 (2002).

    Article  ADS  Google Scholar 

  8. V. Provenzano, A. J. Shapiro and R. D. Shull, Nature 429, 853 (2004).

    Article  ADS  Google Scholar 

  9. H. Wada and Y. Tanabe, Appl. Phys. Lett. 79, 3320 (2001).

    Article  Google Scholar 

  10. A. Giguėre, M. Foldeaki, B. R. Gopal, R. Chahine, T. K. Bose, A. Frydman and J. A. Barclay, Phys. Rev. Lett. 83, 2262 (1999).

    Article  ADS  Google Scholar 

  11. T. Delage, C. Champeaux, A. Catherinot, J. F. Seaux, V. Madrangeas and D. Cros, Thin Solid Films 54, 279 (2004).

    Article  Google Scholar 

  12. F. Zimmermann, M. Voigts, C. Weil, R. Jakoby, P. Wang, W. Meneklou and E. Ivers-Tiffė, J. Eur. Ceram. Soc. 21, 2019 (2001).

    Article  Google Scholar 

  13. J. G. Cheng, X. J. Meng, J. Tang, S. L. Guo and J. H. Chu, Appl. Phys. Lett. 75, 3402 (1999).

    Article  ADS  Google Scholar 

  14. M. Tyunina and J. Levoska, Phys. Rev. B 70, 132105 (2004).

    Article  ADS  Google Scholar 

  15. Y. Yoneda, T. Okabe, K. Sakaue, H. Terauchi, H. Kasatani and Kiyoshi Deguchi, J. Appl. Phys. 83, 2458 (1998).

    Article  ADS  Google Scholar 

  16. S. Sawai, H. Tanaka, K. Morimoto, K. Hisano and T. Yamamoto, Ferroelectrics 242, 59 (2000).

    Article  Google Scholar 

  17. G. Branković, Z. Branković, M. S. Góes, C. O. Paiva-Santos, M. Cilense, J. A. Varela and E. Longo, Mater. Sci. Eng. B 122, 140 (2005).

    Article  Google Scholar 

  18. Y. Bai, G. Zheng and S. Shi, Appl. Phys. Lett. 96, 192902 (2010).

    Article  ADS  Google Scholar 

  19. H. Chen, T. L. Ren, X. M. Wu, Y. Yang and L. T. Liu, Appl. Phys. Lett. 94, 182902 (2009).

    Article  ADS  Google Scholar 

  20. Th. Michael, S. Trimper and J. M. Wesselinowa, Phys. Rev. B 74, 214113 (2006).

    Article  ADS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to N. Hur.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Park, Y.A., Sung, K.D., Jung, J.H. et al. Increased saturation field as the origin of the giant electrocaloric effect in Ba0.8Sr0.2TiO3 thin films. Journal of the Korean Physical Society 67, 551–555 (2015). https://doi.org/10.3938/jkps.67.551

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.3938/jkps.67.551

Keywords

Navigation