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Hierarchical zeolites: synthesis, structural control, and catalytic applications

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Abstract

Zeolites possess unique ion exchange property, abundant acid sites, and highly hydrothermal stability, which have been widely used in catalysis, separation, and adsorption etc. However, the application of zeolite is greatly restrained in catalytic reactions involved in the large molecules due to their small micropore size (< 2 nm). Zeolites with hierarchically porous structure not only keep the crystalline framework, acidic sites, and highly hydrothermal stability but also improve diffusion of larger molecules. Thus, the catalyst life can be prolonged, which can expand their applications in the catalysis. In this review, the research progresses of hierarchical zeolites in terms of the controllable pore structural and synthetic strategy are summarized. Additionally, the applications of these hierarchical zeolites in catalysis are concluded. Furthermore, the hierarchical zeolites exhibit more excellent catalytic performance than conventional zeolite with sole micropores. Therefore, a perspective for promising application of the hierarchical zeolite in catalysis field is provided.

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Funding

This work was supported by the National Natural Science Foundation of China (21805155, 51772162, 51802171 and 21971132); Outstanding Youth Foundation of Shandong Province, China (ZR2019JQ14); Youth Innovation and Technology Foundation of Shandong Higher Education Institutions, China (2019KJC004); and Taishan Scholar Young Talent Program, Natural Science Foundation of Shandong Province, China (ZR2019MB042, ZR2018BB031).

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  1. Key Laboratory of Eco-chemical Engineering, Ministry of Education, College of Chemistry and Molecular Engineering, Qingdao University of Science and Technology, Qingdao, 266042, China

    Huiqi Qu, Yiru Ma & Lei Wang

  2. College of Materials Science and Engineering, Qingdao University of Science and Technology, Qingdao, 266042, China

    Bin Li

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  1. Huiqi Qu
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Qu, H., Ma, Y., Li, B. et al. Hierarchical zeolites: synthesis, structural control, and catalytic applications. emergent mater. 3, 225–245 (2020). https://doi.org/10.1007/s42247-020-00088-z

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