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Magnetic Properties of Proton Irradiated Fe2.7GeTe2 Bulk Crystals

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Abstract

van der Waals (vdW) magnetic materials show promise in being the foundation for future spintronic technology. The magnetic behavior of Fe2.7GeTe2 (FGT), a vdW itinerant ferromagnet, was investigated before and after proton irradiation. Proton irradiation of the sample was carried out at a fluence of 1×1018 cm-2. The magnetization measurements revealed a small increase of saturation magnetization (Ms) of about 4% upon proton irradiation of the sample, in which, the magnetic field was applied parallel to the c-axis. X-ray photoelectron spectroscopy for pristine and irradiated FGT revealed a general decrease in intensity after irradiation for Ge and Te and an increase in peak intensity of unavoidable surface iron oxide. Furthermore, no noticeable change in the Curie temperature (TC =152 K) is observed in temperature dependent magnetization variation. This work signifies the importance of employing protons in tuning the magnetic properties of vdW materials.

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Correspondence to S. R. Singamaneni.

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Olmos, R., Cosio, A., Saiz, C.L. et al. Magnetic Properties of Proton Irradiated Fe2.7GeTe2 Bulk Crystals. MRS Advances 4, 2185–2190 (2019). https://doi.org/10.1557/adv.2019.277

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  • DOI: https://doi.org/10.1557/adv.2019.277

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