Abstract
A complete three-dimensional Proton Exchange Membrane Fuel Cell (PEMFC) model is proposed to study the influence of right-angle turn single serpentine (RAT1S), right-angle turn double serpentine (RAT2S), right-angle turn triple serpentine (RAT3S), and right-angle turn 3–2–1 serpentine (RAT321S) flow fields configuration on PEMFC performance with a commercial CFD code (ANSYS FLUENT). Simulations have been performed to envisage the pressure drop in the channel, the mass fraction of H2 and O2 along the anode and cathode channels, current flux density dispersion on the catalyst layer (CL), the membrane water content and proton conductivity as well as cell performance for proposed 4 flow field designs. A comparison of the simulation results of the four models was carried out. It has been found that the output of RAT321S flow field has improved compared to the RAT1S, RAT2S, and RAT3S flow field designs for the flow of the fixed-flow reactants, and RAT321S flow field model has been validated with experimental literature evidence. The results also show that the pressure drop losses are reduced as the number of passes increases.
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Abbreviations
- \(uV\) :
-
Velocity (ms−1)
- \(p\) :
-
Pressure (N m−2)
- \(w_{i}\) :
-
Species mass fraction i in the mixture
- \(D_{ij}\) :
-
Binary diffusion coefficient (m2s−1)
- \(k_{p}\) :
-
Permeability of GDL (m2)
- \(k_{s}^{\text{eff}}\) :
-
Ionic conductivity of solid phase (Sm−1)
- \(i_{a}\) :
-
Anode transfer current density (Am−2)
- \(i_{c}\) :
-
Cathode transfer current density (Am−2)
- \(C_{{{\text{H}}_{2} }}\) :
-
Hydrogen concentration (molm−3).
- \(C_{{{\text{O}}_{2} }}\) :
-
Oxygen concentration (molm−3).
- \(k_{e}\) :
-
Ionic conductivity of the membrane (Sm−1)
- \(C_{{{\text{H}}_{2} {\text{O}},a}}^{{{\text{MEM}}}}\) :
-
Membrane water concentration at anode (Jmol−1 K−1)
- \(C_{{{\text{H}}_{2} {\text{O}},c}}^{{{\text{MEM}}}}\) :
-
Membrane water concentration at cathode (Jmol−1 K−1)
- T:
-
Cell operating temperature (K)
- \(P_{s}\) :
-
Water saturation pressure (Pa)
- \(W_{{{\text{net}}}}\) :
-
Net power density (Wcm−2)
- \(W_{{{\text{cell}}}}\) :
-
Cell power density (Wcm−2)
- \(A_{{{\text{cha}}}}\) :
-
Cathode channel cross-sectional area
- \(N_{w}\) :
-
Net water flux across the membrane (kg m−2 s−1)
- \(n_{d}\) :
-
Electro-osmotic drag coefficient
- \(D_{w}\) :
-
Water diffusivity
- \(c_{w}\) :
-
Number of water molecules per sulfonic acid group
- \(\alpha_{a}\) :
-
Anode transfer coefficient
- \(\alpha_{c}\) :
-
Cathode transfer coefficient
- \(\emptyset_{s}\) :
-
Phase potential of solid
- \(\emptyset_{e}\) :
-
Phase potential at the electrolyte
- \(\Lambda\) :
-
Water content in the membrane
- \(\eta\) :
-
Dynamic viscosity (kg m−1 s−1)
- \(\eta_{a}\) :
-
Anode potential difference
- \(\eta_{c}\) :
-
Cathode potential difference
- \(\rho\) :
-
Density (kg m−3)
- MEM:
-
Membrane
- ref:
-
Reference
- eff:
-
Effective
References
Caglayan, D.G.; Sezgin, B.; Devrim, Y.; Eroglu, I.: Three-dimensional modeling of a high-temperature polymer electrolyte membrane fuel cell at different operation temperatures. Int. J. Hydrog. Energy 41(23), 10060–10070 (2016). https://doi.org/10.1016/j.ijhydene.2016.03.049
Berning, T.; Lu, D.M.; Djilali, N.: Three-dimensional computational analysis of transport phenomena in a PEM fuel cell. J. Power Sour. 106(1), 284–294 (2002). https://doi.org/10.1016/S0378-7753(01)01057-6
Nguyen, P.T.; Berning, T.; Djilali, N.: Computational model of a PEM fuel cell with serpentine gas flow channels. J. Power Sour. 130(1–2), 149–157 (2004). https://doi.org/10.1016/j.jpowsour.2003.12.027
Li, X.; Sabir, I.; Park, J.: A flow channel design procedure for PEM fuel cells with effective water removal. J. Power Sour. 163(2), 933–942 (2007). https://doi.org/10.1016/j.jpowsour.2006.10.015
Jeon, D.H.; Greenway, S.; Shimpalee, S.Ã.; Van Zee, J.W.; Van Zee, J.W.: The effect of serpentine flowfield designs on PEM fuel cell performance. Int. J. Hydrog. Energy 33(3), 1052–1066 (2008). https://doi.org/10.1016/j.ijhydene.2007.11.015
Wang, X.D.; Duan, Y.Y.; Yan, W.M.; Peng, X.F.: Local transport phenomena and cell performance of PEM fuel cells with various serpentine flow field designs. J. Power Sour. 175(1), 397–407 (2008). https://doi.org/10.1016/j.jpowsour.2007.09.009
Jang, J.-H.; Yan, W.-M.; Li, H.-Y.; Tsai, W.-C.: Three-dimensional numerical study on cell performance and transport phenomena of PEM fuel cells with conventional flow fields. Int. J. Hydrog. Energy 33(1), 156–164 (2008). https://doi.org/10.1016/j.ijhydene.2007.09.005
Carcadea, E., et al.: A computational fluid dynamics analysis of a PEM fuel cell system for power generation. Int. J. Numer. Methods Heat Fluid Flow 17(3), 302–312 (2007). https://doi.org/10.1108/09615530710730166
Akbari, M.H.; Rismanchi, B.: Numerical investigation of flow field configuration and contact resistance for PEM fuel cell performance. Renew. Energy 33(8), 1775–1783 (2008). https://doi.org/10.1016/j.renene.2007.10.009
Chang, D.H.; Wu, S.Y.: The effects of channel depth on the performance of miniature proton exchange membrane fuel cells with serpentine-type flow fields. Int. J. Hydrog. Energy 40(35), 11659–11667 (2015). https://doi.org/10.1016/j.ijhydene.2015.04.153
Lakshminarayanan, V.; Karthikeyan, P.; Muthukumar, M.; Senthil Kumar, A.P.; Kavin, B.; Kavyaraj, A.: Numerical investigation of performance studies on single pass PEM fuel cell with various flow channel design. Appl. Mech. Mater. 592–594, 1672–1676 (2014). https://doi.org/10.4028/www.scientific.net/AMM.592-594.1672
Muthukumar, M.; Karthikeyan, P.; Lakshminarayanan, V.; Senthil Kumar, A.P.; Vairavel, M.; Girimurugan, R.: Performance studies on PEM Fuel cell with 2, 3 and 4 pass serpentine flow field designs. Appl. Mech. Mater. 592–594, 1728–1732 (2014). https://doi.org/10.4028/www.scientific.net/AMM.592-594.1728
Khazaee, I.; Sabadbafan, H.: Numerical study of changing the geometry of the flow field of a PEM fuel cell. Heat Mass Transf. und Stoffuebertragung 52(5), 993–1003 (2016). https://doi.org/10.1007/s00231-015-1621-4
Ruan, H.; Wu, C.; Liu, S.; Chen, T.: Design and simulation of novel flow field plate geometry for proton exchange membrane fuel cells. Heat Mass Transf. 52(10), 2167–2176 (2016). https://doi.org/10.1007/s00231-015-1737-6
Vijayakrishnan, M.K.; Palaniswamy, K.; Ramasamy, J.; Kumaresan, T.; Manoharan, K.; Rajagopal, T.K.R.; Yi, S.C.: Numerical and experimental investigation on 25 cm2 and 100 cm2 PEMFC with novel sinuous flow field for effective water removal and enhanced performance. Int. J. Hydrog. Energy 45(13), 7848–7862 (2020)
Kerkoub, Y.; Benzaoui, A.; Haddad, F.; Ziari, Y.K.: Channel to rib width ratio influence with various flow field designs on performance of PEM fuel cell. Energy Convers. Manag. 174, 260–275 (2018). https://doi.org/10.1016/j.enconman.2018.08.041
Ghanbarian, A.; Kermani, M.J.; Scholta, J.; Abdollahzadeh, M.: Polymer electrolyte membrane fuel cell flow field design criteria application to parallel serpentine flow patterns. Energy Convers. Manag. 166, 281–296 (2018). https://doi.org/10.1016/j.enconman.2018.04.018
Suresh, P.V.; Jayanti, S.; Deshpande, A.P.; Haridoss, P.: An improved serpentine flow field with enhanced crossflow for fuel cell applications. Int. J. Hydrog. Energy 36, 6067–6072 (2011)
Liu, H.; Li, P.; Juarez-robles, D.; Wang, K.; Hernandez-guerrero, A.: Experimental study and comparison of various designs of gas flow fields to PEM fuel cells and cell stack performance. Front. Energy Res. (2014). https://doi.org/10.3389/fenrg.2014.00002
Li, W.; Zhang, Q.; Wang, C.; Yan, X.; Shen, S.; Xia, G.; Zhang, J.: Experimental and numerical analysis of a three-dimensional flow field for PEMFCs. Appl. Energy 195, 278–288 (2017)
Rahimi-Esbo, M.; Ramiar, A.; Ranjbar, A.A.; Alizadeh, E.: Design, manufacturing, assembling and testing of a transparent PEM fuel cell for investigation of water management and contact resistance at dead-end mode. Int. J. Hydrog. Energy 42(16), 11673–11688 (2017)
Xu, C.; Zhao, T.S.: A new flow field design for polymer electrolyte-based fuel cells. Electrochem. Commun. 9, 497–503 (2007)
Manso, A.P.; Marzo, F.F.; Barranco, J.; Garikano, X.; Garmendia, M.M.: Influence of geometric parameters of the flow fields on the performance of a PEM fuel cell a review. Int J Hydrog. Energy 37, 15256–15287 (2012)
Min, C.H.: Performance of a proton exchange membrane fuel cell with a stepped flow field design. J Power Sour. 186(2), 370e6 (2009)
Jang, J.H.; Yan, W.M.; Li, H.Y.; Chou, Y.C.: Humidity of reactant fuel on the cell performance of PEM fuel cell with baffle-blocked flow field designs. J Power Sour. 159(1), 468e77 (2006)
Yin, Y.; Wang, X.; Shangguan, X.; Zhang, J.; Qin, Y.: Numerical investigation on the characteristics of mass transport and performance of PEMFC with baffle plates installed in the flow channel. Int J Hydrog. Energy 43(16), 8048e62 (2018)
Barati, S.; Khoshandam, B.; Ghazi, M.M.: An investigation of channel blockage effects on hydrogen mass transfer in a proton exchange membrane fuel cell with various geometries and optimization by response surface methodology. Int J Hydrog. Energy 43(48), 21928e39 (2018)
Wang, X.D.; Duan, Y.Y.; Yan, W.M.: Novel serpentine-baffle flow field design for proton exchange membrane fuel cells. J Power Sour. 173(1), 210e21 (2007)
Manso, A.P.; Marzo, F.F.; Barranco, J.; Garikano, X.; Mujika, M.G.: Influence of geometric parameters of the flow fields on the performance of a PEM fuel cell a review. Int. J. Hydrog. Energy 37(20), 15256–15287 (2012)
Lim, B.H.; Majlan, E.H.; Daud, W.R.W.; Husaini, T.; Rosli, M.I.: Effects of flow field design on water management and reactant distribution in PEMFC: a review. Ionics 22(3), 301–316 (2016)
Anderson, R.; Zhang, L.; Ding, Y.; Blanco, M.; Bi, X.; Wilkinson, D.P.: A critical review of two-phase flow in gas flow channels of proton exchange membrane fuel cells. J. Power Sour. 195(15), 4531–4553 (2010)
Wang, J.: Theory and practice of flow field designs for fuel cell scaling-up: a critical review. Appl. Energy 157, 640–663 (2015)
Salva, J.A.; Iranzo, A.; Rosa, F.; Tapia, E.: Validation of cell voltage and water content in a PEM (polymer electrolyte membrane) fuel cell model using neutron imaging for different operating conditions. Energy 101, 100–112 (2016). https://doi.org/10.1016/j.energy.2016.02.006
Iranzo, A.; Muñoz, M.; Rosa, F.; Pino, J.: Numerical model for the performance prediction of a PEM fuel cell. Model results and experimental validation. Int. J. Hydrog. Energy 35(20), 11533–11550 (2010). https://doi.org/10.1016/j.ijhydene.2010.04.129
Saripella, B.P.; Koylu, U.O.; Leu, M.C.: Experimental and computational evaluation of performance and water management characteristics of a bio-inspired proton exchange membrane fuel cell. J. Fuel Cell Sci. Technol. 12(6), 061007 (2015). https://doi.org/10.1115/1.4032041
Li, Y.-S.; Han, Y.; Zhan, J.-M.: Uniformity analysis in different flowfield configurations of proton exchange membrane fuel cell. J. Fuel Cell Sci. Technol. 10(3), 031003 (2013). https://doi.org/10.1115/1.4024252
Velisala, V.; Srinivasulu, G.N.: Numerical simulation and experimental comparison of single, double and triple serpentine flow channel configuration on performance of a PEM fuel cell. Arab. J. Sci. Eng. 43(3), 1225–1234 (2017)
Iranzo, A.; Muñoz, M.; López, E.; Pino, J.; Rosa, F.: Experimental fuel cell performance analysis under different operating conditions and bipolar plate designs. Int. J. Hydrog. Energy 35(20), 11437–11447 (2010). https://doi.org/10.1016/j.ijhydene.2010.05.056
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Velisala, V., Pullagura, G., Yarramsetty, N. et al. Three-Dimensional CFD Modeling of Serpentine Flow Field Configurations for PEM Fuel Cell Performance. Arab J Sci Eng 46, 11687–11700 (2021). https://doi.org/10.1007/s13369-021-05544-4
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DOI: https://doi.org/10.1007/s13369-021-05544-4