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Two-Photon Exciton Absorption in CdSe/CdS Nanoplatelets Colloidal Solution

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Abstract

This work devotes to investigation of two-photon absorption in a colloidal solution of nanoplatelets CdSe/CdS (3.5 and 2 monolayers of CdSe core and CdS shell respectively) in the case of light- and heavy-hole exciton excitation (1lh-1e, 536 nm) and (1hh-1e, 578 nm) by femtosecond laser radiation (1064 nm, 100 kHz). An open-aperture z-scan technique was utilized to measure nonlinear two-photon absorption coefficient which was found as β = 0.08 ± 0.01 cm/GW, two-photon absorption cross sections σ(2) ≈ 1.5 × 106 GM and nonlinear refraction index γ ≈ –5 × 10–16 cm2/W. The revealed features of the measured z-scan dependencies can be the evidence of amplified spontaneous emission in the colloidal solution of CdSe/CdS nanoplatelets at high intensity of two-photon excitation.

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Funding

This work was supported by the state task and the Russian Foundation for Basic Research (project nos. 19-32-90240 and 19-03-00481(sample synthesis)).

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Authors and Affiliations

  1. Kotelnikov Institute of Radioengineering and Electronics of Russian Academy of Science, 125009, Moscow, Russia

    I. D. Laktaev, D. V. Przhiialkovskii, A. M. Smirnov & O. V. Butov

  2. Moscow State University, 119991, Moscow, Russia

    B. M. Saidzhonov, R. B. Vasiliev & A. M. Smirnov

Authors
  1. I. D. Laktaev
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  2. D. V. Przhiialkovskii
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  3. B. M. Saidzhonov
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  4. R. B. Vasiliev
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  5. A. M. Smirnov
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  6. O. V. Butov
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Corresponding authors

Correspondence to I. D. Laktaev, D. V. Przhiialkovskii, B. M. Saidzhonov, R. B. Vasiliev, A. M. Smirnov or O. V. Butov.

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Laktaev, I.D., Przhiialkovskii, D.V., Saidzhonov, B.M. et al. Two-Photon Exciton Absorption in CdSe/CdS Nanoplatelets Colloidal Solution. Semiconductors 54, 1900–1903 (2020). https://doi.org/10.1134/S1063782620140158

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  • DOI: https://doi.org/10.1134/S1063782620140158

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